12,593 research outputs found
Nonradiative limitations to plasmon propagation in chains of metallic nanoparticles
We investigate the collective plasmonic modes in a chain of metallic
nanoparticles that are coupled by near-field interactions. The size- and
momentum-dependent nonradiative Landau damping and radiative decay rates are
calculated analytically within an open quantum system approach. These decay
rates determine the excitation propagation along the chain. In particular, the
behavior of the radiative decay rate as a function of the plasmon wavelength
leads to a transition from an exponential decay of the collective excitation
for short distances to an algebraic decay for large distances. Importantly, we
show that the exponential decay is of a purely nonradiative origin. Our
transparent model enables us to provide analytical expressions for the
polarization-dependent plasmon excitation profile along the chain and for the
associated propagation length. Our theoretical analysis constitutes an
important step in the quest for the optimal conditions for plasmonic
propagation in nanoparticle chains.Comment: 14 pages, 6 figures; v2: published versio
Exciton decay dynamics in individual carbon nanotubes at room temperature
We studied the exciton decay dynamics of individual semiconducting single-walled carbon nanotubes at room temperature using time-resolved photoluminescence spectroscopy. The photoluminescence decay from nanotubes of the same (n,m) type follows a single exponential decay function, however, with lifetimes varying between about 1 and 40 ps from nanotube to nanotube. A correlation between broad photoluminescence spectra and short lifetimes was found and explained by defects promoting both nonradiative decay and vibronic dephasing
Enhancing infrared emission of mercury telluride (HgTe) quantum dots by plasmonic structures
The coupling of HgTe quantum dots to a gold nanobump plasmonic array can enhance the spontaneous infrared emission by a factor of five and reduce the influence of nonradiative decay channels
Spontaneous decay of excited atomic states near a carbon nanotube
Spontaneous decay process of an excited atom placed inside or outside (near
the surface) a carbon nanotube is analyzed. Calculations have been performed
for various achiral nanotubes. The effect of the nanotube surface has been
demonstrated to dramatically increase the atomic spontaneous decay rate -- by 6
to 7 orders of magnitude compared with that of the same atom in vacuum. Such an
increase is associated with the nonradiative decay via surface excitations in
the nanotube.Comment: 8 pages, 3 figure
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