2 research outputs found
Electron-spin-resonance in the doped spin-Peierls compound Cu(1-x)Ni(x)GeO3
ESR-study of the Ni-doped spin-Peierls compound CuGeO3 has been performed in
the frequency range 9-75 GHz. At low temperatures the g-factor is smaller than
the value expected for Cu- and Ni-ions. This anomaly is explained by the
formation of magnetic clusters around the Ni-ions within a nonmagnetic
spin-Peierls matrix. The transition into the AFM-state detected earlier by
neutron scattering for doped samples was studied by means of ESR. For x=0.032 a
gap in the magnetic resonance spectrum is found below the Neel temperature and
the spectrum is well described by the theory of antiferromagnetic resonance
based on the molecular field approximation. For x=0.017 the spectrum below the
Neel point remained gapless. The gapless spectrum of the antiferromagnetic
state in weekly doped samples is attributed to the small value of the Neel
order parameter and to the magnetically disordered spin-Peierls background.Comment: 16 pages, LATEX, 12 figures, submitted to Journal of Physics :
Condensed Matte
Magnetic Resonance of the Intrinsic Defects of the Spin-Peierls Magnet CuGeO3
ESR of the pure monocrystals of CuGeO3 is studied in the frequency range 9-75
GHz and in the temperature interval 1.2-25 K. The splitting of the ESR line
into several spectral components is observed below 5 K, in the temperature
range where the magnetic susceptibility is suppressed by the spin-Peierls
dimerization. The analysis of the magnetic resonance signals allows one to
separate the signals of the S=1/2- and S=1 defects of the spin-Peierls phase.
The value of g-factor of these signals is close to that of the Cu-ion. The
additional line of the magnetic resonance is characterized by an anomalous
value of the g-factor and by the threshold-like increase of the microwave
susceptibility when the microwave power is increasing. The ESR signals are
supposingly attributed to two types of the planar magnetic defects, arising at
the boundaries of the domains of the spin-Peierls state with the different
values of the phase of the dimerization.Comment: LATEX-text, 12 PS-figures, typos corrected, LATEX-style change