15 research outputs found
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Variations in the vertical profile of ozone at four high-latitude Arctic sites from 2005 to 2017
Understanding variations in atmospheric ozone in the Arctic is difficult because there are only a few long-term records of vertical ozone profiles in this region. We present 12 years of ozone profiles from February 2005 to February 2017 at four sites: Summit Station, Greenland; Ny-Alesund, Svalbard, Norway; and Alert and Eureka, Nunavut, Canada. These profiles are created by combining ozonesonde measurements with ozone profile retrievals using data from the Microwave Limb Sounder (MLS). This combination creates a high-quality dataset with low uncertainty values by relying on in situ measurements of the maximum altitude of the ozonesondes (similar to 30 km) and satellite retrievals in the upper atmosphere (up to 60 km). For each station, the total column ozone (TCO) and the partial column ozone (PCO) in four atmospheric layers (troposphere to upper stratosphere) are analyzed. Overall, the seasonal cycles are similar at these sites. However, the TCO over Ny-Alesund starts to decline 2 months later than at the other sites. In summer, the PCO in the upper stratosphere over Summit Station is slightly higher than at the other sites and exhibits a higher standard deviation. The decrease in PCO in the middle and upper stratosphere during fall is also lower over Summit Station. The maximum value of the lower- and middle-stratospheric PCO is reached earlier in the year over Eureka. Trend analysis over the 12-year period shows significant trends in most of the layers over Summit and Ny-Alesund during summer and fall. To understand deseasonalized ozone variations, we identify the most important dynamical drivers of Arctic ozone at each level. These drivers are chosen based on mutual selected proxies at the four sites using stepwise multiple regression (SMR) analysis of various dynamical parameters with deseasonalized data. The final regression model is able to explain more than 80 % of the TCO and more than 70 % of the PCO in almost all of the layers. The regression model provides the greatest explanatory value in the middle stratosphere. The important proxies of the deseasonalized ozone time series at the four sites are tropopause pressure (TP) and equivalent latitude (EQL) at 370 K in the troposphere, the quasi-biennial oscillation (QBO) in the troposphere and lower stratosphere, the equivalent latitude at 550 K in the middle and upper stratosphere, and the eddy heat flux (EHF) and volume of polar stratospheric clouds throughout the stratosphere.</p
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Characterizing sources of high surface ozone events in the southwestern US with intensive field measurements and two global models
The detection and attribution of high background ozone (O3) events in the southwestern US is challenging but relevant to the effective implementation of the lowered National Ambient Air Quality Standard (NAAQS; 70 ppbv). Here we leverage intensive field measurements from the Fires, Asian, and Stratospheric Transport−Las Vegas Ozone Study (FAST-LVOS) in May–June 2017, alongside high-resolution simulations with two global models (GFDL-AM4 and GEOS-Chem), to study the sources of O3 during high-O3 events. We show possible stratospheric influence on 4 out of the 10 events with daily maximum 8 h average (MDA8) surface O3 above 65 ppbv in the greater Las Vegas region. While O3 produced from regional anthropogenic emissions dominates pollution events in the Las Vegas Valley, stratospheric intrusions can mix with regional pollution to push surface O3 above 70 ppbv. GFDL-AM4 captures the key characteristics of deep stratospheric intrusions consistent with ozonesondes, lidar profiles, and co-located measurements of O3, CO, and water vapor at Angel Peak, whereas GEOS-Chem has difficulty simulating the observed features and underestimates observed O3 by ∼20 ppbv at the surface. On days when observed MDA8 O3 exceeds 65 ppbv and the AM4 stratospheric ozone tracer shows 20–40 ppbv enhancements, GEOS-Chem simulates ∼15 ppbv lower US background O3 than GFDL-AM4. The two models also differ substantially during a wildfire event, with GEOS-Chem estimating ∼15 ppbv greater O3, in better agreement with lidar observations. At the surface, the two models bracket the observed MDA8 O3 values during the wildfire event. Both models capture the large-scale transport of Asian pollution, but neither resolves some fine-scale pollution plumes, as evidenced by aerosol backscatter, aircraft, and satellite measurements. US background O3 estimates from the two models differ by 5 ppbv on average (greater in GFDL-AM4) and up to 15 ppbv episodically. Uncertainties remain in the quantitative attribution of each event. Nevertheless, our multi-model approach tied closely to observational analysis yields some process insights, suggesting that elevated background O3 may pose challenges to achieving a potentially lower NAAQS level (e.g., 65 ppbv) in the southwestern US.
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Assessing Gender Bias in Particle Physics and Social Science Recommendations for Academic Jobs
We investigated gender bias in letters of recommendation as a possible cause of the under-representation of women in Experimental Particle Physics (EPP), where about 15% of faculty are female—well below the 60% level in psychology and sociology. We analyzed 2206 letters in EPP and these two social sciences using standard lexical measures as well as two new measures: author status and an open-ended search for gendered language. In contrast to former studies, women were not depicted as more communal, less agentic, or less standout. Lexical measures revealed few gender differences in either discipline. The open-ended analysis revealed disparities favoring women in social science and men in EPP. However, female EPP candidates were characterized as “brilliant” in nearly three times as many letters as were men
First reprocessing of Southern Hemisphere ADditional OZonesondes (SHADOZ) profile records (1998-2015): 1. Methodology and evaluation
International audienc
The Fires, Asian, and Stratospheric Transport-Las Vegas Ozone Study (FAST-LVOS)
Abstract. The Fires, Asian, and Stratospheric Transport-Las Vegas Ozone Study (FAST-LVOS) was conducted in May and June of 2017 to study the transport of ozone (O3) to Clark County, Nevada, a marginal non-attainment area in the Southwestern U.S. (SWUS). This 6-week (20 May–30 June 2017) field campaign used lidar, ozonesonde, aircraft, and in-situ measurements in conjunction with a variety of models to characterize the distribution of O3 and related species above southern Nevada and neighbouring California, and to probe the influence of stratospheric intrusions, wildfires, and local, regional, and Asian pollution on surface O3 concentrations in Las Vegas and the surrounding area. In this paper, we describe the FAST-LVOS campaign and present case studies illustrating the influence of different transport processes on background O3 and air quality attainment in the SWUS. The measurements found elevated O3 layers above Las Vegas on more than 75 % (35 of 45) of the sample days, and show that entrainment of these layers contributed to mean 8-h average background O3 concentrations of 50–55 parts-per-billion by volume (ppbv) across southern Nevada. These background concentrations constitute 70–80 % of the current U.S. National Ambient Air Quality Standard (NAAQS) of 70 ppbv, and illustrate some of the challenges facing air quality managers tasked with O3 attainment in the SWUS during late spring and early summer. The companion paper by Zhang et al. (2020) describes the use of the AM4 and GEOS-Chem global models to estimate the impacts of transported O3 on surface air quality in the Southwestern U.S. and Intermountain West during the FAST-LVOS campaign
The <i>Fires, Asian, and Stratospheric Transport</i>–Las Vegas Ozone Study (<i>FAST</i>-LVOS)
International audienceAbstract. The Fires, Asian, and Stratospheric Transport–Las Vegas Ozone Study (FAST-LVOS) was conducted in May and June of 2017 to study the transport of ozone (O3) to Clark County, Nevada, a marginal non-attainment area in the southwestern United States (SWUS). This 6-week (20 May–30 June 2017) field campaign used lidar, ozonesonde, aircraft, and in situ measurements in conjunction with a variety of models to characterize the distribution of O3 and related species above southern Nevada and neighboring California and to probe the influence of stratospheric intrusions and wildfires as well as local, regional, and Asian pollution on surface O3 concentrations in the Las Vegas Valley (≈ 900 m above sea level, a.s.l.). In this paper, we describe the FAST-LVOS campaign and present case studies illustrating the influence of different transport processes on background O3 in Clark County and southern Nevada. The companion paper by Zhang et al. (2020) describes the use of the AM4 and GEOS-Chem global models to simulate the measurements and estimate the impacts of transported O3 on surface air quality across the greater southwestern US and Intermountain West. The FAST-LVOS measurements found elevated O3 layers above Las Vegas on more than 75 % (35 of 45) of the sample days and show that entrainment of these layers contributed to mean 8 h average regional background O3 concentrations of 50–55 parts per billion by volume (ppbv), or about 85–95 µg m−3. These high background concentrations constitute 70 %–80 % of the current US National Ambient Air Quality Standard (NAAQS) of 70 ppbv (≈ 120 µg m−3 at 900 m a.s.l.) for the daily maximum 8 h average (MDA8) and will make attainment of the more stringent standards of 60 or 65 ppbv currently being considered extremely difficult in the interior SWUS