The Cranked Nilsson-Strutinsky versus the Spherical Shell Model: A Comparative Study of pf-Shell Nuclei

A comparative study is performed of a deformed mean field theory, represented by the cranked Nilsson-Strutinsky (CNS) model, and the spherical shell model. Energy spectra, occupation numbers, B(E2)-values, and spectroscopic quadrupole moments in the light pf shell nuclei are calculated in the two models and compared. The result is also compared to available experimental data which are generally well described by the shell model. Although the Nilsson-Strutinsky calculation does not include pairing, both the subshell occupation numbers and quadrupole properties are found to be rather similar in the two models. It is also shown that ``unpaired'' shell model calculations produce very similar energies as the CNS at all spins. The role of the pairing energy in the description of backbending and signature splitting in odd-mass nuclei is also discussed.Comment: 14 pages, 20 figures, submitted to Phys.Rev.

Hydrated-electron population dynamics

A detailed frequency-resolved pump-probe study of hydrated electron dynamics, performed with 5-fs pulses, is presented. We show that the experimental data can be successfully described with a model in which the excited state lifetime is similar to50 fs in regular water and similar to70 A in heavy water. The deuteration effect on the lifetime strongly suggests that OH-vibrational modes in the first solvation shell act as accepting modes for energy relaxation. (C) 2004 Elsevier B.V. All rights reserved