528 research outputs found
Theory of cavity-polariton self-trapping and optical strain in polymer chains
We consider a semiconductor polymer chain coupled to a single electromagnetic
mode in a cavity. The excitations of the chain have a mixed exciton-photon
character and are described as polaritons. Polaritons are coupled to the
lattice by the deformation potential interaction and can propagate in the
chain. We find that the presence of optical excitation in the polymer induces
strain on the lattice. We use a BCS variational wavefunction to calculate the
chemical potential of the polaritons as a function of their density. We analyze
first the case of a short chain with only two unit cells in order to check the
validity of our variational approach. In the case of a long chain and for a
strong coupling with the lattice, the system undergoes a phase transition
corresponding to the self-trapping of polaritons. The role of the exciton
spontaneous emission and cavity damping are discussed in the case of
homogeneous optical lattice strain.Comment: 7 pages, 6 figure
Exciton-phonon effects in carbon nanotube optical absorption
We find that the optical properties of carbon nanotubes reflect remarkably
strong effects of exciton-phonon coupling. Tight-binding calculations show that
a significant fraction of the spectral weight of the absorption peak is
transferred to a distinct exciton+phonon sideband, which is peaked at around
200 meV above the main absorption peak. This sideband provides a distinctive
signature of the excitonic character of the optical transition. The
exciton-phonon coupling is reflected in a dynamical structural distortion,
which contributes a binding energy of up to 100 meV. The distortion is
surprisingly long-ranged, and is strongly dependent on chirality.Comment: 5 pages, 3 figure
In-plane ferromagnetism in charge-ordering
The magnetic and transport properties are systematically studied on the
single crystal with charge ordering and divergency in
resistivity below 50 K. A long-range ferromagnetic ordering is observed in
susceptibility below 20 K with the magnetic field parallel to Co-O plane, while
a negligible behavior is observed with the field perpendicular to the Co-O
plane. It definitely gives a direct evidence for the existence of in-plane
ferromagnetism below 20 K. The observed magnetoresistance (MR) of 30 % at the
field of 6 T at low temperatures indicates an unexpectedly strong spin-charge
coupling in triangle lattice systems.Comment: 4 pages, 5 figure
Optical Absorption Study by Ab initio Downfolding Approach: Application to GaAs
We examine whether essence and quantitative aspects of electronic excitation
spectra are correctly captured by an effective low-energy model constructed
from an {\em ab initio} downfolding scheme. A global electronic structure is
first calculated by {\em ab initio} density-functional calculations with the
generalized gradient approximation. With the help of constrained density
functional theory, the low-energy effective Hamiltonian for bands near the
Fermi level is constructed by the downfolding procedure in the basis of
maximally localized Wannier functions. The excited states of this low-energy
effective Hamiltonian ascribed to an extended Hubbard model are calculated by
using a low-energy solver. As the solver, we employ the Hartree-Fock
approximation supplemented by the single-excitation configuration-interaction
method considering electron-hole interactions. The present three-stage method
is applied to GaAs, where eight bands are retained in the effective model after
the downfolding. The resulting spectra well reproduce the experimental results,
indicating that our downfolding scheme offers a satisfactory framework of the
electronic structure calculation, particularly for the excitations and dynamics
as well as for the ground state.Comment: 14 pages, 6 figures, and 1 tabl
Mass enhancement in narrow band systems
A perturbative study of the Holstein Molecular Crystal Model which accounts
for lattice structure and dimensionality effects is presented. Antiadiabatic
conditions peculiar of narrow band materials and an intermediate to strong
electron-phonon coupling are assumed. The polaron effective mass depends
crucially in all dimensions on the intermolecular coupling strengths which also
affect the size of the lattice deformation associated with the small polaron
formation.Comment: Istituto Nazionale di Fisica della Materia - Dipartimento di
Matematica e Fisica, Istituto Nazionale di Fisica della Materia Universita'
di Camerino, 62032 Camerino, Ital
Negative Giant Longitudinal Magnetoresistance in NiMnSb/InSb: An interface effect
We report on the electrical and magneto-transport properties of the contact
formed between polycrystalline NiMnSb thin films grown using pulsed laser
deposition (PLD) and n-type degenerate InSb (100) substrates. A negative giant
magnetoresistance (GMR) effect is observed when the external magnetic field is
parallel to the surface of the film and to the current direction. We attribute
the observed phenomenon to magnetic precipitates formed during the magnetic
film deposition and confined to a narrow layer at the interface. The effect of
these precipitates on the magnetoresistance depends on the thermal processing
of the system.Comment: 14 pages, 4 figure
Polaron self-trapping in a honeycomb net
Small polaron behavior in a two dimensional honeycomb net is studied by
applying the strong coupling perturbative method to the Holstein molecular
crystal model. We find that small optical polarons can be mobile also if the
electrons are strongly coupled to the lattice. Before the polarons localize and
become very heavy, there is infact a window of {\it e-ph} couplings in which
the polarons are small and have masses of order times the bare
band mass according to the value of the adiabaticity parameter. The 2D
honeycomb net favors the mobility of small optical polarons in comparison with
the square lattice.Comment: 6 pages, 3 figures, to appear in J.Phys.:Condensed Matter {PACS:
63.10.+a, 63.20.Dj, 71.38.+i
Intersublevel Polaron Dephasing in Self-Assembled Quantum Dots
Polaron dephasing processes are investigated in InAs/GaAs dots using
far-infrared transient four wave mixing (FWM) spectroscopy. We observe an
oscillatory behaviour in the FWM signal shortly (< 5 ps) after resonant
excitation of the lowest energy conduction band transition due to coherent
acoustic phonon generation. The subsequent single exponential decay yields long
intraband dephasing times of 90 ps. We find excellent agreement between our
measured and calculated FWM dynamics, and show that both real and virtual
acoustic phonon processes are necessary to explain the temperature dependence
of the polarization decay.Comment: 10 pages, 4 figures, submitted to Phys Rev Let
Negative Magnetoresistance in (In,Mn)As
The magnetotransport properties of an In0.95Mn0.05As thin film grown by
metal-organic vapor phase epitaxy were measured. Resistivity was measured over
the temperature range of 5 to 300 K. The resistivity decreased with increasing
temperature from 90 ohm-cm to 0.05 ohm-cm. The field dependence of the low
temperature magnetoresistance was measured. A negative magnetoresistance was
observed below 17 K with a hysteresis in the magnetoresistance observed at 5 K.
The magnetoresistance as a function of applied field was described by the
Khosla-Fischer model for spin scattering of carriers in an impurity band.Comment: 8 pages, 4 figures, accepted to Physical Review
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