Uniaxial-Pressure induced Ferromagnetism of Enhanced Paramagnetic Sr3Ru2O7

We report a uniaxial pressure-dependence of magnetism in layered perovskite strontium ruthenate Sr3Ru2O7. By applying a relatively small uniaxial pressure, greater than 0.1 GPa normal to the RuO2 layer, ferromagnetic ordering manifests below 80 K from the enhanced-paramagnet. Magnetization at 1 kOe and 2 K becomes 100 times larger than that under ambient condition. Uniaxial pressure dependence of Curie temperature T_C suggests the first order magnetic transition. Origin of this uniaxial-pressure induced ferromagnetism is discussed in terms of the rotation of RuO6 octahedra within the RuO2 plane.Comment: 8 pages, 3 figures. to be published in Journal of the Physical Society of Japan, vol.73, No.5 (2004

Co-appearance of superconductivity and ferromagnetism in a Ca2_2RuO4_4 nanofilm crystal

By tuning the physical and chemical pressures of layered perovskite materials we can realize the quantum states of both superconductors and insulators. By reducing the thickness of a layered crystal to a nanometer level, a nanofilm crystal can provide novel quantum states that have not previously been found in bulk crystals. Here we report the realization of high-temperature superconductivity in Ca$_2$RuO$_4$ nanofilm single crystals. Ca$_2$RuO$_4$ thin film with the highest transition temperature $T_c$ (midpoint) of 64~K exhibits zero resistance in electric transport measurements. The superconducting critical current exhibited a logarithmic dependence on temperature and was enhanced by an external magnetic field. Magnetic measurements revealed a ferromagnetic transition at 180~K and diamagnetic magnetization due to superconductivity. Our results suggest the co-appearance of superconductivity and ferromagnetism in Ca$_2$RuO$_4$ nanofilm crystals. We also found that the induced bias current and the tuned film thickness caused a superconductor-insulator transition. The fabrication of micro-nanocrystals made of layered material enables us to discuss rich superconducting phenomena in ruthenates

Orbital Symmetry and Orbital Excitations in High-TcT_c Superconductors

We discuss a few possibilities of high-$T_c$ superconductivity with more than one orbital symmetry contributing to the pairing. First, we show that the high energies of orbital excitations in various cuprates suggest a simplified model with a single orbital of $x^2-y^2$ symmetry doped by holes. Next, several routes towards involving both $e_g$ orbital symmetries for doped holes are discussed: (i) some give superconductivity in a CuO$_2$ monolayer on Bi2212 superconductors, Sr$_2$CuO$_{4-\delta}$, Ba$_2$CuO$_{4-\delta}$, while (ii) others as nickelate heterostructures or Eu$_{2-x}$Sr$_x$NiO$_4$, could in principle realize it as well. At low electron filling of Ru ions, spin-orbital entangled states of $t_{2g}$ symmetry contribute in Sr$_2$RuO$_4$. Finally, electrons with both $t_{2g}$ and $e_g$ orbital symmetries contribute to the superconducting properties and nematicity of Fe-based superconductors, pnictides or FeSe. Some of them provide examples of orbital-selective Cooper pairing.Comment: 12 pages, 3 figures; in: Special Issue "From Cuprates to Room Temperature Superconductors", dedicated to the anniversary of Professor K. Alex M\"ulle

Effects of hydrostatic pressure on the magnetic susceptibility of ruthenium oxide Sr3Ru2O7: Evidence for pressure-enhanced antiferromagnetic instability

Hydrostatic pressure effects on the temperature- and magnetic field dependencies of the in-plane and out-of-plane magnetization of the bi-layered perovskite Sr3Ru2O7 have been studied by SQUID magnetometer measurements under a hydrostatic helium-gas pressure. The anomalously enhanced low-temperature value of the paramagnetic susceptibility has been found to systematically decrease with increasing pressure. The effect is accompanied by an increase of the temperature Tmax of a pronounced peak of susceptibility. Thus, magnetization measurements under hydrostatic pressure reveal that the lattice contraction in the structure of Sr3Ru2O7 promotes antiferromagnetism and not ferromagnetism, contrary to the previous beliefs. The effects can be explained by the enhancement of the inter-bi-layer antiferromagnetic spin coupling, driven by the shortening of the superexchange path, and suppression, due to the band-broadening effect, of competing itinerant ferromagnetic correlations.Comment: 11 pages, 4 figure