Magnetic Field Modulation of Chirooptical Effects in Magnetoplasmonic Structures

In this work we analyse the magnetic field effects on the chirooptical properties of magnetoplasmonic chiral structures. The structures consist of two-dimensional arrays of Au gammadions in which thin layers of Co have been inserted. Due to the magnetic properties of the Au/Co interface the structures have perpendicular magnetic anisotropy which favours magnetic saturation along the surface normal, allowing magnetic field modulation of the chirooptical response with moderate magnetic fields. These structures have two main resonances. The resonance at 850 nm has a larger chirooptical response than the resonance at 650 nm, which, on the other hand, exhibits a larger magnetic field modulation of its chirooptical response. This dissimilar behaviour is due to the different physical origin of the chirooptical and magneto-optical responses. Whereas the chirooptical effects are due to the geometry of the structures, the magneto-optical response is related to the intensity of the electromagnetic field in the magnetic (Co) layers. We also show that the optical chirality can be modulated by the applied magnetic field, which suggests that magnetoplasmonic chiral structures could be used to develop new strategies for chirooptical sensing.Funding from Spanish Ministry of Economy and Competitiveness through grants “FUNCOAT” CONSOLIDER CSD2008–00023, and MAPS MAT2011–29194-C02–01, and from Comunidad de Madrid through grants “NANOBIOMAGNET” S2009/MAT-1726 and “MICROSERES-CM” S2009/TIC-1476 is acknowledged.Peer Reviewe