Observing backfolded and unfolded acoustic phonons by broadband optical light scattering

Abstract

We use broadband time domain Brillouin scattering to observe coherently generated phonon modes in bulk and nanolayered samples. We transform the measured transients into a frequency wavevector diagram and compare the resulting dispersion relations to calculations. The detected oscillation amplitude depends on the occupation of phonon modes induced by the pump pulse. For nanolayered samples with an appropriately large period, the whole wavevector range of the Brillouin zone becomes observable by broadband optical light scattering. The backfolded modes vanish, when the excitation has passed the nanolayers and propagates through the substrate underneat