753 research outputs found
Effects of in-chain and off-chain substitutions on spin fluctuations in the spin-Peierls compound CuGeO_3
The effect of in-chain and off-chain substitutions on 1D spin fluctuations in
the spin-Peierls compound CuGeO_3 has been studied using Raman scattering in
order to understand the interplay between defect induced states, enhanced
spin-spin correlations and the ground state of low dimensional systems.
In-chain and off-chain substitutions quench the spin-Peierls state and induce
3D antiferromagnetic order at T\leq 5 K. Consequently a suppression of a 1D
gap-induced mode as well as a constant intensity of a spinon continuum are
observed at low temperatures. A 3D two-magnon density of states now gradually
extends to higher temperatures T\leq 60K compared with pure CuGeO_3. This
effect is more pronounced in the case of off-chain substitutions (Si) for which
a N\'eel state occurs over a larger substitution range, starting at very low
concentrations. Besides, additional low energy excitations are induced. These
effects, i.e. the shift of a dimensional crossover to higher temperatures are
due to an enhancement of the spin-spin correlations induced by a small amount
of substitutions. The results are compared with recent Monte Carlo studies on
substituted spin ladders, pointing to a similar instability of coupled,
dimerized spin chains and spin ladders upon substitution.Comment: 14 pages, 6 eps figures, to be published in PR
Charge-Doping driven Evolution of Magnetism and non-Fermi-Liquid Behavior in the Filled Skutterudite CePt4Ge12-xSbx
The filled-skutterudite compound CePt4Ge12 is situated close to the border
between intermediate-valence of Ce and heavy-fermion behavior. Substitution of
Ge by Sb drives the system into a strongly correlated and ultimately upon
further increasing the Sb concentration into an antiferromagnetically ordered
state. Our experiments evidence a delicate interplay of emerging Kondo physics
and the formation of a local 4f moment. An extended non-Fermi-liquid region,
which can be understood in the framework of a Kondo-disorder model, is
observed. Band-structure calculations support the conclusion that the physical
properties are governed by the interplay of electron supply via Sb substitution
and the concomitant volume effects.Comment: 5 pages, 3 Figur
Investigation of the Spin-Peierls transition in CuGeO_3 by Raman scattering
Raman experiments on the spin-Peierls compound CuGeO and the substituted
(Cu,Zn)GeO and Cu(Ge,Ga)O compounds were
performed in order to investigate the response of specific magnetic excitations
of the one-dimensional spin-1/2 chain to spin anisotropies and
substitution-induced disorder. In pure CuGeO, in addition to normal phonon
scattering which is not affected at all by the spin-Peierls transition, four
types of magnetic scattering features were observed. Below T=14 K a
singlet-triplet excitation at 30 cm, two-magnon scattering from 30 to
227 cm and folded phonon modes at 369 and 819 cm were identified.
They were assigned by their temperature dependence and lineshape. For
temperatures between the spin-Peierls transition T and approximately 100
K a broad intensity maximum centered at 300 cm is observed.Comment: 7 pages, LaTex2e, including 3 figures (eps) to be published in
Physica B (1996
Substitution effects on spin fluctuations in the spin-Peierls compound CuGeO_3
Using Raman scattering we studied the effect of substitutions on 1D spin
fluctuations in CuGeO_3 observed as a spinon continuum in frustration induced
exchange scattering. For temperatures below the spin-Peierls transition
(T_{SP}=14K) the intensity of this continuum at 120-500 cm^{-1} is
exponentially suppressed and transferred into a 3D two-magnon density of
states. Besides a spin-Peierls gap-induced mode at 30 cm^{-1} and additional
modes at 105 and 370 cm^{-1} are observed. Substitution of Zn on the Cu-site
and Si on the Ge-site of CuGeO_3 quenches easily the spin-Peierls state.
Consequently a suppression of the spin-Peierls gap observable below T_{SP}=14K
as well as a change of the temperature dependence of the spinon continuum are
observed. These effects are discussed in the context of a dimensional crossover
of this compound below T_{SP} and strong spin-lattice interaction.Comment: 9 pages, 2 eps figures include
Kondo effect in Ce(x)La(1-x)Cu(2.05)Si(2) intermetallics
The magnetic susceptibility and susceptibility anisotropy of the quasi-binary
alloy system Ce(x)La(1-x)Cu(2.05)Si(2) have been studied for low concentration
of Ce ions. The single-ion desc ription is found to be valid for x < 0.1. The
experimental results are discussed in terms of t he degenerate
Coqblin-Schrieffer model with a crystalline electric field splitting Delta =
330 K. The properties of the model, obtained by combining the lowest-order
scaling and the pertur bation theory, provide a satisfactory description of the
experimental data down to 30 K. The e xperimental results between 20 K and 2 K
are explained by the exact solution of the Kondo mode l for an effective
doublet.Comment: 11 pages, 13 Postscript figures, 1 tabl
Electron and hole transmission through superconductor - normal metal interfaces
We have investigated the transmission of electrons and holes through
interfaces between superconducting aluminum (Tc = 1.2 K) and various normal
non-magnetic metals (copper, gold, palladium, platinum, and silver) using
Andreev-reflection spectroscopy at T = 0.1 K. We analyzed the point contacts
with the modified BTK theory that includes Dynes' lifetime as a fitting
parameter G in addition to superconducting energy gap 2D and normal reflection
described by Z. For contact areas from 1 nm^2 to 10000 nm^2 the BTK Z parameter
was 0.5, corresponding to transmission coefficients of about 80 %, independent
of the normal metal. The very small variation of Z indicates that the
interfaces have a negligible dielectric tunneling barrier. Fermi surface
mismatch does not account for the observed transmission coefficient.Comment: 9 pages, 4 figures, submitted to Proceedings of the 19th
International Conference on Magnetism ICM2012 (Busan 2012
Crystallographic disorder and electron scattering on structural two-level systems in ZrAs1.4Se0.5
Single crystals of ZrAs1.4Se0.5 (PbFCl type structure) were grown by chemical
vapour transport. While their thermodynamic and transport properties are
typical for ordinary metals, the electrical resistivity exhibits a shallow
minimum at low temperatures. Application of strong magnetic fields does not
influence this anomaly. The minimum of the resistivity in ZrAs1.4Se0.5
apparently originates from interaction between the conduction electrons and
structural two-level systems. Significant disorder in the As-Se substructure is
inferred from X-ray diffraction and electron microprobe studies
Magnetism and unconventional superconductivity in CeMIn heavy-fermion crystals
We review magnetic, superconducting and non-Fermi-liquid properties of the
structurally layered heavy-fermion compounds CeMIn (M=Co, Rh,
Ir). These properties suggest d-wave superconductivity and proximity to an
antiferromagetic quantum-critical point.Comment: submitted 23rd International Conference on Low Temperature Physics
(LT-23), Aug. 200
Phase Diagram of the Two-Channel Kondo Lattice
The phase diagram of the two-channel Kondo lattice model is examined with a
Quantum Monte Carlo simulation in the limit of infinite dimensions.
Commensurate (and incommensurate) antiferromagnetic and superconducting states
are found. The antiferromagnetic transition is very weak and continuous;
whereas the superconducting transition is discontinuous to an odd-frequency
channel-singlet and spin-singlet pairing state.Comment: 5 pages, LaTeX and 4 PS figures (see also cond-mat/9609146 and
cond-mat/9605109
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