Resonant Scattering of Surface Plasmon Polaritons by Dressed Quantum Dots

The resonant scattering of surface plasmon-polariton waves by embedded semiconductor quantum dots above the dielectric/metal interface is explored in the strong-coupling regime. In contrast to non-resonant scattering by a localized dielectric surface defect, a strong resonant peak in the scattering field spectrum is predicted and accompanied by two side valleys. The peak height depends nonlinearly on the amplitude of surface plasmon-polariton waves, reflecting the feedback dynamics from a photon-dressed electron-hole plasma inside the quantum dots. This unique behavior in the scattering field peak strength is correlated with the occurrence of a resonant dip in the absorption spectrum of surface plasmon-polariton waves due to interband photon-dressing effect. Our result on the scattering of surface plasmon-polariton waves may be experimentally observable and applied to spatially selective illumination and imaging of individual molecules.Comment: 15 pages, 3 figure

Lifetime reduction of surface states at Cu, Ag and Au(111) caused by impurity scattering

We present density-functional results on the lifetime of the (111) surface state of the noble metals. We consider scattering on the Fermi surface caused by impurity atoms belonging to the 3d and 4sp series. The results are analyzed with respect to film thickness and with respect to separation of scattering into bulk or into surface states. While for impurities in the surface layer the overall trends are similar to the long-known bulk-state scattering, for adatom-induced scattering we find a surprising behavior with respect to the adatom atomic number. A plateau emerges in the scattering rate of the 3d adatoms, instead of a peak characteristic of the d resonance. Additionally, the scattering rate of 4sp adatoms changes in a zig-zag pattern, contrary to a smooth parabolic increase following Linde's rule that is observed in bulk. We interpret these results in terms of the weaker charge-screening and of interference effects induced by the lowering of symmetry at the surface

X-ray scattering from surfaces: discrete and continuous components of roughness

Incoherent surface scattering yields a statistical description of the surface, due to the ensemble averaging over many independently sampled volumes. Depending on the state of the surface and direction of the scattering vector relative to the surface normal, the height distribution is discrete, continuous, or a combination of the two. We present a treatment for the influence of multimodal surface height distributions on Crystal Truncation Rod scattering. The effects of a multimodal height distribution are especially evident during in situ monitoring of layer-by-layer thin-film growth via Pulsed Laser Deposition. We model the total height distribution as a convolution of discrete and continuous components, resulting in a broadly applicable parameterization of surface roughness which can be applied to other scattering probes, such as electrons and neutrons. Convolution of such distributions could potentially be applied to interface or chemical scattering. Here we find that this analysis describes accurately our experimental studies of SrTiO3 annealing and homoepitaxial growth.Comment: 15 pages, 7 figure

Dependence of resistivity on surface profile in nanoscale metal films and wires

We extend quantum models of nanowire surface scattering to incorporate bulk resistivity and extract an expression for the increased resistivity due to surface roughness. To learn how to improve conductivity, we calculate conductivity degradation from individual wavelengths of surface roughness, and show how these can be convolved to give resistivity for arbitrary surfaces. We review measurements from Cu films and conclude that roughness at short wavelengths (less than 100 nm) dominates scattering, and that primarily specular scattering should be achievable for RMS roughness below about 0.7 nm

Scattered light mapping of protoplanetary disks

High-contrast scattered light observations have revealed the surface morphology of several dozens of protoplanetary disks at optical and near-infrared wavelengths. Inclined disks offer the opportunity to measure part of the phase function of the dust grains that reside in the disk surface which is essential for our understanding of protoplanetary dust properties and the early stages of planet formation. We aim to construct a method which takes into account how the flaring shape of the scattering surface of an (optically thick) protoplanetary disk projects onto the image plane of the observer. This allows us to map physical quantities (scattering radius and scattering angle) onto scattered light images and retrieve stellar irradiation corrected (r^2-scaled) images and dust phase functions. We apply the method on archival polarized intensity images of the protoplanetary disk around HD 100546 that were obtained with VLT/SPHERE in R'-band and VLT/NACO in H- and Ks-band. The brightest side of the r^2-scaled R'-band polarized intensity image of HD 100546 changes from the far to the near side of the disk when a flaring instead of a geometrically flat disk surface is used for the r^2-scaling. The decrease in polarized surface brightness in the scattering angle range of ~40-70 deg is likely a result of the dust phase function and degree of polarization which peak in different scattering angle regimes. The derived phase functions show part of a forward scattering peak which indicates that large, aggregate dust grains dominate the scattering opacity in the disk surface. Projection effects of a protoplanetary disk surface need to be taken into account to correctly interpret scattered light images. Applying the correct scaling for the correction of stellar irradiation is crucial for the interpretation of the images and the derivation of the dust properties in the disk surface layer.Comment: Accepted for publication in A&A, 6 pages, 3 figure