Report on Airborne Radiometric Survey of the Thurso Area, 15th to 17th November 2006

A survey of part of Caithness near Thurso has been conducted as a performance test for a new Airborne Gamma Spectrometry (AGS) system developed at SUERC. The system deployed for this work consisted of a 16 litre NaI(Tl) spectrometer using a 2s measurement time. A total of 7500 spectra were collected in 13.5 hours flight time between the 15th-17th November 2006. The survey comprised a 60x31km area with a 5km line spacing providing an overview of the regional radiation environment, and a 15x20km area at 250m and 500m line spacings providing detailed information on the radiation environment of the Forss Water and River Thurso and their catchments. The survey areas did not include the Dounreay site and the town of Thurso. The data were processed to estimate activity concentrations of 137Cs (kBq m-2), naturally occurring 40K, 214Bi and 208Tl (Bq kg-1) and the gamma ray dose rate (mGy a-1). Maps were produced for the distribution of these activities within both the larger and more detailed survey areas. The gamma dose rate is driven by the natural activity, with no significant contribution from 137Cs activity. The region has considerable areas of saturated peat, suppressing the radiation from the underlying geology. The demarcation between the peat and the flagstone formations with thin soil overlays is clearly seen in the natural series activity and dose rate maps. 137Cs activities of up to 10 kBq m-2 have been observed on the drier land, consistent with Chernobyl fallout, with strongly suppressed signals from the peaty areas indicating that any fallout on these areas has migrated down through the peat. This work confirms the presence of features which accumulate 137Cs in the Forss Water system that had been noted in the survey commissioned by UKAEA in 1998. One feature observed in 1998 is absent in the data recorded in this work. Additional features were also recorded for the first time in the Forss Water upstream of the 1998 survey, and a series of similar featured, potentially of more limited extent, in the River Thurso system. The exploratory survey to the west also showed possible small scale features in Strath Halladale. Additional work would be needed to assess the dynamics of these systems, and their detailed local spatial characteristics and activity profiles, and to explore the extent to which similar features can be found in the fluvial catchments of other areas subjected to radioactive fallout in upper catchments, particularly those with peaty substrates. Time series analysis of these new data in comparison with older airborne data sets from the region would be of value, as would additional work in the future to extend the spatial and temporal boundaries of this survey

Review of Past Nuclear Accidents: Source Terms and Recorded Gamma-Ray Spectra

Airborne gamma ray spectrometry using high volume scintillation detectors, optionally in conjunction with Ge detectors, has potential for making rapid environmental measurements in response to nuclear accidents. A literature search on past nuclear accidents has been conducted to define the source terms which have been experienced so far. Selected gamma ray spectra recorded after past accidents have also been collated to examine the complexity of observed behaviour

Integrating nuclide specific and dose rate based methods for airborne and ground based gamma spectrometry

Results of joint airborne survey work conducted by SUERC and JAEA are presented, for areas to the north and south of Fukushima Daiichi using four different airborne survey systems, cross calibrated at reference sites in Scotland and near Namie. Airborne measurements were made at a series of different survey heights using three high volume NaI based spectrometers, and for the first time using a high resolution system based on the Ortec IDM HPGe spectrometer. The JAEA data sets were analysed using the same methods applied to national scale mapping in Japan since the accident. The SUERC data sets were analysed using nuclide specific approaches validated in the European ECCOMAGS project. The data presented on a digital terrain model show marked correspondence with landscape features, which both suggest the initial deposition processes, and indicate trajectories for future re-deposition by natural processes. All data sets are traceable to each other, and to the ground based calibration sites. Nuclide specific inventories have been defined, which can serve as a future reference to evaluate environmental change

Uranium exploration methodology in cold climates

The uranium prospecting boom of the past decade had, as a major consequence, the rapid development and proliferation of exploration methods for source materials. Numerous established methods were developed and refined whilst new techniques were introduced proving, in some instances, to be highly successful. To the explorationist the proliferation of instrumental hardware and detection systems was something of a headache with the result that in uranium exploration, more so than in other types of prospecting, the choice of exploration method at the appropriate stage of prospecting was frequently ill founded. The situation also spawned ‘black box’ purveyors who made extravagant claims for their equipment. Money was wasted through over kill applications of exploration method accompanied in many instances by deficiencies in the interpretation of results. This project was originally conceived as a means of evaluating, reviewing and filtering from a burgeoning array of systems the most appropriate exploration techniques applicable to cold climate environments. This goal has been trimmed somewhat since it had been hoped to incorporate site investigation data assembled in the field by the writer as appropriate case history material. This was not possible and as a consequence this report is a 'state of the art review' of the applicability of currently available techniques in Arctic and Subarctic environments. Reference is made to published case history data, where appropriate, supportive of the techniques or methods reviewed.Abstract -- Introduction -- Prospecting methods in relation to Arctic and Subarctic environments -- Review of direct exploration methods -- Radiometric methods -- Airborne spectrometry -- Car borne and hand held instrumentation -- Geochemical methods -- Soil and stream sediment methods -- Geobotanical methods -- Water sampling - Hydrogeochemical methods -- Other metods -- Optimal exploration method selection -- References -- Table of exploration methods discussed in this report

Exploring atmospheric radon with airborne gamma-ray spectroscopy

$^{222}$Rn is a noble radioactive gas produced along the $^{238}$U decay chain, which is present in the majority of soils and rocks. As $^{222}$Rn is the most relevant source of natural background radiation, understanding its distribution in the environment is of great concern for investigating the health impacts of low-level radioactivity and for supporting regulation of human exposure to ionizing radiation in modern society. At the same time, $^{222}$Rn is a widespread atmospheric tracer whose spatial distribution is generally used as a proxy for climate and pollution studies. Airborne gamma-ray spectroscopy (AGRS) always treated $^{222}$Rn as a source of background since it affects the indirect estimate of equivalent $^{238}$U concentration. In this work the AGRS method is used for the first time for quantifying the presence of $^{222}$Rn in the atmosphere and assessing its vertical profile. High statistics radiometric data acquired during an offshore survey are fitted as a superposition of a constant component due to the experimental setup background radioactivity plus a height dependent contribution due to cosmic radiation and atmospheric $^{222}$Rn. The refined statistical analysis provides not only a conclusive evidence of AGRS $^{222}$Rn detection but also a (0.96 $\pm$ 0.07) Bq/m$^{3}$ $^{222}$Rn concentration and a (1318 $\pm$ 22) m atmospheric layer depth fully compatible with literature data.Comment: 17 pages, 8 figures, 2 table

An Airborne and Vehicular Gamma Survey of Greenham Common, Newbury District and Surrounding Areas

The airborne gamma ray survey recorded more than 40,000 scintillation spectra and 20,000 spectra from semiconductor detectors. The vehicular survey produced a further 1346 and 763 spectral sets respectively. The installation, calibration, recording and analysis followed SURRC procedures which have been developed and validated over many years and are fully documented. Pre flight checks on detector performance for energy calibration, energy resolution and sensitivity were performed on a daily basis. Background readings over water were taken on a daily basis. All data were registered and backed up in duplicate to form a digital archive of the survey. Subsequent analysis and mapping has used a combination of standard procedures established over many years, and new techniques developed to analyse the low energy spectra. All results have been retained to facilitate traceability and further analysis in the future. The sensitivity of the aircraft and vehicle were also checked at Greenham Common by collecting a set of 31 core samples for independent laboratory analysis. The key points arising from the airborne survey of the entire area show that there has been sufficient sensitivity to record variations in the natural background. The levels of 137Cs are consistent with weapons' testing fallout, and are substantially lower than in other parts of the UK and Europe. The average levels of K (0.5%), U (1 ppm) and Th (3 ppm) are lower than national averages and show variations within the area which reflect local geology and landcover. The area as a whole therefore is one of low environmental radiation background compared with national averages. There is no evidence of signals at Greenham Common or in its vicinity which would present a local radiation hazard. However, signals were detected in the vicinity of Harwell and the Rutherford laboratory which would, at the time of the survey, represent radiation projected off-site as a result of materials stored on-site or on-site activities. Examination of the low energy gamma ray spectra recorded from the semiconductor detectors reveals no evidence, within the sensitivity limits of the method, for excess gamma ray signals at the energies associated with 235U around Greenham Common, Newbury and Thatcham. The low energy data are sufficiently sensitive to record variations in the distribution of natural activity in the area. There is tentative evidence for 241Am in the vicinity of AWE Aldermaston. The vehicular survey demonstrated that the grass areas in between the runway and taxi lanes, and around the hardstand associated with the 1958 fire have retained weapons' testing 137Cs. This supports the view that these represent authentic undisturbed areas for sampling. The built surfaces remaining at the time of the survey were of lower natural activity and 137Cs content than their surroundings. High resolution gamma ray spectra at selected sites were also consistent with the known sources of background radioactivity. On the basis of the results, Newbury District and surrounding areas represent an area with low environmental radioactivity compared with national and European averages. There is no evidence to substantiate fears about the quality of the radiation environment in the vicinity of Greenham Common

An Aerial Gamma Ray Survey of Springfields and the Ribble Estuary in September 1992

<p>A short aerial gamma ray survey was conducted in the vicinity of the Springfields site and Ribble Estuary from 1st-5th September 1992, to define existing background radiation levels, against which any future changes can be assessed. A twin engine AS 355 "Squirrel" helicopter chartered from Dollar Helicopters was used for this work. It was loaded with a 16 litre NaI(Tl) gamma ray detector and spectroscopy system on the 31st August and during the following days over 2700 separate spectra were recorded within a survey area of 20 x 12 km. Gamma ray spectra were recorded every 5 seconds at survey speed and altitude of 120 kph and 75 m respectively. A flight line spacing of 0.3km was chosen for the main survey area. On the 3rd September a low altitude, high spatial resolution (flight line spacing 100m and altitude 30m) was made over Banks Marsh (an area frequented by local wild fowlers).</p> <p>Survey results have been stored archivally and used to map the naturally occurring radionuclides 40K, 214Bi and 208Tl together with 137Cs and total gamma ray flux. In addition, for the first time, estimates of 234mPa in terms of deconvoluted count rate (normalised to 100m altitude) were made in the presence of 228Ac interference probably in disequilibrium with its parent thorium series.</p> <p>The maps provide a clear indication of the distribution and sources of environmental radioactivity in the Ribble at the time of the survey. The Ribble estuary is subject to regular and ongoing ground based studies by BNF, MAFF, HMIP, and University based groups, as a result of the authorised discharges of low level radioactivity from the Springfields site. The results of this survey complement this ground based work, and add to confidence that the estuarine system, it's associated sediments, tide washed pastures, salt marshes and river banks, have been thoroughly examined. There is support for earlier conclusions that the Cs on the salt marshes is the dominant source of external gamma exposure, and that the Springfields contribution to these locations is minor in comparison with this, Sellafield derived, signal. Upstream the situation is more complex, particularly where the dynamic sources of beta radiation are considered. As far as critical group assessments are concerned the survey provides clear evidence that the areas affected by 137Cs, where external gamma dose and possible food chain effects are of greatest interest, are in the lower reaches of the Ribble, whereas, at the time of the survey the 234mPa distribution was in the upper reaches of the river. This not only confirms the findings of ground based work, but provides some assurance that the different exposure paths (external gamma dose, skin dose) are not entirely synergistic. The discovery of possible transient sources of natural 228Ac in the salt marsh environment as a consequence of Th series disequilibrium immediately following spring tides is extremely interesting. If substantiated by further studies using semiconductor detectors this provides a new insight into the dynamic radiation environment of tide washed contexts.</p> <p>Aerial survey can potentially provide a rapid and cost effective means of studying environmentally dynamic sources such as 234mPa. In the case of the Ribble it would be necessary to reduce survey height to below 50m ground clearance to improve spatial resolution. Possible inconvenience to residents and property owners of such low altitude flights would have to be considered in addition to the potential value of environmental knowledge of the behaviour of short lived nuclides in a dynamic system such the Ribble estuary. There is nonetheless considerable potential for time series studies of this location. Recent flight trials by SURRC incorporating high efficiency germanium semiconductor detectors have verified the feasibility and potential a hybrid scintillation⁄ semiconductor spectrometer. Such a device can resolve any ambiguities arising from overlapping gamma ray peaks. This is particularly relevant to the confirmation of 228Ac in salt marshes. Ground based sampling at the time of measurement would enable concentration calibrations to be made for these dynamic sources. Further ground based measurements would be desirable to establish the extent to which low energy photons contribute to external gamma ray dose rates from sources with pronounced subsurface activity maxima.</p&gt