We have observed a bimodal behaviour of the distribution of the asymmetry
between the charges of the two heaviest products resulting from the decay of
the quasi-projectile released in binary Xe+Sn and Au+Au collisions from 60 to
100 MeV/u. Event sorting has been achieved through the transverse energy of
light charged particles emitted on the quasi-target side, thus avoiding
artificial correlations between the bimodality signal and the sorting variable.
Bimodality is observed for intermediate impact parameters for which the
quasi-projectile is identified. A simulation shows that the deexcitation step
rather than the geometry of the collision appears responsible for the bimodal
behaviour. The influence of mid-rapidity emission has been verified. The two
bumps of the bimodal distribution correspond to different excitation energies
and similar temperatures. It is also shown that it is possible to correlate the
bimodality signal with a change in the distribution of the heaviest fragment
charge and a peak in potential energy fluctuations. All together, this set of
data is coherent with what would be expected in a finite system if the
corresponding system in the thermodynamic limit exhibits a first order phase
transition.Comment: 30 pages, 31 figure