405 research outputs found

    The multiple quantum NMR dynamics in systems of equivalent spins with the dipolar ordered initial state

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    The multiple quantum (MQ) NMR dynamics in the system of equivalent spins with the dipolar ordered initial state is considered. The high symmetry of the MQ Hamiltonian is used in order to develop the analytical and numerical methods for an investigation of the MQ NMR dynamics in the systems consisting of hundreds of spins from "the first principles". We obtain the dependence of the intensities of the MQ NMR coherences on their orders (profiles of the MQ NMR coherences) for the systems of 200−600200 - 600 spins. It is shown that these profiles may be well approximated by the exponential distribution functions. We also compare the MQ NMR dynamics in the systems of equivalent spins having two different initial states, namely the dipolar ordered state and the thermal equilibrium state in the strong external magnetic field.Comment: 11 pages 4 figure

    Multiple Quantum NMR Dynamics in Dipolar Ordered Spin Systems

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    We investigate analytically and numerically the Multiple Quantum (MQ) NMR dynamics in systems of nuclear spins 1/2 coupled by the dipole-dipole interactions in the case of the dipolar ordered initial state. We suggest two different methods of MQ NMR. One of them is based on the measurement of the dipolar temperature in the quasi-equilibrium state which establishes after the time of order T2 after the MQ NMR experiment. The other method uses an additional resonance 45^0 -pulse after the preparation period of the standard MQ NMR experiment in solids. Many-spin clusters and correlations are created faster in such experiments than in the usual MQ NMR experiments and can be used for the investigation of many-spin dynamics of nuclear spins in solids.Comment: 11 pages, 3 figures. accepted for publication in Physical Review

    The high probability state transfers and entanglements between different nodes of the homogeneous spin 1/2 chain in inhomogeneous external magnetic field

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    We consider the high probability state transfers and entanglements between different nodes of the spin-1/2 chains governed by the XXZ-Hamiltonian using the inhomogeneous stationary external magnetic field. Examples of three-, four-, ten- and twenty-node chains are represented. A variant of realization of the proper inhomogeneous magnetic field is discussed.Comment: 16 pages, 2 figure

    Relationship between probabilities of the state transfers and entanglements in spin systems with simple geometrical configurations

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    In this paper we derive analytical relations between probabilities of the excited state transfers and entanglements calculated by both the Wootters and positive partial transpose (PPT) criteria for the arbitrary spin system with single excited spin in the external magnetic field and Hamiltonian commuting with IzI_z. We apply these relations to study the arbitrary state transfers and entanglements in the simple systems of nuclear spins having two- and three-dimensional geometrical configurations with XXZXXZ Hamiltonian. It is shown that High-Probability State Transfers (HPSTs) are possible among all four nodes placed in the corners of the rectangle with the proper ratio of sides as well as among all eight nodes placed in the corners of the parallelepiped with the proper ratio of sides. Entanglements responsible for these HPSTs have been identified.Comment: 27pages, 10 figure

    Luminescence evidence for bulk and surface excitons in free xenon clusters

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    Cathodoluminescence spectra of free xenon clusters produced by condensation of xenon-argon gas mixtures in supersonic jets expanding into vacuum were studied. By varying initial experimental parameters, including xenon concentration, we could obtain clusters with a xenon core (300-3500 atoms) covered by an argon outer shell as well as shell-free xenon clusters (about 1500 atoms). The cluster size and temperature (about 40 K for both cases) were measured electronographically. Luminescence bands evidencing the existence of bulk and surface excitons were detected for shell-free xenon clusters. The emission from bulk excitons in small clusters is supposed to be due to processes of their multiple elastic reflections from the xenon-vacuum interface. A presence of an argon shell causes extinction of the excitonic bands. In addition, some new bands were found which have no analogs for bulk xenon cryosamples.Comment: The final modified version will be published in Phys. Rev. A 76 (2007
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