211 research outputs found
Noise-induced switching between vortex states with different polarization in classical two-dimensional easy-plane magnets
In the 2-dimensional anisotropic Heisenberg model with XY-symmetry there are
non-planar vortices which exhibit a localized structure of the z-components of
the spins around the vortex center. We study how thermal noise induces a
transition of this structure from one polarization to the opposite one. We
describe the vortex core by a discrete Hamiltonian and consider a stationary
solution of the Fokker-Planck equation. We find a bimodal distribution function
and calculate the transition rate using Langer's instanton theory (1969). The
result is compared with Langevin dynamics simulations for the full many-spin
model.Comment: 15 pages, 4 figures, Phys. Rev. B., in pres
Intrinsic hole mobility and trapping in a regio-regular poly(thiophene)
The transport properties of high-performance thin-film transistors (TFT) made
with a regio-regular poly(thiophene) semiconductor (PQT-12) are reported. The
room-temperature field-effect mobility of the devices varied between 0.004
cm2/V s and 0.1 cm2/V s and was controlled through thermal processing of the
material, which modified the structural order. The transport properties of TFTs
were studied as a function of temperature. The field-effect mobility is
thermally activated in all films at T<200 K and the activation energy depends
on the charge density in the channel. The experimental data is compared to
theoretical models for transport, and we argue that a model based on the
existence of a mobility edge and an exponential distribution of traps provides
the best interpretation of the data. The differences in room-temperature
mobility are attributed to different widths of the shallow localized state
distribution at the edge of the valence band due to structural disorder in the
film. The free carrier mobility of the mobile states in the ordered regions of
the film is the same in all structural modifications and is estimated to be
between 1 and 4 cm2/V s.Comment: 20 pages, 8 figure
Electron spin-lattice relaxation in Mn2+-doped ferroelectric TSCC
The spin-lattice relaxation of ferroelectric TSCC: Mn2+ has been investigated by means of the electron spin echo method in the range between 4.2 and 160 K. In the vicinity of the phase transition an anomalous increase of T1 has been detected deviating from the spin-lattice relaxation in the remaining temperature range. © 1978
Evidence for Different Freeze-Out Radii of High- and Low-Energy Pions Emitted in Au+Au Collisions at 1 GeV/nucleon
Double differential production cross sections of negative and positive pions
and the number of participating protons have been measured in central Au+Au
collisions at 1 GeV per nucleon incident energy. At low pion energies the pi^-
yield is strongly enhanced over the pi^+ yield. The energy dependence of the
pi^-/pi^+ ratio is assigned to the Coulomb interaction of the charged pions
with the protons in the reaction zone. The deduced Coulomb potential increases
with increasing pion c.m. energy. This behavior indicates different freeze-out
radii for different pion energies in the c.m.~frame.Comment: IKDA is the Institute for Nuclear Physics in Darmstadt/German
Dynamics of ferroelectric nano cluster in BaTiO3 observed as a real time correlation between two soft X-ray laser pulses
We carry out a theoretical investigation to clarify the dynamic property of
photo-created nano-sized ferroelectric cluster observed in the paraelectric
BaTiO3 as a real time correlation of speckle pattern between two soft X-ray
laser pulses, at just above the paraelectric-ferroelectric phase transition
temperature. Based on a model with coupled soft X-ray photon and ferroelectric
phonon mode, we study the time dependence of scattering probability by using a
perturbative expansion approach. The cluster-associated phonon softening as
well as central peak effects are well reproduced in the phonon spectral
function via quantum Monte Carlo simulation. Besides, it is found that the time
dependence of speckle correlation is determined by the relaxation dynamics of
ferroelectric clusters. Near the transition point, cluster excitation is
stable, leading to a long relaxation time. While, at high temperature, cluster
structure is subject to the thermal fluctuation, ending up with a short
relaxation time.Comment: 9 pages, 3 figure
Far-infrared study of the Jahn-Teller distorted C60 monoanion in C60 tetraphenylphosphoniumiodide
We report high-resolution far-infrared transmission measurements on C(60)-tetraphenylphosphoniumiodide as a function of temperature. In the spectral region investigated (20-650 cm(-1)), we assign intramolecular modes of the C(60) monoanion and identify low-frequency combination modes. The well-known F(1u)(1) and F(1u)(2) modes are split into doublers at room temperature, indicating a D(5d) or D(3d) distorted ball. This result is consistent with a dynamic Jahn-Teller effect in the strong-coupling limit or with a static distortion stabilized by low-symmetry perturbations. The appearance of silent odd modes is in keeping with symmetry reduction of the hall, while activation of even modes is attributed to interband electron-phonon coupling and orientational disorder in the fulleride salt. Temperature dependences reveal a weak transition in the region 125-150 K in both C(60)(-) and counterion modes, indicating a bulk, rather than solely molecular, effect. Anomalous softening (with decreasing temperature) in several modes may correlate with the radial character of those vibrations. [S0163-1829(98)03245-7]
Magnetic Vortex Core Reversal by Excitation of Spin Waves
Micron-sized magnetic platelets in the flux closed vortex state are
characterized by an in-plane curling magnetization and a nanometer-sized
perpendicularly magnetized vortex core. Having the simplest non-trivial
configuration, these objects are of general interest to micromagnetics and may
offer new routes for spintronics applications. Essential progress in the
understanding of nonlinear vortex dynamics was achieved when low-field core
toggling by excitation of the gyrotropic eigenmode at sub-GHz frequencies was
established. At frequencies more than an order of magnitude higher vortex state
structures possess spin wave eigenmodes arising from the magneto-static
interaction. Here we demonstrate experimentally that the unidirectional vortex
core reversal process also occurs when such azimuthal modes are excited. These
results are confirmed by micromagnetic simulations which clearly show the
selection rules for this novel reversal mechanism. Our analysis reveals that
for spin wave excitation the concept of a critical velocity as the switching
condition has to be modified.Comment: Minor corrections and polishing of previous versio
In vivo and ex vivo percutaneous absorption of [14C]-bisphenol A in rats: a possible extrapolation to human absorption?
Bisphenol A (BPA) is a monomer used mainly in the synthesis of polycarbonates and epoxy resins. Percutaneous absorption is the second source of exposure, after inhalation, in the work environment. However, studies on this route of absorption are lacking or incomplete. In this study, percutaneous BPA absorption was measured in vivo and ex vivo in the rat, and ex vivo in humans. An approximately 12-fold difference in permeability between rat skin and human skin was found, with permeability being higher in the rat. In addition, inter- and intra-individual variability of up to tenfold was observed in humans. No accumulation of BPA in the skin was found during exposure. The skin clearance rate following exposure was estimated at 0.4Â ÎŒg/cmÂČ/h. Ex vivo and in vivo percutaneous absorption fluxes of BPA in the rat were in the same range (about 2.0Â ÎŒg/cmÂČ/h), suggesting that extrapolation to the in vivo situation in humans may be possible. The European tolerable daily intake (TDI) of BPA is 50Â ÎŒg/kg body weight. However, many research projects have highlighted the significant effects of BPA in rodents at doses lower than 10Â ÎŒg/kg/day. A 1-h occupational exposure over 2,000Â cmÂČ (forearms and hands) may lead to a BPA absorption of 4Â ÎŒg/kg/day. This is 8% of the European TDI and is very close to the value at which effects have been observed in animals. This absorption must therefore be taken into account when evaluating risks of BPA exposure, at least until more relevant results on the toxicity of BPA in humans are available
Critical dynamics in the 2d classical XY-model: a spin dynamics study
Using spin-dynamics techniques we have performed large-scale computer
simulations of the dynamic behavior of the classical three component XY-model
(i.e. the anisotropic limit of an easy-plane Heisenberg ferromagnet), on square
lattices of size up to 192^2, for several temperatures below, at, and above
T_KT. The temporal evolution of spin configurations was determined numerically
from coupled equations of motion for individual spins by a fourth order
predictor-corrector method, with initial spin configurations generated by a
hybrid Monte Carlo algorithm. The neutron scattering function S(q,omega) was
calculated from the resultant space-time displaced spin-spin correlation
function. Pronounced spin-wave peaks were found both in the in-plane and the
out-of-plane scattering function over a wide range of temperatures. The
in-plane scattering function S^xx also has a large number of clear but weak
additional peaks, which we interpret to come from two-spin-wave scattering. In
addition, we observed a small central peak in S^xx, even at temperatures well
below the phase transition. We used dynamic finite size scaling theory to
extract the dynamic critical exponent z. We find z=1.00(4) for all T <= T_KT,
in excellent agreement with theoretical predictions, although the shape of
S(q,omega) is not well described by current theory.Comment: 31 pages, LaTex, 13 figures (38 subfigures) included as eps-files,
needs psfig, 260 K
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