Gold, copper, silver and aluminum nanoantennas to enhance spontaneous emission

We compute the decay rates of emitters coupled to spheroidal nanoantennas made of gold, copper, silver, and aluminum. The spectral position of the localized surface plasmon-polariton resonance, the enhancement factors and the quantum efficiency are investigated as a function of the aspect ratio, background index and the metal composing the nanoantenna. While copper yields results similar to gold, silver and aluminum exhibit different performances. Our results show that with a careful choice of the parameters these nanoantennas can enhance emitters ranging from the UV to the near-IR spectrum.Comment: 7 pages, 10 figure

A high-fidelity photon gun: intensity-squeezed light from a single molecule

A two-level atom cannot emit more than one photon at a time. As early as the 1980s, this quantum feature was identified as a gateway to "single-photon sources", where a regular excitation sequence would create a stream of light particles with photon number fluctuations below the shot noise. Such an intensity squeezed beam of light would be desirable for a range of applications such as quantum imaging, sensing, enhanced precision measurements and information processing. However, experimental realizations of these sources have been hindered by large losses caused by low photon collection efficiencies and photophysical shortcomings. By using a planar metallo-dielectric antenna applied to an organic molecule, we demonstrate the most regular stream of single photons reported to date. Measured intensity fluctuations reveal 2.2 dB squeezing limited by our detection efficiency, equivalent to 6.2 dB intensity squeezing right after the antenna.Comment: 9 pages, 3 figure

Coherent interaction of a metallic structure with a single quantum emitter: from super absorption to cloaking

We provide a general theoretical platform based on quantized radiation in absorptive and inhomogeneous media for investigating the coherent interaction of light with metallic structures in the immediate vicinity of quantum emitters. In the case of a very small metallic cluster, we demonstrate extreme regimes where a single emitter can either counteract or enhance particle absorption by three orders of magnitude. For larger structures, we show that an emitter can eliminate both scattering and absorption and cloak a plasmonic antenna. We provide physical interpretations of our results and discuss their applications in active metamaterials and quantum plasmonics

Highly efficient interfacing of guided plasmons and photons in nanowires

Successful exploitations of strongly confined surface plasmon-polaritons critically rely on their efficient and rapid conversion to lossless channels. We demonstrate a simple, robust, and broad-band butt-coupling technique for connecting a metallic nanowire and a dielectric nanofiber. Conversion efficiencies above 95% in the visible and close to 100% in the near infrared can be achieved with realistic parameters. Moreover, by combining butt-coupling with nanofocusing, we propose a broad-band high-throughput near-field optical microscope.Comment: 5 figure

Polaritonic states in a dielectric nanoguide: localization and strong coupling

Propagation of light through dielectrics lies at the heart of optics. However, this ubiquitous process is commonly described using phenomenological dielectric function $\varepsilon$ and magnetic permeability $\mu$, i.e. without addressing the quantum graininess of the dielectric matter. Here, we present a theoretical study where we consider a one-dimensional ensemble of atoms in a subwavelength waveguide (nanoguide) as fundamental building blocks of a model dielectric. By exploring the roles of the atom-waveguide coupling efficiency, density, disorder, and dephasing, we establish connections among various features of polaritonic light-matter states such as localization, super and subradiance, and strong coupling. In particular, we show that coherent multiple scattering of light among atoms that are coupled via a single propagating mode can gives rise to Rabi splitting. These results provide important insight into the underlying physics of strong coupling reported by recent room-temperature experiments with microcavities and surface plasmons.Comment: 10 pages, 6 figure

Direct optical sensing of single unlabeled small proteins and super-resolution microscopy of their binding sites

More than twenty years ago, scientists succeeded in pushing the limits of optical detection to single molecules using fluorescence. This breakthrough has revolutionized biophysical measurements, but restrictions in photophysics and labeling protocols have motivated many efforts to achieve fluorescence-free single-molecule sensitivity in biological studies. Although several interesting mechanisms using vibrational spectroscopy, photothermal detection, plasmonics or microcavities have been proposed for biosensing at the single-protein level, no method has succeeded in direct label-free detection of single proteins. Here, we present the first results using interferometric detection of scattering (iSCAT) from single proteins without the need for any label, optical nanostructure or microcavity. Furthermore, we demonstrate super-resolution imaging of protein binding with nanometer localization precision. The ease of iSCAT instrumentation promises a breakthrough for industrial usage as well as fundamental laboratory experiments

Light Microscopy: An ongoing contemporary revolution

Optical microscopy is one of the oldest scientific instruments that is still used in forefront research. Ernst Abbe's nineteenth century formulation of the resolution limit in microscopy let generations of scientists believe that optical studies of individual molecules and resolving sub-wavelength structures were not feasible. The Nobel Prize in 2014 for super-resolution fluorescence microscopy marks a clear recognition that the old beliefs have to be revisited. In this article, we present a critical overview of various recent developments in optical microscopy. In addition to the popular super-resolution fluorescence methods, we discuss the prospects of various other techniques and imaging contrasts and consider some of the fundamental and practical challenges that lie ahead.Comment: 37 pages, 13 figure

High-resolution spectroscopy of single Pr3+^{3+} ions on the 3^3H4_4-1^1D2_2 transition

Rare earth ions in crystals exhibit narrow spectral features and hyperfine-split ground states with exceptionally long coherence times. These features make them ideal platforms for quantum information processing in the solid state. Recently, we reported on the first high-resolution spectroscopy of single Pr$^{3+}$ ions in yttrium orthosilicate (YSO) nanocrystals. While in that work we examined the less explored $^3$H$_4$-$^3$P$_0$ transition at a wavelength of 488 nm, here we extend our investigations to the $^3$H$_4$-$^1$D$_2$ transition at 606 nm. In addition, we present measurements of the second-order autocorrelation function, fluorescence lifetime, and emission spectra of single ions as well as their polarization dependencies on both transitions; these data were not within the reach of the first experiments reported earlier. Furthermore, we show that by a proper choice of the crystallite, one can obtain narrower spectral lines and, thus, resolve the hyperfine levels of the excited state. We expect our results to make single-ion spectroscopy accessible to a larger scientific community.Comment: 5 pages, 5 figure

A Single-Emitter Gain Medium for Bright Coherent Radiation from a Plasmonic Nanoresonator

We theoretically demonstrate the generation and radiation of coherent nanoplasmons powered by a single three-level quantum emitter on a plasmonic nanoresonator. By pumping the three-level emitter in a Raman configuration, we show a pathway to achieve macroscopic accumulation of nanoplasmons due to stimulated emission in the nanoresonator despite their fast relaxation. Thanks to the antenna effect of the nanoresonator, the system acts as an efficient and bright nanoscopic coherent light source with a photon emission rate of hundreds of Terahertz and could be realized with solid-state emitters at room temperatures in pulse mode. We provide physical interpretations of the results and discuss their realization and implications for ultra-compact integration of optoelectronics.Comment: 15 pages, 7 figure