1,878 research outputs found
Hall effect of quasi-hole gas in organic single-crystal transistors
Hall effect is detected in organic field-effect transistors, using
appropriately shaped rubrene (C42H28) single crystals. It turned out that
inverse Hall coefficient, having a positive sign, is close to the amount of
electric-field induced charge upon the hole accumulation. The presence of the
normal Hall effect means that the electromagnetic character of the surface
charge is not of hopping carriers but resembles that of a two-dimensional
hole-gas system
Ferroelectric polarization flop in a frustrated magnet MnWO induced by magnetic fields
The relationship between magnetic order and ferroelectric properties has been
investigated for MnWO with long-wavelength magnetic structure. Spontaneous
electric polarization is observed in an elliptical spiral spin phase. The
magnetic-field dependence of electric polarization indicates that the
noncollinear spin configuration plays a key role for the appearance of
ferroelectric phase. An electric polarization flop from the b direction to the
a direction has been observed when a magnetic field above 10T is applied along
the b axis. This result demonstrates that an electric polarization flop can be
induced by a magnetic field in a simple system without rare-earth f-moments.Comment: 9 pages, 4 figure
Charge transfer excitons in optical absorption spectra of C60-dimers and polymers
Charge-transfer (CT) exciton effects are investigated for the optical
absorption spectra of crosslinked C60 systems by using the intermediate exciton
theory. We consider the C60-dimers, and the two (and three) molecule systems of
the C60-polymers. We use a tight-binding model with long-range Coulomb
interactions among electrons, and the model is treated by the Hartree-Fock
approximation followed by the single-excitation configuration interaction
method. We discuss the variations in the optical spectra by changing the
conjugation parameter between molecules. We find that the total CT-component
increases in smaller conjugations, and saturates at the intermediate
conjugations. It decreases in the large conjugations. We also find that the
CT-components of the doped systems are smaller than those of the neutral
systems, indicating that the electron-hole distance becomes shorter in the
doped C60-polymers.Comment: Figures should be requested to the autho
Electronic Orders Induced by Kondo Effect in Non-Kramers f-Electron Systems
This paper clarifies the microscopic nature of the staggered scalar order,
which is specific to even number of f electrons per site. In such systems,
crystalline electric field (CEF) can make a singlet ground state. As exchange
interaction with conduction electrons increases, the CEF singlet at each site
gives way to Kondo singlets. The collective Kondo singlets are identified with
itinerant states that form energy bands. Near the boundary of itinerant and
localized states, a new type of electronic order appears with staggered Kondo
and CEF singlets. We present a phenomenological three-state model that
qualitatively reproduces the characteristic phase diagram, which have been
obtained numerically with use of the continuous-time quantum Monte Carlo
combined with the dynamical mean-field theory. The scalar order observed in
PrFe_4P_{12} is ascribed to this staggered order accompanying charge density
wave (CDW) of conduction electrons. Accurate photoemission and tunneling
spectroscopy should be able to probe sharp peaks below and above the Fermi
level in the ordered phase.Comment: 7 pages, 8 figure
On the origin of multiple ordered phases in PrFe4P12
The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is
discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction
of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively
provided (i) ferro-type interactions are introduced between the dipoles as well
as between the octupoles of localized f-electrons, and (ii) separation is
vanishingly small between the \Gamma_1-\Gamma_4^{(1)} crystalline electric
field (CEF) levels. The high-field phase can have either the same ordering
vector q=(1,0,0) as in the low-field phase, or a different one q=0 depending on
the parameters. In the latter case, distortion of the crystal perpendicular to
the (111) axis is predicted. The corresponding anomaly in elastic constants
should also appear. The electrical resistivity is calculated with account of
scattering within the CEF quasi-quartet. It is found that the resistivity as a
function of the direction of magnetic field shows a sharp maximum around the
(111) axis at low temperatures because of the level crossing.Comment: 16 pages, 5 figure
Effect of cation size variance on spin and orbital order in Eu(LaY)VO
We have investigated the -ion ( = rare earth or Y) size variance effect
on spin/orbital order in Eu(LaY)VO. The
size variance disturbs one-dimensional orbital correlation in -type
spin/-type orbital ordered states and suppresses this spin/orbital order. In
contrast, it stabilizes the other spin/orbital order. The results of neutron
and resonant X-ray scattering denote that in the other ordered phase, the
spin/orbital patterns are -type/-type, respectively.Comment: 4 pages, 4 figures, accepted to Rapid Communication in Physical
Review
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