Point-contact spectroscopy of Al- and C-doped MgB2. Superconducting energy gaps and scattering studies

The two-band/two-gap superconductivity in aluminium and carbon doped MgB$_2$ has been addressed by the point-contact spectroscopy. Two gaps are preserved in all samples with $T_c's$ down to 22 K. The evolution of two gaps as a function of the critical temperature in the doped systems suggest the dominance of the band-filling effects but for the increased Al-doping the enhanced interband scattering approaching two gaps must be considered. The magnetic field dependences of the Andreev reflection excess currents as well as zero-energy density of states determined from the experimental data are used to analyze the intraband scattering. It is shown, that while the C-doping increases the intraband scattering in the $\pi$-band more rapidly then in the $\sigma$ band, the Al-doping does not change their relative weight.Comment: 8 pages, incl. 6 figure

Direct observation of Fe spin reorientation in single crystalline YbFe6Ge6

We have grown single crystals of YbFe6Ge6 and LuFe6Ge6 and characterized their anisotropic behaviour through low field magnetic susceptibility, field-dependent magnetization, resistivity and heat capacity measurements. The Yb+3 valency is confirmed by LIII XANES measurements. YbFe6Ge6 crystals exhibit a field-dependent, sudden reorientation of the Fe spins at about 63 K, a unique effect in the RFe6Ge6 family (R = rare earths) where the Fe ions order anti-ferromagnetically with Neel temperatures above 450 K and the R ions' magnetism appears to behave independently. The possible origins of this unusual behaviour of the ordered Fe moments in this compound are discussed.Comment: 12 pages, 8 figures, accepted in J. Phys.: Cond. Matte

Intrinsic pinning on structural domains in underdoped single crystals of Ba(Fe1−x_{1-x}Cox_x)2_2As2_2

Critical current density was studied in single crystals of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ for the values of $x$ spanning the entire doping phase diagram. A noticeable enhancement was found for slightly underdoped crystals with the peak at $x = 0.058$. Using a combination of polarized-light imaging, x-ray diffraction and magnetic measurements we associate this behavior with the intrinsic pinning on structural domains in the orthorhombic phase. Domain walls extend throughout the sample thickness in the direction of vortices and act as extended pinning centers. With the increasing $x$ domain structure becomes more intertwined and fine due to a decrease of the orthorhombic distortion. This results in the energy landscape with maze-like spatial modulations favorable for pinning. This finding shows that iron-based pnictide superconductors, characterized by high values of the transition temperature, high upper critical fields, and low anisotropy may intrinsically have relatively high critical current densities.Comment: estimation of Jc correcte

Magnetic field-induced quantum critical point in YbPtIn and YbPt0.98_{0.98}In single crystals

Detailed anisotropic (H$\parallel$ab and H$\parallel$c) resistivity and specific heat measurements were performed on online-grown YbPtIn and solution-grown YbPt$_{0.98}$In single crystals for temperatures down to 0.4 K, and fields up to 140 kG; H$\parallel$ab Hall resistivity was also measured on the YbPt$_{0.98}$In system for the same temperature and field ranges. All these measurements indicate that the small change in stoichiometry between the two compounds drastically affects their ordering temperatures (T$_{ord}\approx3.4$ K in YbPtIn, and $\sim2.2$ K in YbPt$_{0.98}$In). Furthermore, a field-induced quantum critical point is apparent in each of these heavy fermion systems, with the corresponding critical field values of YbPt$_{0.98}$In (H$^{ab}_c$ around 35-45 kG and H$^{c}_c\approx120$ kG) also reduced compared to the analogous values for YbPtIn (H$^{ab}_c\approx60$ kG and H$^{c}_c>140$ kG

Temperature-dependent Hc2H_{c2} anisotropy in MgB2_2 as inferred from measurements on polycrystals

We present data on temperature-dependent anisotropy of the upper critical field of MgB$_2$ obtained from the analysis of measurements on high purity, low resistivity polycrystals. The anisotropy decreases in a monotonic fashion with increase of temperature

Anisotropic thermal expansion of Fe1.06Te and FeTe0.5Se0.5 single crystals

Heat capacity and anisotropic thermal expansion was measured for Fe1.06Te and FeTe0.5Se0.5 single crystals. Previously reported phase transitions are clearly seen in both measurements. In both cases the thermal expansion is anisotropic. The uniaxial pressure derivatives of the superconducting transition temperature in FeTe0.5Se0.5 inferred from the Ehrenfest relation have opposite signs for in-plane and c-axis pressures. Whereas the Gruneisen parameters for both materials are similar and only weakly temperature-dependent above ~ 80 K, at low temperatures (in the magnetically ordered phase) the magnetic contribution to the Gruneisen parameter in Fe1.06Te is significantly larger than electron and phonon contributions combined

Systematic study of the two band/two gap superconductivity in carbon-substituted MgB2 by point-contact spectroscopy

Point-contact measurements on the carbon-substituted Mg(B$_{1-x}$C$_x$)$_2$ filament/powder samples directly reveal a retention of the two superconducting energy gaps in the whole doping range from $x = 0$ to $x \approx 0.1$. The large gap on the $\sigma$-band is decreased in an essentially linear fashion with increasing the carbon concentrations. The changes in the the small gap $\Delta_{\pi}$ up to 3.8 % C are proportionally smaller and are more difficult to detect but for the heavily doped sample with $x \approx 0.1$ and $T_c = 22$ K both gaps are still present, and significantly reduced, consistent with a strong essentially linear, reduction of each gap with the transition temperature.Comment: 5 eps figure

Magnetoresistivity and Complete Hc2(T)H_{c2}(T) in MgB2MgB_2

Detailed magneto-transport data on dense wires of $MgB_2$ are reported for applied magnetic fields up to 18 T. The temperature and field dependencies of the electrical resistivity are consistent with $MgB_2$ behaving like a simple metal and following a generalized form of Kohler's rule. In addition, given the generally high $T_c$ values and narrow resistive transition widths associated with $MgB_2$ synthesized in this manner, combined with applied magnetic fields of up to 18 T, an accurate and complete $H_{c2}(T)$ curve could be determined. This curve agrees well with curves determined from lower field measurements on sintered pellets and wires of $MgB_2$. $H_{c2}(T)$ is linear in $T$ over a wide range of temperature (7 K $\le~T~\le$ 32 K) and has an upward curvature for $T$ close to $T_c$. These features are similar to other high $\kappa$, clean limit, boron-bearing intermetallics: $YNi_2B_2C$ and $LuNi_2B_2C$.Comment: minor changes in styl

Bose-Einstein condensation and entanglement in magnetic systems

We present a study of magnetic field induced quantum phase transitions in insulating systems. A generalized scaling theory is used to obtain the temperature dependence of several physical quantities along the quantum critical trajectory ($H=H_{C}$, $T\to0$) where $H$ is a longitudinal external magnetic field and $H_{C}$ the critical value at which the transition occurs. We consider transitions from a spin liquid at a critical field $H_{C1}$ and from a fully polarized paramagnet, at $H_{C2}$, into phases with long range order in the transverse components. The transitions at $H_{C1}$ and $H_{C2}$ can be viewed as Bose-Einstein condensations of magnons which however belong to different universality classes since they have different values of the dynamic critical exponent $z$. Finally, we use that the magnetic susceptibility is an entanglement witness to discuss how this type of correlation sets in as the system approaches the quantum critical point along the critical trajectory, $H=H_{C2}$, $T\to0$.Comment: 7 pages, 1 Table; accepted version; changes in text and new reference

Thermoelectric power of Ba(Fe1-xRux)2As2 and Ba(Fe1-xCox)2As2: possible changes of Fermi surface with and without changes in electron count

Temperature-dependent, in-plane, thermoelectric power (TEP) data are presented for Ba(Fe1-xRux)2As2 (0 < x < 0.36) single crystals. The previously outlined x - T phase diagram for this system is confirmed. The analysis of TEP evolution with Ru-doping suggests significant changes in the electronic structure, correlations and/or scattering occurring near ~7% and ~30% of Ru-doping levels. These results are compared with an extended set of TEP data for the electron-doped Ba(Fe1-xCox)2As2 series