7,334 research outputs found

    Ground states with cluster structures in a frustrated Heisenberg chain

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    We examine the ground state of a Heisenberg model with arbitrary spin S on a one-dimensional lattice composed of diamond-shaped units. A unit includes two types of antiferromagnetic exchange interactions which frustrate each other. The system undergoes phase changes when the ratio λ\lambda between the exchange parameters varies. In some phases, strong frustration leads to larger local structures or clusters of spins than a dimer. We prove for arbitrary S that there exists a phase with four-spin cluster states, which was previously found numerically for a special value of λ\lambda in the S=1/2 case. For S=1/2 we show that there are three ground state phases and determine their boundaries.Comment: 4 pages, uses revtex.sty, 2 figures available on request from [email protected], to be published in J. Phys.: Cond. Mat

    Spin Gap of Two-Dimensional Antiferromagnet Representing CaV4_4O9_9

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    We examined a two-dimensional Heisenberg model with two kinds of exchange energies, JeJ_e and JcJ_c. This model describes localized spins at vanadium ions in a layer of CaV4_4O9_9, for which a spin gap is found by a recent experiment. Comparing the high temperature expansion of the magnetic susceptibility to experimental data, we determined the exchange energies as JeJ_e \simeq 610 K and JcJ_c \simeq 150 K. By the numerical diagonalization we estimated the spin gap as Δ0.2Je\Delta \sim 0.2J_e \simeq 120 K, which consists with the experimental value 107 K. Frustration by finite JcJ_c enhances the spin gap.Comment: 12 pages of LaTex, 4 figures availavule upon reques

    Prebiotic Organic Microstructures

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    Micro- and sub-micrometer spheres, tubules and fiber-filament soft structures have been synthesized in our experiments conducted with 3 MeV proton irradiations of a mixture of simple inorganic constituents, CO, N2 and H2O. We analysed the irradiation products, with scanning electron microscopy (SEM) and atomic force microscopy (AFM). These laboratory organic structures produced wide variety of proteinous and non-proteinous amino acids after HCl hydrolysis. The enantiomer analysis for D-, L- alanine confirmed that the amino acids were abiotically synthesized during the laboratory experiment. Considering hydrothermal activity, the presence of CO2 and H2, of a ferromagnesian silicate mineral environment, of an Earth magnetic field which was much less intense during Archean times than nowadays and consequently of a proton excitation source which was much more abundant, we propose that our laboratory organic microstructures might be synthesized during Archean times. We show similarities in morphology and in formation with some terrestrial Archean microstructures and we suggest that some of the observed Archean carbon spherical and filamentous microstructures might be composed of abiogenic organic molecules. We further propose a search for such prebiotic organic signatures on Mars. This article has been posted on Nature precedings on 21 July 2010 [1]. Extinct radionuclides as source of excitation have been replaced by cosmic radiations which were much more intense 3.5 Ga ago because of a much less intense Earth magnetic field. The new version of the article has been presented at the ORIGINS conference in Montpellier in july 2011 [2] and has since been published in Origins of Life and Evolution of Biospheres 42 (4) 307-316, 2012. 
DOI: 10.1007/s11084-012-9290-5 

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    Boron Spectral Density and Disorder Broadening in B-doped Diamond

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    Comparison of periodic B dopants with a random alloy of substitional boron in diamond is carried out using several supercells and the coherent potential approximation (CPA) for the random alloy case. The main peak in the B local density of states is shifted to lower binding energy compared to the corresponding C peak in intrinsic diamond. In supercells, this shows up as strongly B-character bands split from bulk C bands away from the zone center,in an energy region around -1 eV. Even for a 4*4*4 supercell (BC127_{127}), effects of the dopant order are evident in the form of primarily B-character bands just below the Fermi level at the supercell zone boundary. The bands resulting from the CPA are of continuous mixed C-B character. They resemble virtual crystal bands, but broadened somewhat reflecting the disorder-induced lifetime, and are consistent with angle-resolved photoemission band maps. The B character is 1.7 times larger than for C (per atom) near the top of the valence bands for CPA, and roughly the same for supercells. CPA results are particularly useful since they characterize the wavevector and energy dependence of disorder broadening.Comment: 8 pages and 9 embedded figures (To appear in PRB

    Numerical simulation of the world ocean circulation

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    A multi-level model, based on the primitive equations, is developed for simulating the temperature and velocity fields produced in the world ocean by differential heating and surface wind stress. The model ocean has constant depth, free slip at the lower boundary, and neglects momentum advection; so that there is no energy exchange between the barotropic and baroclinic components of the motion, although the former influences the latter through temperature advection. The ocean model was designed to be coupled to the UCLA atmospheric general circulation model, for the study of the dynamics of climate and climate changes. But here, the model is tested by prescribing the observed seasonally varying surface wind stress and the incident solar radiation, the surface air temperature and humidity, cloudiness and the surface wind speed, which, together with the predicted ocean surface temperature, determine the surface flux of radiant energy, sensible heat and latent heat

    Spin Gap of S=1/2 Heisenberg Model on Distorted Diamond Chain

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    We study the spin gap of the S=1/2 Heisenberg model on the distorted diamond chain, which is recently proposed to represent magnetic properties of Cu_3 Cl_6 (H_2 O)_2 2H_8 C_4 SO_2. This model is composed of stacked trimers and has three kinds of exchange interactions J_1, J_2 and J_3. Using the numerical diagonalization, we obtain a contour map of the spin gap in the J_2/J_1-J_3/J_1 plane. We argue possible values of the exchange constants based on the contour map and the observed value of the spin gap.Comment: 2 pages, 4 figure
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