Electrical Noise From Phase Separation In Pr2/3Ca1/3MnO3 Single Crystal

Low frequency electrical noise measurements have been used to probe the electronic state of the perovskite-type manganese oxide Pr2/3Ca1/3MnO3 versus temperature and in the vicinity of the field-induced transition from the insulating, charge-ordered state (I-CO) to the metallic, ferromagnetic state (M-F). At high temperature we have observed a high level of the excess noise with mainly a gaussian distribution of the resistance fluctuations, and the associated power spectral density has a standard 1/f dependence. However, in the hysteretic region, where the electrical resistance depends dramatically on the sample history, we have observed a huge non-gaussian noise characterized by two level fluctuator-like switching (TLS) in the time domain. We discuss the origin of the noise in terms of percolative behavior of the conductivity. We speculate that the dominant fluctuators are manganese clusters switching between the M-F and the I-CO phases.Comment: RevTeX, 6 pages with 3 figure

Precision microwave dielectric and magnetic susceptibility measurements of correlated electronic materials using superconducting cavities

We analyze microwave cavity perturbation methods, and show that the technique is an excellent, precision method to study the dynamic magnetic and dielectric response in the $GHz$ frequency range. Using superconducting cavities, we obtain exceptionally high precision and sensitivity for measurements of relative changes. A dynamic electromagnetic susceptibility $\tilde{\zeta}(T)=\zeta ^{\prime}+i\zeta ^{\prime \prime}$ is introduced, which is obtained from the measured parameters: the shift of cavity resonant frequency $\delta f$ and quality factor $Q$. We focus on the case of a spherical sample placed at the center of a cylindrical cavity resonant in the $TE_{011}$ mode. Depending on the sample characteristics, the magnetic permeability $\tilde{\mu}$, the dielectric permittivity $\tilde{\epsilon}$ and the complex conductivity $\tilde{\sigma}$ can be extracted from $\tilde{\zeta}_{H}$. A full spherical wave analysis of the cavity perturbation is given. This analysis has led to the observation of new phenomena in novel low dimensional materials.Comment: 16 pages, 5 figure

Inversion symmetry in the spin-Peierls compound NaV2O5

At room-temperature NaV2O5 was found to have the centrosymmetric space group Pmmn. This space group implies the presence of only one kind of V site in contrast with previous reports of the non-centrosymmetric counterpart P21mn. This indicates a non-integer valence state of vanadium. Furthermore, this symmetry has consequences for the interpretation of the transition at 34 K, which was ascribed to a spin-Peierls transition of one dimensional chains of V4+.Comment: Revtex, 3 pages, 2 postscript pictures embedded in the text. Corrected a mistake in one pictur

Amorphous ferromagnetism and re-entrant magnetic glassiness in Sm2_{2}Mo2_{2}O7_{7}: new insights into the electronic phase diagram of pyrochlore molybdates

We discuss the magnetic properties of a Sm$_{2}$Mo$_{2}$O$_{7}$ single crystal as investigated by means of different experimental techniques. In the literature, a conventional itinerant ferromagnetic state is reported for the Mo$^{4+}$ sublattice below $\sim 78$ K. However, our results of dc magnetometry, muon spin spectroscopy ($\mu^{+}$SR) and high-harmonics magnetic ac susceptibility unambiguously evidence highly disordered conditions in this phase, in spite of the crystalline and chemical order. This disordered magnetic state shares several common features with amorphous ferromagnetic alloys. This scenario for Sm$_{2}$Mo$_{2}$O$_{7}$ is supported by the anomalously high values of the critical exponents, as mainly deduced by a scaling analysis of our dc magnetization data and confirmed by the other techniques. Moreover, $\mu^{+}$SR detects a significant static magnetic disorder at the microscopic scale. At the same time, the critical divergence of the third-harmonic component of the ac magnetic susceptibility around $\sim 78$ K leads to additional evidence towards the glassy nature of this magnetic phase. Finally, the longitudinal relaxation of $\mu^{+}$ spin polarization (also supported by results of ac susceptibility) evidences re-entrant glassy features similar to amorphous ferromagnets.Comment: 15 pages, 13 figure

Does EELS haunt your photoemission measurements?

It has been argued in a recent paper by R. Joynt (R. Joynt, Science 284, p 777 (1999)) that in the case of poorly conducting solids the photoemission spectrum close to the Fermi Energy may be strongly influenced by extrinsic loss processes similar to those occurring in High Resolution Electron Energy Loss Spectroscopy (HR-EELS), thereby obscuring information concerning the density of states or one electron Green's function sought for. In this paper we present a number of arguments, both theoretical and experimental, that demonstrate that energy loss processes occurring once the electron is outside the solid, contribute only weakly to the spectrum and can in most cases be either neglected or treated as a weak structureless background.Comment: 6 pages, figures included. Submitted to PR