The
exact fabrication of precise three-dimensional structures for
piezoresistive sensors necessitates superior manufacturing methods
or tooling, which are accompanied by time-consuming processes and
the potential for environmental harm. Herein, we demonstrated a method
for in situ synthesis of zinc oxide nanorod (ZnO
NR) arrays on graphene-treated cotton and paper substrates and constructed
highly sensitive, flexible, wearable, and chemically stable strain
sensors. Based on the structure of pine trees and needles in nature,
the hybrid sensing layer consisted of graphene-attached cotton or
paper fibers and ZnO NRs, and the results showed a high sensitivity
of 0.389, 0.095, and 0.029 kPa–1 and an ultra-wide
linear range of 0–100 kPa of this sensor under optimal conditions.
Our study found that water absorption and swelling of graphene fibers
and the associated reduction of pore size and growth of zinc oxide
were detrimental to pressure sensor performance. A random line model
was developed to examine the effects of different hydrothermal times
on sensor performance. Meanwhile, pulse detection, respiration detection,
speech recognition, and motion detection, including finger movements,
walking, and throat movements, were used to show their practical application
in human health activity monitoring. In addition, monolithically grown
ZnO NRs on graphene cotton sheets had been integrated into a flexible
sensing platform for outdoor UV photo-indication, which is, to our
knowledge, the first successful case of an integrated UV photo-detector
and motion sensor. Due to its excellent strain detection and UV detection
abilities, these strategies are a step forward in developing wearable
sensors that are cost-controllable and high-performance