250 research outputs found
Frustrated three-leg spin tubes: from spin 1/2 with chirality to spin 3/2
Motivated by the recent discovery of the spin tube
[(CuCltachH)Cl]Cl, we investigate the properties of a frustrated
three-leg spin tube with antiferromagnetic intra-ring and inter-ring couplings.
We pay special attention to the evolution of the properties from weak to strong
inter-ring coupling and show on the basis of extensive density matrix
renormalization group and exact diagonalization calculations that the system
undergoes a first-order phase transition between a dimerized gapped phase at
weak coupling that can be described by the usual spin-chirality model and a
gapless critical phase at strong coupling that can be described by an effective
spin-3/2 model. We also show that there is a magnetization plateau at 1/3 in
the gapped phase and slightly beyond. The implications for
[(CuCltachH)Cl]Cl are discussed, with the conclusion that this
system behaves essentially as a spin-3/2 chain.Comment: 8 pages, 9 figures, revised versio
Spin-1/2 frustrated antiferromagnet on a spatially anisotopic square lattice: contribution of exact diagonalizations
The phase diagram of a spin-1/2 model is investigated by means of
exact diagonalizations on finite samples. This model is a generalization of the
model on the square lattice with two different nearest-neighbor
couplings and may be also viewed as an array of coupled Heisenberg
chains. The results suggest that the resonnating valence bond state predicted
by Nersesyan and Tsvelik [Phys. Rev. B {\bf 67}, 024422 (2003)] for is realized and extends beyond the limit of small interchain coupling
along a curve nearly coincident with the line where the energy per spin is
maximum. This line is likely bordered on both side by a columnar dimer long
range order. This columnar order could extends for which correspond
to the model.Comment: 14 pages, 21 figures, final versio
On the valence-bond solid phase of the crossed-chain quantum spin model
Using a series expansion based on the flow-equation method we study the
ground state energy and the elementary triplet excitations of a generalized
model of crossed spin-1/2 chains starting from the limit of decoupled
quadrumers. The triplet dispersion is shown to be very sensitive to the
inter-quadrumer frustration, exhibiting a line of almost complete localization
as well as lines of quantum phase transitions limiting the stability of the
valence-bond solid phase. In the vicinity of the checkerboard-point a finite
window of exchange couplings is found with a non-zero spin-gap, consistent with
known results from exact diagonalization. The ground state energy is lower than
that of the bare quadrumer case for all exchange couplings investigated. In the
limiting situation of the fully frustrated checkerboard magnet our results
agree with earlier series expansion studies.Comment: 8 pages, 7 figure
Quantum Heisenberg antiferromagnet on low-dimensional frustrated lattices
Using a lattice-gas description of the low-energy degrees of freedom of the
quantum Heisenberg antiferromagnet on the frustrated two-leg ladder and bilayer
lattices we examine the magnetization process at low temperatures for these
spin models. In both cases the emergent discrete degrees of freedom implicate a
close relation of the frustrated quantum Heisenberg antiferromagnet to the
classical lattice gas with finite nearest-neighbor repulsion or, equivalently,
to the Ising antiferromagnet in a uniform magnetic field. Using this relation
we obtain analytical results for thermodynamically large systems in the
one-dimensional case. In the two-dimensional case we perform classical Monte
Carlo simulations for systems of up to sites.Comment: Submitted to Teoreticheskaya i Matematicheskaya Fizika (special issue
dedicated to the 90th anniversary of Professor Sergei Vladimirovich
Tyablikov
Motion of Bound Domain Walls in a Spin Ladder
The elementary excitation spectrum of the spin-
antiferromagnetic (AFM) Heisenberg chain is described in terms of a pair of
freely propagating spinons. In the case of the Ising-like Heisenberg
Hamiltonian spinons can be interpreted as domain walls (DWs) separating
degenerate ground states. In dimension , the issue of spinons as
elementary excitations is still unsettled. In this paper, we study two
spin- AFM ladder models in which the individual chains are
described by the Ising-like Heisenberg Hamiltonian. The rung exchange
interactions are assumed to be pure Ising-type in one case and Ising-like
Heisenberg in the other. Using the low-energy effective Hamiltonian approach in
a perturbative formulation, we show that the spinons are coupled in bound
pairs. In the first model, the bound pairs are delocalized due to a four-spin
ring exchange term in the effective Hamiltonian. The appropriate dynamic
structure factor is calculated and the associated lineshape is found to be
almost symmetric in contrast to the 1d case. In the case of the second model,
the bound pair of spinons lowers its kinetic energy by propagating between
chains. The results obtained are consistent with recent theoretical studies and
experimental observations on ladder-like materials.Comment: 12 pages, 7 figure
Clothianidin-resistant Anopheles gambiae adult mosquitoes from Yaoundé, Cameroon, display reduced susceptibility to SumiShield® 50WG, a neonicotinoid formulation for indoor residual spraying
Background:
Chronic exposure of mosquito larvae to pesticide residues and cross-resistance mechanisms are major drivers of tolerance to insecticides used for vector control. This presents a concern for the efficacy of clothianidin, an agricultural neonicotinoid prequalified for Indoor Residual Spraying (IRS).
Methods:
Using standard bioassays, we tested if reduced susceptibility to clothianidin can affect the efficacy of SumiShield® 50WG, one of four new IRS formulations containing clothianidin. We simultaneously monitored susceptibility to clothianidin and to SumiShield 50WG, testing adults of Anopheles gambiae, An. coluzzii and Culex sp sampled from urban, suburban and agricultural areas of Yaoundé, Cameroon.
Results:
We found that in this geographic area, the level of susceptibility to the active ingredient predicted the efficacy of SumiShield 50WG. This formulation was very potent against populations that reached 100% mortality within 72 h of exposure to a discriminating concentration of clothianidin. By contrast, mortality leveled off at 75.4 ± 3.5% within 7 days of exposure to SumiShield 50WG in An. gambiae adults collected from a farm where the spraying of the two neonicotinoids acetamiprid and imidacloprid for crop protection is likely driving resistance to clothianidin.
Conclusions:
Despite the relatively small geographic extend of the study, the findings suggest that cross-resistance may impact the efficacy of some new IRS formulations and that alternative compounds could be prioritized in areas where neonicotinoid resistance is emerging
Bond order from disorder in the planar pyrochlore magnet
We study magnetic order in the Heisenberg antiferromagnet on the checkerboard
lattice, a two-dimensional version of the pyrochlore network with strong
geometric frustration. By employing the semiclassical (1/S) expansion we find
that quantum fluctuations of spins induce a long-range order that breaks the
four-fold rotational symmetry of the lattice. The ordered phase is a
valence-bond crystal. We discuss similarities and differences with the extreme
quantum case S = 1/2 and find a useful phenomenology to describe the
bond-ordered phases.Comment: Minor clarifications + reference to an informal introduction
cond-mat/030809
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