3 research outputs found
A novel high resolution contactless technique for thermal field mapping and thermal conductivity determination: Two-Laser Raman Thermometry
We present a novel high resolution contactless technique for thermal
conductivity determination and thermal field mapping based on creating a
thermal distribution of phonons using a heating laser, while a second laser
probes the local temperature through the spectral position of a Raman active
mode. The spatial resolution can be as small as nm, whereas its
temperature accuracy is K. We validate this technique investigating the
thermal properties of three free-standing single crystalline Si membranes with
thickness of 250, 1000, and 2000 nm. We show that for 2-dimensional materials
such as free-standing membranes or thin films, and for small temperature
gradients, the thermal field decays as in the diffusive
limit. The case of large temperature gradients within the membranes leads to an
exponential decay of the thermal field, . The
results demonstrate the full potential of this new contactless method for
quantitative determination of thermal properties. The range of materials to
which this method is applicable reaches far beyond the here demonstrated case
of Si, as the only requirement is the presence of a Raman active mode
A novel contactless technique for thermal field mapping and thermal conductivity determination: Two-Laser Raman Thermometry
Under the terms of the Creative Commons Attribution (CC BY) license to their work.We present a novel contactless technique for thermal conductivity determination and thermal field mapping based on creating a thermal distribution of phonons using a heating laser, while a second laser probes the local temperature through the spectral position of a Raman active mode. The spatial resolution can be as small as 300 nm, whereas its temperature accuracy is ±2 K. We validate this technique investigating the thermal properties of three free-standing single crystalline Si membranes with thickness of 250, 1000, and 2000 nm. We show that for two-dimensional materials such as free-standing membranes or thin films, and for small temperature gradients, the thermal field decays as T(r) ∝ ln(r) in the diffusive limit. The case of large temperature gradients within the membranes leads to an exponential decay of the thermal field, T ∝ exp[ − A·ln(r)]. The results demonstrate the full potential of this new contactless method for quantitative determination of thermal properties. The range of materials to which this method is applicable reaches far beyond the here demonstrated case of Si, as the only requirement is the presence of a Raman active mode.The authors acknowledge the financial support from the FP7 projects MERGING (Grant No. 309150), NANO-RF (Grant No. 318352), NANOTHERM (Grant No. 318117), NANOTEG-ENIAC (Grant No. 270789-2), and the Spanish MICINN projects nanoTHERM (Grant No. CSD2010-0044) and TAPHOR (MAT2012-31392). E.C.A. gratefully acknowledges a Becas Chile 2010 CONICYT fellowship from the Chilean government.Peer Reviewe