Noncommutative optimal control and quantum networks

Optimal control is formulated based on a noncommutative calculus of operator derivatives. The use of optimal control methods in the design of quantum systems relies on the differentiation of an operator-valued function with respect to the relevant operator. Noncommutativity between the operator and its derivative leads to a generalization of the conventional method of control for classical systems. This formulation is applied to quantum networks of both spin and bosonic particles for the purpose of quantum state control via quantum random walks

Quantum control theory and applications: A survey

This paper presents a survey on quantum control theory and applications from a control systems perspective. Some of the basic concepts and main developments (including open-loop control and closed-loop control) in quantum control theory are reviewed. In the area of open-loop quantum control, the paper surveys the notion of controllability for quantum systems and presents several control design strategies including optimal control, Lyapunov-based methodologies, variable structure control and quantum incoherent control. In the area of closed-loop quantum control, the paper reviews closed-loop learning control and several important issues related to quantum feedback control including quantum filtering, feedback stabilization, LQG control and robust quantum control.Comment: 38 pages, invited survey paper from a control systems perspective, some references are added, published versio

Achieving robust and high-fidelity quantum control via spectral phase optimization

Achieving high-fidelity control of quantum systems is of fundamental importance in physics, chemistry and quantum information sciences. However, the successful implementation of a high-fidelity quantum control scheme also requires robustness against control field fluctuations. Here, we demonstrate a robust optimization method for control of quantum systems by optimizing the spectral phase of an ultrafast laser pulse, which is accomplished in the framework of frequency domain quantum optimal control theory. By incorporating a filtering function of frequency into the optimization algorithm, our numerical simulations in an abstract two-level quantum system as well as in a three-level atomic rubidium show that the optimization procedure can be enforced to search optimal solutions while achieving remarkable robustness against the control field fluctuations, providing an efficient approach to optimize the spectral phase of the ultrafast laser pulse to achieve a desired final quantum state of the system.Comment: 17 pages, 8 figure

Time optimal quantum control of two-qubit systems

We study the optimal quantum control of heteronuclear two-qubit systems described by a Hamiltonian containing both nonlocal internal drift and local control terms. We derive an explicit formula to compute the minimum time required to steer the system from an initial state to a specified final state. As applications the minimal time to implement Controlled-NOT gate, SWAP gate and Controlled-U gate is calculated in detail. The experimental realizations of these quantum gates are explicitly presented.Comment: 11 page

Singular extremals for the time-optimal control of dissipative spin 1/2 particles

We consider the time-optimal control by magnetic fields of a spin 1/2 particle in a dissipative environment. This system is used as an illustrative example to show the role of singular extremals in the control of quantum systems. We analyze a simple case where the control law is explicitly determined. We experimentally implement the optimal control using techniques of nuclear magnetic resonance. To our knowledge, this is the first experimental demonstration of singular extremals in quantum systems with bounded control amplitudes.Comment: 10 pages, 3 figure

Experimentally Attainable Optimal Pulse Shapes Obtained with the Aid of Genetic Algorithms

We propose a methodology to design optimal pulses for achieving quantum optimal control on molecular systems. Our approach constrains pulse shapes to linear combinations of a fixed number of experimentally relevant pulse functions. Quantum optimal control is obtained by maximizing a multi-target fitness function with genetic algorithms. As a first application of the methodology we generated an optimal pulse that successfully maximized the yield on a selected dissociation channel of a diatomic molecule. Our pulse is obtained as a linear combination of linearly chirped pulse functions. Data recorded along the evolution of the genetic algorithm contained important information regarding the interplay between radiative and diabatic processes. We performed a principal component analysis on these data to retrieve the most relevant processes along the optimal path. Our proposed methodology could be useful for performing quantum optimal control on more complex systems by employing a wider variety of pulse shape functions.Comment: 7 pages, 6 figure

Unified analysis of terminal-time control in classical and quantum systems

Many phenomena in physics, chemistry, and biology involve seeking an optimal control to maximize an objective for a classical or quantum system which is open and interacting with its environment. The complexity of finding an optimal control for maximizing an objective is strongly affected by the possible existence of sub-optimal maxima. Within a unified framework under specified conditions, control objectives for maximizing at a terminal time physical observables of open classical and quantum systems are shown to be inherently free of sub-optimal maxima. This attractive feature is of central importance for enabling the discovery of controls in a seamless fashion in a wide range of phenomena transcending the quantum and classical regimes.Comment: 10 page