Simultaneous resonant x-ray diffraction measurement of polarization inversion and lattice strain in polycrystalline ferroelectrics

International audienceStructure-property relationships in ferroelectrics extend over several length scales from the individual unit cell to the macroscopic device, and with dynamics spanning a broad temporal domain. Characterizing the multi-scale structural origin of electric field-induced polarization reversal and strain in ferroelectrics is an ongoing challenge that so far has obscured its fundamental behaviour. By utilizing small intensity differences between Friedel pairs due to resonant scattering, we demonstrate a time-resolved X-ray diffraction technique for directly and simultaneously measuring both lattice strain and, for the first time, polarization reversal during in-situ electrical perturbation. This technique is demonstrated for BaTiO3-BiZn0.5Ti0.5O3 (BT-BZT) polycrystalline ferroelectrics, a prototypical lead-free piezoelectric with an ambiguous switching mechanism. This combines the benefits of spectroscopic and diffraction-based measurements into a single and robust technique with time resolution down to the ns scale, opening a new door to in-situ structure-property characterization that probes the full extent of the ferroelectric behaviou

The continuum limit of quark number susceptibilities

We report the continuum limit of quark number susceptibilities in quenched QCD. Deviations from ideal gas behaviour at temperature T increase as the lattice spacing is decreased from T/4 to T/6, but a further decrease seems to have very little effect. The measured susceptibilities are 20% lower than the ideal gas values, and also 10% below the hard thermal loop (HTL) results. The off-diagonal susceptibility is several orders of magnitude smaller than the HTL results. We verify a strong correlation between the lowest screening mass and the susceptibility. We also show that the quark number susceptibilities give a reasonable account of the Wroblewski parameter, which measures the strangeness yield in a heavy-ion collision.Comment: 8 pages, 5 figure

Spatiotemporal Stochastic Resonance in Fully Frustrated Josephson Ladders

We consider a Josephson-junction ladder in an external magnetic field with half flux quantum per plaquette. When driven by external currents, periodic in time and staggered in space, such a fully frustrated system is found to display spatiotemporal stochastic resonance under the influence of thermal noise. Such resonance behavior is investigated both numerically and analytically, which reveals significant effects of anisotropy and yields rich physics.Comment: 8 pages in two columns, 8 figures, to appear in Phys. Rev.

The QCD thermal phase transition in the presence of a small chemical potential

We propose a new method to investigate the thermal properties of QCD with a small quark chemical potential $\mu$. Derivatives of the phase transition point with respect to $\mu$ are computed at $\mu=0$ for 2 flavors of p-4 improved staggered fermions with $ma=0.1,0.2$ on a $16^3\times4$ lattice. The resulting Taylor expansion is well behaved for the small values of $\mu_{\rm q}/T_c\sim0.1$ relevant for RHIC phenomenology, and predicts a critical curve $T_c(\mu)$ in reasonable agreement with estimates obtained using exact reweighting. In addition, we contrast the case of isoscalar and isovector chemical potentials, quantify the effect of $\mu\not=0$ on the equation of state, and comment on the complex phase of the fermion determinant in QCD with $\mu\not=0$.Comment: 26 pages, 25 figures, minor modificatio

Test of the Kolmogorov-Johnson-Mehl-Avrami picture of metastable decay in a model with microscopic dynamics

The Kolmogorov-Johnson-Mehl-Avrami (KJMA) theory for the time evolution of the order parameter in systems undergoing first-order phase transformations has been extended by Sekimoto to the level of two-point correlation functions. Here, this extended KJMA theory is applied to a kinetic Ising lattice-gas model, in which the elementary kinetic processes act on microscopic length and time scales. The theoretical framework is used to analyze data from extensive Monte Carlo simulations. The theory is inherently a mesoscopic continuum picture, and in principle it requires a large separation between the microscopic scales and the mesoscopic scales characteristic of the evolving two-phase structure. Nevertheless, we find excellent quantitative agreement with the simulations in a large parameter regime, extending remarkably far towards strong fields (large supersaturations) and correspondingly small nucleation barriers. The original KJMA theory permits direct measurement of the order parameter in the metastable phase, and using the extension to correlation functions one can also perform separate measurements of the nucleation rate and the average velocity of the convoluted interface between the metastable and stable phase regions. The values obtained for all three quantities are verified by other theoretical and computational methods. As these quantities are often difficult to measure directly during a process of phase transformation, data analysis using the extended KJMA theory may provide a useful experimental alternative.Comment: RevTex, 21 pages including 14 ps figures. Submitted to Phys. Rev. B. One misprint corrected in Eq.(C1

Plasmoid-Induced-Reconnection and Fractal Reconnection

As a key to undertanding the basic mechanism for fast reconnection in solar flares, plasmoid-induced-reconnection and fractal reconnection are proposed and examined. We first briefly summarize recent solar observations that give us hints on the role of plasmoid (flux rope) ejections in flare energy release. We then discuss the plasmoid-induced-reconnection model, which is an extention of the classical two-ribbon-flare model which we refer to as the CSHKP model. An essential ingredient of the new model is the formation and ejection of a plasmoid which play an essential role in the storage of magnetic energy (by inhibiting reconnection) and the induction of a strong inflow into reconnection region. Using a simple analytical model, we show that the plasmoid ejection and acceleration are closely coupled with the reconnection process, leading to a nonlinear instability for the whole dynamics that determines the macroscopic reconnection rate uniquely. Next we show that the current sheet tends to have a fractal structure via the following process path: tearing, sheet thinning, Sweet- Parker sheet, secondary tearing, further sheet thinning... These processes occur repeatedly at smaller scales until a microscopic plasma scale (either the ion Larmor radius or the ion inertial length) is reached where anomalous resistivity or collisionless reconnection can occur. The current sheet eventually has a fractal structure with many plasmoids (magnetic islands) of different sizes. When these plasmoids are ejected out of the current sheets, fast reconnection occurs at various different scales in a highly time dependent manner. Finally, a scenario is presented for fast reconnection in the solar corona on the basis of above plasmoid-induced-reconnection in a fractal current sheet.Comment: 9 pages, 11 figures, with using eps.sty; Earth, Planets and Space in press; ps-file is also available at http://stesun8.stelab.nagoya-u.ac.jp/~tanuma/study/shibata2001

Biomarker analysis in stage III–IV (M0) gastric cancer patients who received curative surgery followed by adjuvant 5-fluorouracil and cisplatin chemotherapy: epidermal growth factor receptor (EGFR) associated with favourable survival

The aim of this study was to analyse the impact of epidermal growth factor receptor (EGFR), thymidylate synthase (TS), dihydropyrimidine dehydrogenase (DPD), thymidine phosphorylase (TP), aurora kinase (ARK) A/B, and excision repair cross-complementing gene 1 (ERCC1) on the efficacy of adjuvant chemotherapy with 5-fluorouracil and cisplatin (FP) after curative gastric resection. Normal and cancer tissue were separately obtained from gastrectomy samples of 153 patients with AJCC stage III–IV (M0) who subsequently treated with adjuvant FP chemotherapy. TS, DPD, TP, ERCC1, and ARK proteins were measured by immunohistochemistry (IHC). EGFR expression was investigated using a standardized IHC with the EGFR PharmDx assay. Amplification of EGFR gene was analysed using fluorescent in situ hybridisation (FISH). In multivariate analysis, stage, ratio of positive to removed lymph nodes, and EGFR expression were significant prognostic factors for overall survival. Patients with higher EGFR expression had better overall survival than those with lower expression (relative risk: 0.475 (95% confidence interval, 0.282–0.791, P=0.005). Low EGFR expression might be a predictive marker for relapse in curative resected stage III–IV (M0) gastric cancer patients who received adjuvant FP chemotherapy

Parameterizing the Power Spectrum: Beyond the Truncated Taylor Expansion

The power spectrum is traditionally parameterized by a truncated Taylor series: $ln P(k) = ln P_* + (n_*-1) ln(k/k_*) + {1/2} n'_* ln^2(k/k_*)$. It is reasonable to truncate the Taylor series if $|n'_* ln(k/k_*)| << |n_*-1|$, but it is not if $|n'_* ln(k/k_*)| \gtrsim |n_*-1|$. We argue that there is no good theoretical reason to prefer $|n'_*| << |n_*-1|$, and show that current observations are consistent with $|n'_* ln(k/k_*)| ~ |n_*-1|$ even for $|ln(k/k_*)| ~ 1$. Thus, there are regions of parameter space, which are both theoretically and observationally relevant, for which the traditional truncated Taylor series parameterization is inconsistent, and hence it can lead to incorrect parameter estimations. Motivated by this, we propose a simple extension of the traditional parameterization, which uses no extra parameters, but that, unlike the traditional approach, covers well motivated inflationary spectra with $|n'_*| ~ |n_*-1|$. Our parameterization therefore covers not only standard-slow-roll inflation models but also a much wider class of inflation models. We use this parameterization to perform a likelihood analysis for the cosmological parameters.Comment: References added. Typo correcte

First Results from the AMoRE-Pilot neutrinoless double beta decay experiment

The Advanced Molybdenum-based Rare process Experiment (AMoRE) aims to search for neutrinoless double beta decay (0$\nu\beta\beta$) of $^{100}$Mo with $\sim$100 kg of $^{100}$Mo-enriched molybdenum embedded in cryogenic detectors with a dual heat and light readout. At the current, pilot stage of the AMoRE project we employ six calcium molybdate crystals with a total mass of 1.9 kg, produced from $^{48}$Ca-depleted calcium and $^{100}$Mo-enriched molybdenum ($^{48\textrm{depl}}$Ca$^{100}$MoO$_4$). The simultaneous detection of heat(phonon) and scintillation (photon) signals is realized with high resolution metallic magnetic calorimeter sensors that operate at milli-Kelvin temperatures. This stage of the project is carried out in the Yangyang underground laboratory at a depth of 700 m. We report first results from the AMoRE-Pilot $0\nu\beta\beta$ search with a 111 kg$\cdot$d live exposure of $^{48\textrm{depl}}$Ca$^{100}$MoO$_4$ crystals. No evidence for $0\nu\beta\beta$ decay of $^{100}$Mo is found, and a upper limit is set for the half-life of 0$\nu\beta\beta$ of $^{100}$Mo of $T^{0\nu}_{1/2} > 9.5\times10^{22}$ y at 90% C.L.. This limit corresponds to an effective Majorana neutrino mass limit in the range $\langle m_{\beta\beta}\rangle\le(1.2-2.1)$ eV

Simultaneous resonant x-ray diffraction measurement of polarization inversion and lattice strain in polycrystalline ferroelectrics

Structure-property relationships in ferroelectrics extend over several length scales from the individual unit cell to the macroscopic device, and with dynamics spanning a broad temporal domain. Characterizing the multi-scale structural origin of electric field-induced polarization reversal and strain in ferroelectrics is an ongoing challenge that so far has obscured its fundamental behaviour. By utilizing small intensity differences between Friedel pairs due to resonant scattering, we demonstrate a time-resolved X-ray diffraction technique for directly and simultaneously measuring both lattice strain and, for the first time, polarization reversal during in-situ electrical perturbation. This technique is demonstrated for BaTiO₃-BiZn₀.₅Ti₀.₅O₃ (BT-BZT) polycrystalline ferroelectrics, a prototypical lead-free piezoelectric with an ambiguous switching mechanism. This combines the benefits of spectroscopic and diffraction-based measurements into a single and robust technique with time resolution down to the ns scale, opening a new door to in-situ structure-property characterization that probes the full extent of the ferroelectric behaviour.This is the publisher’s final pdf. The published article is copyrighted by the author(s) and published by the Nature Publishing Group. The published article can be found at: http://www.nature.com/srep