research articlejournal article
oaioai:dspace.mit.edu:1721.1/82467

Concise Total Synthesis and Stereochemical Revision of all (−)-Trigonoliimines

Authors
Publication date
1 May 2011
Publisher
American Chemical Society (ACS)
Doi

    Abstract

    The concise and enantioselective total syntheses of (−)-trigonoliimines A, B, and C are described. Our unified strategy to all three natural products is based on asymmetric oxidation and reorganization of a single bistryptamine, a sequence of transformations with possible biogenetic relevance. We revise the absolute stereochemistry of (−)-trigonoliimines A, B, and C.National Institute of General Medical Sciences (U.S.) (GM074825)National Science Foundation (U.S.) (CHE-0946721)Amgen Inc.DuPont (Firm

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