2,233 research outputs found
Exciton and negative trion dissociation by an external electric field in vertically coupled quantum dots
We study the Stark effect for an exciton confined in a pair of vertically
coupled quantum dots. A single-band approximation for the hole and a parabolic
lateral confinement potential are adopted which allows for the separation of
the lateral center-of-mass motion and consequently for an exact numerical
solution of the Schr\"odinger equation. We show that for intermediate tunnel
coupling the external electric field leads to the dissociation of the exciton
via an avoided crossing of bright and dark exciton energy levels which results
in an atypical form of the Stark shift. The electric-field-induced dissociation
of the negative trion is studied using the approximation of frozen lateral
degrees of freedom. It is shown that in a symmetric system of coupled dots the
trion is more stable against dissociation than the exciton. For an asymmetric
system of coupled dots the trion dissociation is accompanied by a positive
curvature of the recombination energy line as a function of the electric field.Comment: PRB - in prin
Ultrafast optical control of entanglement between two quantum dot spins
The interaction between two quantum bits enables entanglement, the
two-particle correlations that are at the heart of quantum information science.
In semiconductor quantum dots much work has focused on demonstrating single
spin qubit control using optical techniques. However, optical control of
entanglement of two spin qubits remains a major challenge for scaling from a
single qubit to a full-fledged quantum information platform. Here, we combine
advances in vertically-stacked quantum dots with ultrafast laser techniques to
achieve optical control of the entangled state of two electron spins. Each
electron is in a separate InAs quantum dot, and the spins interact through
tunneling, where the tunneling rate determines how rapidly entangling
operations can be performed. The two-qubit gate speeds achieved here are over
an order of magnitude faster than in other systems. These results demonstrate
the viability and advantages of optically controlled quantum dot spins for
multi-qubit systems.Comment: 24 pages, 5 figure
Anomalous Stark Shifts in Single Vertically Coupled Pairs of InGaAs Quantum Dots
Vertically coupled Stranski Krastanow QDs are predicted to exhibit strong
tunnelling interactions that lead to the formation of hybridised states. We
report the results of investigations into single pairs of coupled QDs in the
presence of an electric field that is able to bring individual carrier levels
into resonance and to investigate the Stark shift properties of the excitons
present. Pronounced changes in the Stark shift behaviour of exciton features
are identified and attributed to the significant redistribution of the carrier
wavefunctions as resonance between two QDs is achieved. At low electric fields
coherent tunnelling between the two QD ground states is identified from the
change in sign of the permanent dipole moment and dramatic increase of the
electron polarisability, and at higher electric fields a distortion of the
Stark shift is attributed to a coherent tunnelling effect between the ground
state of the upper QD and the excited state of the lower QD.Comment: Conference paper for QD2004 3 figure
High-finesse optical quantum gates for electron spins in artificial molecules
A doped semiconductor double-quantum-dot molecule is proposed as a qubit
realization. The quantum information is encoded in the electron spin, thus
benefiting from the long relevant decoherence times; the enhanced flexibility
of the molecular structure allows to map the spin degrees of freedom onto the
orbital ones and vice versa, and opens the possibility for high-finesse
(conditional and unconditional) quantum gates by means of stimulated Raman
adiabatic passage.Comment: To appear in Phys. Rev. Let
Single and vertically coupled type II quantum dots in a perpendicular magnetic field: exciton groundstate properties
The properties of an exciton in a type II quantum dot are studied under the
influence of a perpendicular applied magnetic field. The dot is modelled by a
quantum disk with radius , thickness and the electron is confined in the
disk, whereas the hole is located in the barrier. The exciton energy and
wavefunctions are calculated using a Hartree-Fock mesh method. We distinguish
two different regimes, namely (the hole is located at the radial
boundary of the disk) and (the hole is located above and below the
disk), for which angular momentum transitions are predicted with
increasing magnetic field. We also considered a system of two vertically
coupled dots where now an extra parameter is introduced, namely the interdot
distance . For each and for a sufficient large magnetic field,
the ground state becomes spontaneous symmetry broken in which the electron and
the hole move towards one of the dots. This transition is induced by the
Coulomb interaction and leads to a magnetic field induced dipole moment. No
such symmetry broken ground states are found for a single dot (and for three
vertically coupled symmetric quantum disks). For a system of two vertically
coupled truncated cones, which is asymmetric from the start, we still find
angular momentum transitions. For a symmetric system of three vertically
coupled quantum disks, the system resembles for small the pillar-like
regime of a single dot, where the hole tends to stay at the radial boundary,
which induces angular momentum transitions with increasing magnetic field. For
larger the hole can sit between the disks and the state
remains the groundstate for the whole -region.Comment: 11 pages, 16 figure
Resonant optical pumping of a Mn spin in a strain free quantum dot
We report on the spin properties of individual Mn atoms in II-VI
semiconductor strain free quantum dots. Strain free Mn-doped CdTe quantum dots
are formed by width fluctuations in thin quantum wells lattice matched on a
CdTe substrate. These quantum dots permit to optically probe and address any
spin state of a Mn atom in a controlled strain environment. The absence of
strain induced magnetic anisotropy prevents an optical pumping of the Mn spin
at zero magnetic field. Thus, a large photoluminescence is obtained under
resonant optical excitation of the exciton-Mn complex. An efficient optical
pumping of the coupled electronic and nuclear spins of the Mn is restored under
a weak magnetic field. The observed reduction of the resonant photoluminescence
intensity under magnetic field is well described by a model including the
hyperfine coupling and a residual crystal field splitting of the Mn atom.
Finally, we show that the second order correlation function of the resonant
photoluminescence presents a large photon bunching at short delay which is a
probe of the dynamics of coupled electronic and nuclear spins of the Mn atom
Direct observation of acoustic phonon mediated relaxation between coupled exciton states in a single quantum dot molecule
We probe acoustic phonon mediated relaxation between tunnel coupled exciton
states in an individual quantum dot molecule in which the inter-dot quantum
coupling and energy separation between exciton states is continuously tuned
using static electric field. Time resolved and temperature dependent optical
spectroscopy are used to probe inter-level relaxation around the point of
maximum coupling. The radiative lifetimes of the coupled excitonic states can
be tuned from ~2 ns to ~10 ns as the spatially direct and indirect character of
the wavefunction is varied by detuning from resonance. Acoustic phonon mediated
inter-level relaxation is shown to proceed over timescales comparable to the
direct exciton radiative lifetime, indicative of a relaxation bottleneck for
level spacings in the range $\Delta E\$ ~3-6 meV.Comment: 6 pages, 4 figures, submitted for publicatio
Influence of the charge carrier tunneling processes on the recombination dynamics in single lateral quantum dot molecules
We report on the charge carrier dynamics in single lateral quantum dot
molecules and the effect of an applied electric field on the molecular states.
Controllable electron tunneling manifests itself in a deviation from the
typical excitonic decay behavior which is strongly influenced by the tuning
electric field and inter-molecular Coulomb energies. A rate equation model is
developed to gain more insight into the charge transfer and tunneling
mechanisms. Non-resonant (phonon-mediated) electron tunneling which changes the
molecular exciton character from direct to indirect, and vice versa, is found
to be the dominant tunable decay mechanism of excitons besides radiative
recombination.Comment: 4 pages, 4 figure
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