566 research outputs found
Magnetic order in the frustrated Ising-like chain compound SrNiIrO
We have studied the field and temperature dependence of the magnetization of
single crystals of Sr3NiIrO6. These measurements evidence the presence of an
easy axis of anisotropy and two anomalies in the magnetic susceptibility.
Neutron powder diffraction realized on a polycrystalline sample reveals the
emergence of magnetic reflections below 75 K with magnetic propagation vector k
~ (0, 0, 1), undetected in previous neutron studies [T.N. Nguyen and H.-C zur
Loye, J. Solid State Chem., 117, 300 (1995)]. The nature of the magnetic ground
state, and the presence of two anomalies common to this family of material, are
discussed on the basis of the results obtained by neutron diffraction,
magnetization measurements, and symmetry arguments
Domain Wall Spin Dynamics in Kagome Antiferromagnets
We report magnetization and neutron scattering measurements down to 60 mK on
a new family of Fe based kagome antiferromagnets, in which a strong local spin
anisotropy combined with a low exchange path network connectivity lead to
domain walls intersecting the kagome planes through strings of free spins.
These produce unfamiliar slow spin dynamics in the ordered phase, evolving from
exchange-released spin-flips towards a cooperative behavior on decreasing the
temperature, probably due to the onset of long-range dipolar interaction. A
domain structure of independent magnetic grains is obtained that could be
generic to other frustrated magnets.Comment: 5 pages, 4 figure
Subtle competition between ferromagnetic and antiferromagnetic order in a Mn(II) - free radical ferrimagnetic chain
The macroscopic magnetic characterization of the Mn(II) - nitronyl nitroxide
free radical chain (Mn(hfac)2(R)-3MLNN) evidenced its transition from a
1-dimensional behavior of ferrimagnetic chains to a 3-dimensional ferromagnetic
long range order below 3 K. Neutron diffraction experiments, performed on a
single crystal around the transition temperature, led to a different conclusion
: the magnetic Bragg reflections detected below 3 K correspond to a canted
antiferromagnet where the magnetic moments are mainly oriented along the chain
axis. Surprisingly in the context of other compounds in this family of magnets,
the interchain coupling is antiferromagnetic. This state is shown to be very
fragile since a ferromagnetic interchain arrangement is recovered in a weak
magnetic field. This peculiar behavior might be explained by the competition
between dipolar interaction, shown to be responsible for the antiferromagnetic
long range order below 3 K, and exchange interaction, the balance between these
interactions being driven by the strong intrachain spin correlations. More
generally, this study underlines the need, in this kind of molecular compounds,
to go beyond macroscopic magnetization measurements.Comment: 12 pages, 10 figures, submitted to Phys. Rev.
Formation of collective spins in frustrated clusters
Using magnetization, specific heat and neutron scattering measurements, as
well as exact calculations on realistic models, the magnetic properties of the
\lacuvo compound are characterized on a wide temperature range. At high
temperature, this oxide is well described by strongly correlated atomic =1/2
spins while decreasing the temperature it switches to a set of weakly
interacting and randomly distributed entangled pseudo spins and
. These pseudo-spins are built over frustrated clusters, similar to
the kagom\'e building block, at the vertices of a triangular superlattice, the
geometrical frustration intervening then at different scales.Comment: 10 page
Magnetoelectric MnPS3 thiophosphate as a new candidate for ferrotoroidicity
We have revisited the magnetic structure of manganese phosphorus trisulfide
MnPS3 using neutron diffrac- tion and polarimetry. MnPS3 undergoes a transition
toward a collinear antiferromagnetic order at 78 K. The resulting magnetic
point-group breaks both the time reversal and the space inversion thus allowing
a linear magnetoelectric coupling. Neutron polarimetry was subsequently used to
prove that this coupling provides a way to manipulate the antiferromagnetic
domains simply by cooling the sample under crossed magnetic and electrical
fields, in agreement with the nondiagonal form of the magnetoelectric tensor.
In addition, this tensor has, in principle, an antisymmetric part that results
in a toroidic moment and provides with a pure ferrotoroidic compound
Meeting report : 1st international functional metagenomics workshop May 7–8, 2012, St. Jacobs, Ontario, Canada
This report summarizes the events of the 1st International Functional Metagenomics Workshop. The workshop was held on May 7 and 8 in St. Jacobs, Ontario, Canada and was focused on building a core international functional metagenomics community, exploring strategic research areas, and identifying opportunities for future collaboration and funding. The workshop was initiated by researchers at the University of Waterloo with support from the Ontario Genomics Institute (OGI), Natural Sciences and Engineering Research Council of Canada (NSERC) and the University of Waterloo
Kitaev interactions in the Co honeycomb antiferromagnets Na3Co2SbO6 and Na2Co2TeO6
Co ions in an octahedral crystal field, stabilise a j = 1/2
ground state with an orbital degree of freedom and have been recently put
forward for realising Kitaev interactions, a prediction we have tested by
investigating spin dynamics in two cobalt honeycomb lattice compounds,
NaCoTeO and NaCoSbO, using inelastic neutron
scattering. We used linear spin wave theory to show that the magnetic spectra
can be reproduced with a spin Hamiltonian including a dominant Kitaev
nearest-neighbour interaction, weaker Heisenberg interactions up to the third
neighbour and bond-dependent off-diagonal exchange interactions. Beyond the
Kitaev interaction that alone would induce a quantum spin liquid state, the
presence of these additional couplings is responsible for the zigzag-type
long-range magnetic ordering observed at low temperature in both compounds.
These results provide evidence for the realization of Kitaev-type coupling in
cobalt-based materials, despite hosting a weaker spin-orbit coupling than their
4d and 5d counterparts
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