Faithful test of non-local realism with entangled coherent states

We investigate the violation of Leggett's inequality for non-local realism using entangled coherent states and various types of local measurements. We prove mathematically the relation between the violation of the Clauser-Horne-Shimony-Holt form of Bell's inequality and Leggett's one when tested by the same resources. For Leggett inequalities, we generalize the non-local realistic bound to systems in Hilbert spaces larger than bidimensional ones and introduce an optimization technique that allows to achieve larger degrees of violation by adjusting the local measurement settings. Our work describes the steps that should be performed to produce a self-consistent generalization of Leggett's original arguments to continuous-variable states.Comment: 8 pages, 6 figures, to be published in Phys. Rev.

A generalized structure of Bell inequalities for bipartite arbitrary dimensional systems

We propose a generalized structure of Bell inequalities for arbitrary d-dimensional bipartite systems, which includes the existing two types of Bell inequalities introduced by Collins-Gisin-Linden-Massar-Popescu [Phys. Rev. Lett. 88, 040404 (2002)] and Son-Lee-Kim [Phys. Rev. Lett. 96, 060406 (2006)]. We analyze Bell inequalities in terms of correlation functions and joint probabilities, and show that the coefficients of correlation functions and those of joint probabilities are in Fourier transform relations. We finally show that the coefficients in the generalized structure determine the characteristics of quantum violation and tightness.Comment: 6 pages, 1 figur

Effects of squeezing on quantum nonlocality of superpositions of coherent states

We analyze effects of squeezing upon superpositions of coherent states (SCSs) and entangled coherent states (ECSs) for Bell-inequality tests. We find that external squeezing can always increase the degrees of Bell violations, if the squeezing direction is properly chosen, for the case of photon parity measurements. On the other hand, when photon on/off measurements are used, the squeezing operation can enhance the degree of Bell violations only for moderate values of amplitudes and squeezing. We point out that a significant improvement is required over currently available squeezed SCSs in order to directly demonstrate a Bell-inequality violation in a real experiment.Comment: 7 pages, 4 figures, accepted for publication in Phys. Rev.

Inverted polymer fullerene solar cells exceeding 10% efficiency with poly(2-ethyl-2-oxazoline) nanodots on electron-collecting buffer layers

Polymer solar cells have been spotlighted due to their potential for low-cost manufacturing but their efficiency is still less than required for commercial application as lightweight/flexible modules. Forming a dipole layer at the electron-collecting interface has been suggested as one of the more attractive approaches for efficiency enhancement. However, only a few dipole layer material types have been reported so far, including only one non-ionic (charge neutral) polymer. Here we show that a further neutral polymer, namely poly(2-ethyl-2-oxazoline) (PEOz) can be successfully used as a dipole layer. Inclusion of a PEOz layer, in particular with a nanodot morphology, increases the effective work function at the electron-collecting interface within inverted solar cells and thermal annealing of PEOz layer leads to a state-of-the-art 10.74% efficiency for single-stack bulk heterojunction blend structures comprising poly[4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)benzo[1,2-b:4,5-b′]dithiophene-alt-3-fluorothieno[3,4-b]thiophene-2-carboxylate] as donor and [6,6]-phenyl-C71-butyric acid methyl ester as acceptor