Electron spin diffusion in monolayer MoS2_2

Electron spin diffusion is investigated in monolayer MoS$_2$ in the absence of external electric and magnetic fields. The electron-impurity scattering, which is shown to play a negligible role in spin relaxation in time domain in this material, has a marked effect on the in-plane spin diffusion due to the anisotropic spin precession frequency in the spatial domain. With the electron-impurity and inter-valley electron-phonon scatterings separately included in the scattering term, we study the intra- and inter-valley diffusion processes of the in-plane spins by analytically solving the kinetic spin Bloch equations. The intra-valley process is found to be dominant in the in-plane spin diffusion, in contrast to the case of spin relaxation in time domain, where the inter-valley process can be comparable to or even more important than the intra-valley one. For the intra-valley process, we find that the in-plane spin diffusion is suppressed with the increase of impurity density but effectively enhanced by increasing electron density in both the degenerate and nondegenerate limits. We also take into account the electron-electron Coulomb scattering in the intra-valley process. Interestingly, we find that in the nondegenerate limit, the intra-valley spin diffusion length presents an opposite trend in the electron density dependence compared to the one with only electron-impurity scattering.Comment: 6 pages, 1 figur

Modeling inward diffusion and slow decay of energetic electrons in the Earth\u27s outer radiation belt

Abstract A new 3-D diffusion code is used to investigate the inward intrusion and slow decay of energetic radiation belt electrons (\u3e0.5 MeV) observed by the Van Allen Probes during a 10 day quiet period on March 2013. During the inward transport, the peak differential electron fluxes decreased by approximately an order of magnitude at various energies. Our 3-D radiation belt simulation including radial diffusion and pitch angle and energy diffusion by plasmaspheric hiss and electromagnetic ion cyclotron (EMIC) waves reproduces the essential features of the observed electron flux evolution. The decay time scales and the pitch angle distributions in our simulation are consistent with the Van Allen Probe observations over multiple energy channels. Our study suggests that the quiet time energetic electron dynamics are effectively controlled by inward radial diffusion and pitch angle scattering due to a combination of plasmaspheric hiss and EMIC waves in the Earth\u27s radiation belts

Hot-electron thermocouple and the diffusion thermopower of two-dimensional electrons in GaAs

A simple hot-electron thermocouple is realized in a two-dimensional electron system (2DES) and used to measure the diffusion thermopower of the 2DES at zero magnetic field. This hot-electron technique, which requires no micron-scale patterning of the 2DES, is much less sensitive than conventional methods to phonon-drag effects. Our thermopower results are in good agreement with the Mott formula for diffusion thermopower for temperatures up to T~2 K

Modulation of the thermodynamic, kinetic and magnetic properties of the hydrogen monomer on graphene by charge doping

The thermodynamic, kinetic and magnetic properties of the hydrogen monomer on doped graphene layers were studied by ab initio simulations. Electron doping was found to heighten the diffusion potential barrier, while hole doping lowers it. However, both kinds of dopings heighten the desorption potential barrier. The underlying mechanism was revealed by investigating the effect of doping on the bond strength of graphene and on the electron transfer and the coulomb interaction between the hydrogen monomer and graphene. The kinetic properties of H and D monomers on doped graphene layers during both the annealing process (annealing time $t_0 =$300 s) and the constant-rate heating process (heating rate $\alpha =$1.0 K/s) were simulated. Both electron and hole dopings were found to generally increase the desorption temperatures of hydrogen monomers. Electron doping was found to prevent the diffusion of hydrogen monomers, while the hole doping enhances their diffusion. Macroscopic diffusion of hydrogen monomers on graphene can be achieved when the doping-hole density reaches $5.0\times10^{13}$ cm$^{-2}$. The magnetic moment and exchange splitting were found to be reduced by both electron and hole dopings, which was explained by a simple exchange model. The study in this report can further enhance the understanding of the interaction between hydrogen and graphene and is expected to be helpful in the design of hydrogenated-graphene-based devices.Comment: Submitte

Spin diffusion in nn-type (111) GaAs quantum wells

We utilize the kinetic spin Bloch equation approach to investigate the steady-state spin diffusion in $n$-type (111) GaAs quantum wells, where the in-plane components of the Dresselhaus spin-orbit coupling term and the Rashba term can be partially canceled by each other. A peak of the spin diffusion length due to the cancellation is predicted in the perpendicular electric field dependence. It is shown that the spin diffusion length around the peak can be markedly controlled via temperature and doping. When the electron gas enters into the degenerate regime, the electron density also leads to observable influence on the spin diffusion in the strong cancellation regime. Furthermore, we find that the spin diffusion always presents strong anisotropy with respect to the direction of the injected spin polarization. The anisotropic spin diffusion depends on whether the electric field is far away from or in the strong cancellation regime.Comment: 5 pages, 3 figures, to be published in Solid State Commu

Dynamics of Overhauser Field under nuclear spin diffusion in a quantum dot

The coherence of electron spin can be significantly enhanced by locking the Overhauser field from nuclear spins using the nuclear spin preparation. We propose a theoretical model to calculate the long time dynamics of the Overhauser field under intrinsic nuclear spin diffusion in a quantum dot. We obtain a simplified diffusion equation that can be numerically solved and show quantitatively how the Knight shift and the electron-mediated nuclear spin flip-flop affect the nuclear spin diffusion. The results explain several recent experimental observations, where the decay time of Overhauser field is measured under different configurations, including variation of the external magnetic field, the electron spin configuration in a double dot, and the initial nuclear spin polarization rate.Comment: 6 pages, 5 figure