27 research outputs found
Rydberg trimers and excited dimers bound by internal quantum reflection
Quantum reflection is a pure wave phenomena that predicts reflection of a
particle at a changing potential for cases where complete transmission occurs
classically. For a chemical bond, we find that this effect can lead to
non-classical vibrational turning points and bound states at extremely large
interatomic distances. Only recently has the existence of such ultralong-range
Rydberg molecules been demonstrated experimentally. Here, we identify a broad
range of molecular lines, most of which are shown to originate from two
different novel sources: a single-photon associated triatomic molecule formed
by a Rydberg atom and two ground state atoms and a series of excited dimer
states that are bound by a so far unexplored mechanism based on internal
quantum reflection at a steep potential drop. The properties of the Rydberg
molecules identified in this work qualify them as prototypes for a new type of
chemistry at ultracold temperatures.Comment: 6 pages, 3 figures, 1 tabl
Ion detection in the photoionization of a Rb Bose-Einstein condensate
Two-photon ionization of Rubidium atoms in a magneto-optical trap and a
Bose-Einstein condensate (BEC) is experimentally investigated. Using 100 ns
laser pulses, we detect single ions photoionized from the condenstate with a
35(10)% efficiency. The measurements are performed using a quartz cell with
external electrodes, allowing large optical access for BECs and optical
lattices.Comment: 14 pages, 7 figure
The physics of dipolar bosonic quantum gases
This article reviews the recent theoretical and experimental advances in the
study of ultracold gases made of bosonic particles interacting via the
long-range, anisotropic dipole-dipole interaction, in addition to the
short-range and isotropic contact interaction usually at work in ultracold
gases. The specific properties emerging from the dipolar interaction are
emphasized, from the mean-field regime valid for dilute Bose-Einstein
condensates, to the strongly correlated regimes reached for dipolar bosons in
optical lattices.Comment: Review article, 71 pages, 35 figures, 350 references. Submitted to
Reports on Progress in Physic
Formation and interactions of cold and ultracold molecules: new challenges for interdisciplinary physics
Progress on researches in the field of molecules at cold and ultracold
temperatures is reported in this review. It covers extensively the experimental
methods to produce, detect and characterize cold and ultracold molecules
including association of ultracold atoms, deceleration by external fields and
kinematic cooling. Confinement of molecules in different kinds of traps is also
discussed. The basic theoretical issues related to the knowledge of the
molecular structure, the atom-molecule and molecule-molecule mutual
interactions, and to their possible manipulation and control with external
fields, are reviewed. A short discussion on the broad area of applications
completes the review.Comment: to appear in Reports on Progress in Physic
Lifetimes of ultralong-range Rydberg molecules in vibrational ground and excited states
Since their first experimental observation, ultralong-range Rydberg molecules consisting of a highly excited Rydberg atom and a ground state atom [1, 2] have attracted the interest in the field of ultracold chemistry [3, 4]. Especially the intriguing properties such as size, polarizability and type of binding they inherit from the Rydberg atom are of interest. An open question in the field is the reduced lifetime of the molecules compared to the corresponding atomic Rydberg states [2]. In this paper we present an experimental study on the lifetimes of the (3)Sigma (5s - 35s) molecule in its vibrational ground state and in an excited state. We show that the lifetimes depend on the density of ground state atoms and that this can be described in the frame of a classical scattering between the molecules and ground state atoms. We also find that the excited molecular state has an even more reduced lifetime compared to the ground state which can be attributed to an inward penetration of the bound atomic pair due to imperfect quantum reflection that takes place in the special shape of the molecular potential [5]