Rapid estimation of /sup 226/Ra in soil for the Grand Junction RASA/UMTRA project

Abstract

The Radiological Survey Activities (RASA) Group of the Health and Safety Research Division at Oak Ridge National Laboratory (ORNL) is an Inclusion Survey Contractor (ISC) for the Uranium Mill Tailings Remedial Action Program (UMTRAP). The purpose of the ISC is to survey designated sites potentially contaminated with radioactive material originating from the 24 inactive uranium mill sites and make recommendations as to whether the site should be included in or excluded from further consideration by UMTRAP. An important aspect of the program is a prompt and inexpensive estimation of Radium-226 (/sup 226/Ra) concentration in soil samples. A large sodium iodide (NaI) well crystal coupled to a multichannel analyzer is used to count soil samples. Count data are currently analyzed with an algorithm that utilizes three regions of interest (ROI). A lack of agreement was observed when samples were also analyzed with lithium-drifted germanium (GeLi) spectrometers. The average estimate of /sup 226/Ra obtained using the current algorithm was 19% greater than the GeLi determination. Some possible reasons for these differences were examined. In 8.5% of the samples, the relative concentration of Cesium-137 (/sup 137/Cs) was highly correlated to the extent of error. Using alternative analysis techniques, the error for /sup 226/Ra estimations may be reduced by a factor of 2 for randomly selected samples and by a factor of 4 for samples containing high concentrations of /sup 137/Cs relative to the concentrations of /sup 226/Ra. 9 refs., 4 figs., 3 tabs