Excitation and characterization of long-lived hydrogenic Rydberg states of nitric oxide

High Rydberg states of nitric oxide (NO) with principal quantum numbers between 40 and 100 and lifetimes in excess of 10 $\mu$s have been prepared by resonance enhanced two-color two-photon laser excitation from the X $^2\Pi_{1/2}$ ground state through the A $^2\Sigma^+$ intermediate state. Molecules in these long-lived Rydberg states were detected and characterized 126 $\mu$s after laser photoexcitation by state-selective pulsed electric field ionization. The laser excitation and electric field ionization data were combined to construct two-dimensional spectral maps. These maps were used to identify the rotational states of the NO$^+$ ion core to which the observed series of long-lived hydrogenic Rydberg states converge. The results presented pave the way for Rydberg-Stark deceleration and electrostatic trapping experiments with NO, which are expected to shed further light on the decay dynamics of these long-lived excited states, and are of interest for studies of ion-molecule reactions at low temperatures.Comment: 12 pages, 10 figure

Coupling Rydberg atoms to microwave fields in a superconducting coplanar waveguide resonator

Rydberg helium atoms traveling in pulsed supersonic beams have been coupled to microwave fields in a superconducting coplanar waveguide (CPW) resonator. The atoms were initially prepared in the 1s55s $^3$S$_1$ Rydberg level by two-color two-photon laser excitation from the metastable 1s2s $^3$S$_1$ level. Two-photon microwave transitions between the 1s55s $^3$S$_1$ and 1s56s $^3$S$_1$ levels were then driven by the 19.556 GHz third-harmonic microwave field in a quarter-wave CPW resonator. This superconducting microwave resonator was fabricated from niobium nitride on a silicon substrate and operated at temperatures between 3.65 and 4.30 K. The populations of the Rydberg levels in the experiments were determined by state-selective pulsed electric field ionization. The coherence of the atom-resonator coupling was studied by time-domain measurements of Rabi oscillations.Comment: 6 pages, 5 figure

The scattering map in two coupled piecewise-smooth systems, with numerical application to rocking blocks

We consider a non-autonomous dynamical system formed by coupling two piecewise-smooth systems in \RR^2 through a non-autonomous periodic perturbation. We study the dynamics around one of the heteroclinic orbits of one of the piecewise-smooth systems. In the unperturbed case, the system possesses two $C^0$ normally hyperbolic invariant manifolds of dimension two with a couple of three dimensional heteroclinic manifolds between them. These heteroclinic manifolds are foliated by heteroclinic connections between $C^0$ tori located at the same energy levels. By means of the {\em impact map} we prove the persistence of these objects under perturbation. In addition, we provide sufficient conditions of the existence of transversal heteroclinic intersections through the existence of simple zeros of Melnikov-like functions. The heteroclinic manifolds allow us to define the {\em scattering map}, which links asymptotic dynamics in the invariant manifolds through heteroclinic connections. First order properties of this map provide sufficient conditions for the asymptotic dynamics to be located in different energy levels in the perturbed invariant manifolds. Hence we have an essential tool for the construction of a heteroclinic skeleton which, when followed, can lead to the existence of Arnol'd diffusion: trajectories that, on large time scales, destabilize the system by further accumulating energy. We validate all the theoretical results with detailed numerical computations of a mechanical system with impacts, formed by the linkage of two rocking blocks with a spring

Driving Rydberg-Rydberg transitions from a co-planar microwave waveguide

The coherent interaction between ensembles of helium Rydberg atoms and microwave fields in the vicinity of a solid-state co-planar waveguide is reported. Rydberg-Rydberg transitions, at frequencies between 25 GHz and 38 GHz, have been studied for states with principal quantum numbers in the range 30 - 35 by selective electric-field ionization. An experimental apparatus cooled to 100 K was used to reduce effects of blackbody radiation. Inhomogeneous, stray electric fields emanating from the surface of the waveguide have been characterized in frequency- and time-resolved measurements and coherence times of the Rydberg atoms on the order of 250 ns have been determined.Comment: 5 pages, 5 figure

The Bell-Szekeres Solution and Related Solutions of the Einstein-Maxwell Equations

A novel technique for solving some head-on collisions of plane homogeneous light-like signals in Einstein-Maxwell theory is described. The technique is a by-product of a re-examination of the fundamental Bell-Szekeres solution in this field of study. Extensions of the Bell-Szekeres collision problem to include light-like shells and gravitational waves are described and a family of solutions having geometrical and topological properties in common with the Bell-Szekeres solution is derived.Comment: 18 pages, Latex fil