1,039 research outputs found

    Natural orbits of atomic Cooper pairs in a nonuniform Fermi gas

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    We examine the basic mode structure of atomic Cooper pairs in an inhomogeneous Fermi gas. Based on the properties of Bogoliubov quasi-particle vacuum, the single particle density matrix and the anomalous density matrix share the same set of eigenfunctions. These eigenfunctions correspond to natural pairing orbits associated with the BCS ground state. We investigate these orbits for a Fermi gas in a spherical harmonic trap, and construct the wave function of a Cooper pair in the form of Schmidt decomposition. The issue of spatial quantum entanglement between constituent atoms in a pair is addressed.Comment: 14 pages, 4 figures, submitted to Phys. Rev.

    Morphology-controlled growth of magnetic iron oxide components on gold nanoparticles as bi-functional agents

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    Summary form only given. Hybrid nanostructure can inherit the physiochemical properties of its individual components to realize its multi-functionality. The coupling of plasmonic effect of gold nanoparticles with magnetic properties of iron oxide nanoparticles has shown great promise as bi-functional agents allowing simultaneous magnetic resonance imaging (MRI)/computed tomography (CT) imaging and magnetic/photonic thermal therapy. However, since gold and iron oxide are two dissimilar materials, the precise morphology and structure control for the hybrid nanostructure remains a great challenge, and there are few published studies on the correlation between composites morphologies and the optical/magnetic properties. In this work, we aim to fabricate gold/iron oxide hybrid nano-structures using less toxic precursors, control the morphology growth of iron oxide component on gold nanoparticles surface, and study the effects on optical and magnetic properties of final products. Here, nearly monodisperse gold/iron oxide hybrid nanoparticles were fabricated through thermal decomposition method. Spherical gold nanoparticles were pre-synthesized and used as seeds for the reduction of iron precursor to produce hybrid nanostructures. Various morphologies of iron oxide grown on the gold nanospheres surfaces were realized, including nano-shell, nano-octahedron, nano-flower, and dumbbell-shaped end. Pure gold nanospheres and iron oxide nanospheres were synthesized for comparison. The morphology and structure of obtained products were characterized by using TEM, EDX, electron diffraction pattern, and SEM. Their optical and magnetic properties were studied using UV-Vis spectroscopy and VSM. The plasmonic property of gold nanoparticles was shown to be affected by the optical index of its environment, and its absorbance peak was right-shifted after iron oxide shell coating. The gold/iron oxide dumbbell-shaped nanostructures displayed typical superparamagnetic behavior with no coerc- vity while the coercivity of gold/iron oxide nano-octahedron was about 45 Oe. The morphology-related blocking temperatures of the gold/iron oxide nano-structured samples were also studied through their ZFC/FC curves.postprin

    Effect of oxygen stoichiometry on microstructural and magnetic properties of FePt/TaOx bilayer fabricated by ion-beam-bombardment deposition

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    Temperature Induced Degradation of Nb Ti/Cu Composite Superconductors

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    The degradation mechanisms of state-of-the-art Nb-Ti/Cu superconductors are described, based on in-situ synchrotron X-ray diffraction measurements during heat treatment. A quantitative description of the Nb-Ti/Cu degradation in terms of critical current density, Cu stabiliser resistivity and mechanical composite strength is presented. In an applied magnetic field a significant critical current degradation is already observed after a 5-minute 400 °C heat treatment, due to variations of a-Ti precipitate size and distribution within the Nb-Ti alloy filaments. A strong degradation of the strand mechanical properties is observed after several minutes heating above 550 °C, which is also the temperature at which the formation of Cu Ti intermetallic phases is detected. Several minutes heating at 250 °C are sufficient to increase the RRR of the strongly cold work strands inside a Rutherford type cable from about 80 to about 240. Heating for several minutes at 400 °C does not cause a significant conductor degradation in self-field and, thus, leaves enough temperature margin for the electrical interconnection of Nb-Ti/Cu conductors with common low temperature solders

    Phase Transformations during the Reaction Heat Treatment

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    The evolution of Nb containing phases during the diffusion heat treatment of three different high critical current Nb3_{3}Sn strand types is compared, based on synchrotron X-ray diffraction results that have been obtained at the ID15 beam line of the European Synchrotron Radiation Facility (ESRF). In all strands studied, Nb3_{3}Sn formation is preceded by the formation of a Cu-Nb-Sn ternary phase, NbSn2 and Nb6Sn5. As compared to the PIT and Tube Type strand, the amount of these phases formed in the RRP strand is relatively small. In the RRP strand subelements with a fine filament structure Nb3_{3}Sn grows more quickly, thereby preventing to a large extent the formation of the other higher tin phases

    Nitrogen-Functionalized Graphene Nanoflakes (GNFs:N): Tunable Photoluminescence and Electronic Structures

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    This study investigates the strong photoluminescence (PL) and X-ray excited optical luminescence observed in nitrogen-functionalized 2D graphene nanoflakes (GNFs:N), which arise from the significantly enhanced density of states in the region of {\pi} states and the gap between {\pi} and {\pi}* states. The increase in the number of the sp2 clusters in the form of pyridine-like N-C, graphite-N-like, and the C=O bonding and the resonant energy transfer from the N and O atoms to the sp2 clusters were found to be responsible for the blue shift and the enhancement of the main PL emission feature. The enhanced PL is strongly related to the induced changes of the electronic structures and bonding properties, which were revealed by the X-ray absorption near-edge structure, X-ray emission spectroscopy, and resonance inelastic X-ray scattering. The study demonstrates that PL emission can be tailored through appropriate tuning of the nitrogen and oxygen contents in GNFs and pave the way for new optoelectronic devices.Comment: 8 pages, 6 figures (including toc figure

    X-ray absorption spectroscopy study of diluted magnetic semiconductors: Zn1-xMxSe (M = Mn, Fe, Co) and Zn1-xMnxY (Y = Se, Te)

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    We have investigated 3d electronic states of doped transition metals in II-VI diluted magnetic semiconductors, Zn1-xMxSe (M = Mn, Fe, Co) and Zn1-xMnxY (Y = Se, Te), using the transition-metal L2,3-edge X-ray absorption spectroscopy (XAS) measurements. In order to explain the XAS spectra, we employed a tetragonal cluster model calculation, which includes not only the full ionic multiplet structure but also configuration interaction (CI). The results show that CI is essential to describe the experimental spectra adequately, indicating the strong hybridization between the transition metal 3d and the ligand p orbitals. In the study of Zn1-xMnxY (Y = Se, Te), we also found considerable spectral change in the Mn L2,3-edge XAS spectra for different ligands, confirming the importance of the hybridization effects in these materials.Comment: This paper consists of 22 pages including 4 figures. This paper is submitted to Physical Review
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