Toward quantum processing in molecules: A THz-bandwidth coherent memory for light

The unusual features of quantum mechanics are enabling the development of technologies not possible with classical physics. These devices utilize nonclassical phenomena in the states of atoms, ions, and solid-state media as the basis for many prototypes. Here we investigate molecular states as a distinct alternative. We demonstrate a memory for light based on storing photons in the vibrations of hydrogen molecules. The THz-bandwidth molecular memory is used to store 100-fs pulses for durations up to 1ns, enabling 10,000 operational time bins. The results demonstrate the promise of molecules for constructing compact ultrafast quantum photonic technologies.Comment: 5 pages, 3 figures, 1 tabl

Ultrafast slow-light: Raman-induced delay of THz-bandwidth pulses

We propose and experimentally demonstrate a scheme to generate optically-controlled delays based on off-resonant Raman absorption. Dispersion in a transparency window between two neighboring, optically-activated Raman absorption lines is used to reduce the group velocity of broadband 765 nm pulses. We implement this approach in a potassium titanyl phosphate (KTP) waveguide at room temperature, and demonstrate Raman-induced delays of up to 140 fs for a 650-fs duration, 1.8-THz bandwidth, signal pulse; the available delay-bandwidth product is $\approx1$. Our approach is applicable to single photon signals, offers wavelength tunability, and is a step toward processing ultrafast photons.Comment: 5+4 pages, 4+2 figure

Intensity correlation holography for remote phase sensing and 3D imaging

Holography is an established technique for measuring the wavefront of optical signals through interferometric combination with a reference wave. Conventionally the integration time of a hologram is limited by the interferometer coherence time, thus making it challenging to prepare holograms of remote objects, especially using weak illumination. Here, we circumvent this limitation by using intensity correlation interferometry. Although the exposure time of individual holograms must be shorter than the interferometer coherence time, we show that any number of randomly phase-shifted holograms can be combined into a single intensity-correlation hologram. In a proof-of-principle experiment, we use this technique to perform phase imaging and 3D reconstruction of an object at a ~3m distance using weak illumination and without active phase stabilization.Comment: 10 pages; 3 figure

Metrics Pilot Project for Military Avionics Sustainment: Experimental Design and Implementation Plan

This working paper outlines the design of an experiment, employing a pilot project, for identifying and validating new metrics for managing the US Air Force military avionics sustainment system. The paper also presents a plan for implementing the pilot project. The experimental design allows for the quantitifation of the effects of the new metrics, while controlling for the effects of other factors impacting the observed outcomes. Underlying the pilot project, and the proposed experimental design, are three main hypotheses derived from earlier research: (a) currently used metrics foster local optimization rather than system-wide optimization; (b) they do not allow measures of progress towards the achievement of system-wide goals and objectives, and, hence, do not allow visibility into the impact of depot maintenance on the warfighter; and (c) they are driving the “wrong behavior,” causing suboptimal decisions governing maintenance and repair priorities and practices and, as a result, undermining the efficiency and effectiveness of the sustainment system, despite the fact that the Air Force sustainment system has a dedicated and highly skilled workforce supporting the warfighter

Characterisation of a single photon event camera for quantum imaging

We show a simple yet effective method that can be used to characterize the per pixel quantum efficiency and temporal resolution of a single photon event camera for quantum imaging applications. Utilizing photon pairs generated through spontaneous parametric down-conversion, the detection efficiency of each pixel, and the temporal resolution of the system, are extracted through coincidence measurements. We use this method to evaluate the TPX3CAM, with appended image intensifier, and measure an average efficiency of 7.4% and a temporal resolution of 7.3ns. Furthermore, this technique reveals important error mechanisms that can occur in post-processing. We expect that this technique, and elements therein, will be useful to characterise other quantum imaging systems.Comment: 9 pages, 5 figure

Reconfigurable phase contrast microscopy with correlated photon pairs

A phase-sensitive microscopy technique is proposed and demonstrated that employs the momentum correlations inherent in spontaneous parametric down-conversion. One photon from a correlated pair is focused onto a microscopic target while the other is measured in the Fourier plane. This provides knowledge of the position and angle of illumination for every photon striking the target, allowing full post-production control of the illumination angle used to form an image. The versatility of this approach is showcased with asymmetric illumination and differential phase contrast imaging, without any beam blocks or moving parts.Comment: 5 pages, 3 figure

Time-bin to Polarization Conversion of Ultrafast Photonic Qubits

The encoding of quantum information in photonic time-bin qubits is apt for long distance quantum communication schemes. In practice, due to technical constraints such as detector response time, or the speed with which co-polarized time-bins can be switched, other encodings, e.g. polarization, are often preferred for operations like state detection. Here, we present the conversion of qubits between polarization and time-bin encodings using a method that is based on an ultrafast optical Kerr shutter and attain efficiencies of 97% and an average fidelity of 0.827+/-0.003 with shutter speeds near 1 ps. Our demonstration delineates an essential requirement for the development of hybrid and high-rate optical quantum networks

Time-resolved photoelectron imaging of excited state relaxation dynamics in phenol, catechol, resorcinol and hydroquinone

Time-resolved photoelectron imaging was used to investigate the dynamical evolution of the initially prepared S1 (\u3c0\u3c0*) excited state of phenol (hydroxybenzene), catechol (1,2-dihydroxybenzene), resorcinol (1,3-dihydroxybenzene), and hydroquinone (1,4-dihydroxybenzene) following excitation at 267 nm. Our analysis was supported by ab initio calculations at the coupled-cluster and CASSCF levels of theory. In all cases, we observe rapid (<1 ps) intramolecular vibrational redistribution on the S1potential surface. In catechol, the overall S1 state lifetime was observed to be 12.1 ps, which is 1\u20132 orders of magnitude shorter than in the other three molecules studied. This may be attributed to differences in the H atom tunnelling rate under the barrier formed by a conical intersection between the S1 state and the close lying S2 (\u3c0\u3c3*) state, which is dissociative along the O\u2013H stretching coordinate. Further evidence of this S1/S2 interaction is also seen in the time-dependent anisotropy of the photoelectron angular distributions we have observed. Our data analysis was assisted by a matrix inversion method for processing photoelectron images that is significantly faster than most other previously reported approaches and is extremely quick and easy to implement.Peer reviewed: YesNRC publication: Ye