Substitution Effect by Deuterated Donors on Superconductivity in κ\kappa-(BEDT-TTF)2_2Cu[N(CN)2_2]Br

We investigate the superconductivity in the deuterated BEDT-TTF molecular substitution system $\kappa$-[(h8-BEDT-TTF)$_{1-x}$(d8-BEDT-TTF)$_x$]$_2$Cu[N(CN)$_2$]Br, where h8 and d8 denote fully hydrogenated and deuterated molecules, respectively. Systematic and wide range ($x$ = 0 -- 1) substitution can control chemical pressure finely near the Mott boundary, which results in the modification of the superconductivity. After cooling slowly, the increase of $T_{\textrm{c}}$ observed up to $x \sim$ 0.1 is evidently caused by the chemical pressure effect. Neither reduction of $T_{\textrm{c}}$ nor suppression of superconducting volume fraction is found below $x \sim$ 0.5. This demonstrates that the effect of disorder by substitution is negligible in the present system. With further increase of $x$, both $T_{\textrm{c}}$ and superconducting volume fraction start to decrease toward the values in $x$ = 1.Comment: J. Phys. Soc. Jp

Debye relaxation in high magnetic fields

Dielectric relaxation is universal in characterizing polar liquids and solids, insulators, and semiconductors, and the theoretical models are well developed. However, in high magnetic fields, previously unknown aspects of dielectric relaxation can be revealed and exploited. Here, we report low temperature dielectric relaxation measurements in lightly doped silicon in high dc magnetic fields B both parallel and perpendicular to the applied ac electric field E. For B//E, we observe a temperature and magnetic field dependent dielectric dispersion e(w)characteristic of conventional Debye relaxation where the free carrier concentration is dependent on thermal dopant ionization, magnetic freeze-out, and/or magnetic localization effects. However, for BperpE, anomalous dispersion emerges in e(w) with increasing magnetic field. It is shown that the Debye formalism can be simply extended by adding the Lorentz force to describe the general response of a dielectric in crossed magnetic and electric fields. Moreover, we predict and observe a new transverse dielectric response EH perp B perp E not previously described in magneto-dielectric measurements. The new formalism allows the determination of the mobility and the ability to discriminate between magnetic localization/freeze out and Lorentz force effects in the magneto-dielectric response.Comment: 19 pages, 6 figure

A bulk 2D Pauli Limited Superconductor

We present a nearly perfect Pauli-limited critical field phase diagram for the anisotropic organic superconductor \$\alpha$-(ET)$_2$NH$_4$(SCN)$_4$ when the applied magnetic field is oriented parallel to the conducting layers. The critical fields ({H_{c_2}) were found by use of penetration depth measurements. Because {H_{c_2} is Pauli-limited, the size of the superconducting energy gap can be calculated. The role of spin-orbit scattering and many-body effects play a role in explaining our measurements.Comment: 4 pages, 5 figures. V5, corrections were made to the text, present data was include

Superconductivity in an organic insulator at very high magnetic fields

We investigate by electrical transport the field-induced superconducting state (FISC) in the organic conductor $\lambda$-(BETS)$_2$FeCl$_4$. Below 4 K, antiferromagnetic-insulator, metallic, and eventually superconducting (FISC) ground states are observed with increasing in-plane magnetic field. The FISC state survives between 18 and 41 T, and can be interpreted in terms of the Jaccarino-Peter effect, where the external magnetic field {\em compensates} the exchange field of aligned Fe$^{3+}$ ions. We further argue that the Fe$^{3+}$ moments are essential to stabilize the resulting singlet, two-dimensional superconducting stateComment: 9 pages 3 figure

Critical State Behaviour in a Low Dimensional Metal Induced by Strong Magnetic Fields

We present the results of magnetotransport and magnetic torque measurements on the alpha-(BEDT-TTF)2KHg(SCN)4 charge-transfer salt within the high magnetic field phase, in magnetic fields extending to 33 T and temperatures as low as 27 mK. While the high magnetic field phase (at fields greater than ~ 23 T) is expected, on theoretical grounds, to be either a modulated charge-density wave phase or a charge/spin-density wave hybrid, the resistivity undergoes a dramatic drop below ~ 3 K within the high magnetic field phase, falling in an approximately exponential fashion at low temperatures, while the magnetic torque exhibits pronounced hysteresis effects. This hysteresis, which occurs over a broad range of fields, is both strongly temperature-dependent and has several of the behavioural characteristics predicted by critical-state models used to describe the pinning of vortices in type II superconductors in strong magnetic fields. Thus, rather than exhibiting the usual behaviour expected for a density wave ground state, both the transport and the magnetic properties of alpha-(BEDT-TTF)2KHg(SCN)4, at high magnetic fields, closely resembles those of a type II superconductor