1,707 research outputs found

    Polar and magnetic order in GaV4Se8

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    In the present work, we provide results from specific heat, magnetic susceptibility, dielectric constant, ac conductivity, and electrical polarization measurements performed on the lacunar spinel GaV4Se8. With decreasing temperature, we observe a transition from the paraelectric and paramagnetic cubic state into a polar, probably ferroelectric state at 42 K followed by magnetic ordering at 18 K. The polar transition is likely driven by the Jahn-Teller effect due to the degeneracy of the V4 cluster orbitals. The excess polarization arising in the magnetic phase indicates considerable magnetoelectric coupling. Overall, the behavior of GaV4Se8 in many respects is similar to that of the skyrmion host GaV4S8, exhibiting a complex interplay of orbital, spin, lattice, and polar degrees of freedom. However, its dielectric behavior at the polar transition markedly differs from that of the Jahn-Teller driven ferroelectric GeV4S8, which can be ascribed to the dissimilar electronic structure of the Ge compound.Comment: 7 pages, 6 figures. Revised version according to suggestions of referee

    Polar Dynamics at the Jahn-Teller Transition in Ferroelectric GaV4S8

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    We present a dielectric spectroscopy study of the polar dynamics linked to the orbitally driven ferroelectric transition in the skyrmion host GaV4S8. By combining THz and MHz-GHz spectroscopy techniques, we succeed in detecting the relaxational dynamics arising from coupled orbital and polar fluctuations in this material and traced its temperature dependence in the paraelectric as well as in the ferroelectric phase. The relaxation time significantly increases when approaching the critical temperature from both sides of the transition. It is natural to assume that these polar fluctuations map the orbital dynamics at the Jahn-Teller transition. Due to the first-order character of the orbital-ordering transition, the relaxation time shows an enormous jump of about five orders of magnitude at the polar and structural phase transition.Comment: 5 pages, 4 figure

    Quantum rainbow scattering at tunable velocities

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    Elastic scattering cross sections are measured for lithium atoms colliding with rare gas atoms and SF6 molecules at tunable relative velocities down to ~50 m/s. Our scattering apparatus combines a velocity-tunable molecular beam with a magneto-optic trap that provides an ultracold cloud of lithium atoms as a scattering target. Comparison with theory reveals the quantum nature of the collision dynamics in the studied regime, including both rainbows as well as orbiting resonances

    Completely splittable representations of affine Hecke-Clifford algebras

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    We classify and construct irreducible completely splittable representations of affine and finite Hecke-Clifford algebras over an algebraically closed field of characteristic not equal to 2.Comment: 39 pages, v2, added a new reference with comments in section 4.4, added two examples (Example 5.4 and Example 5.11) in section 5, mild corrections of some typos, to appear in J. Algebraic Combinatoric

    Structural Fluctuations in the Spin Liquid State of Tb2Ti2O7

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    High resolution X-ray scattering measurements on single crystal Tb2Ti2O7 reveal finite structural correlations at low temperatures. This geometrically frustrated pyrochlore is known to exhibit a spin liquid, or cooperative paramagnetic state, at temperatures below ~ 20 K. Parametric studies of structural Bragg peaks appropriate to the Fd3ˉ\bar{3}m space group of Tb2Ti2O7 reveal substantial broadening and peak intensity reduction in the temperature regime 20 K to 300 mK. We also observe a small, anomalous lattice expansion on cooling below a density maximum at ~ 18 K. These measurements are consistent with the development of fluctuations above a cooperative Jahn-Teller, cubic-tetragonal phase transition at very low temperatures.Comment: 5 pages, 4 figures, submitted for publicatio

    Magnetoelastics of a spin liquid: X-ray diffraction studies of Tb2Ti2O7 in pulsed magnetic fields

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    We report high resolution single crystal x-ray diffraction measurements of the frustrated pyrochlore magnet Tb2Ti2O7, collected using a novel low temperature pulsed magnet system. This instrument allows characterization of structural degrees of freedom to temperatures as low as 4.4 K, and in applied magnetic fields as large as 30 Tesla. We show that Tb2Ti2O7 manifests intriguing structural effects under the application of magnetic fields, including strongly anisotropic giant magnetostriction, a restoration of perfect pyrochlore symmetry in low magnetic fields, and ultimately a structural phase transition in high magnetic fields. It is suggested that the magnetoelastic coupling thus revealed plays a significant role in the spin liquid physics of Tb2Ti2O7 at low temperatures.Comment: 4 pages, 4 figures, submitted for publicatio

    Interplay of Spin-Orbit Interactions, Dimensionality, and Octahedral Rotations in Semimetallic SrIrO3_3

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    We employ reactive molecular-beam epitaxy to synthesize the metastable perovskite SrIrO3_{3} and utilize {\it in situ} angle-resolved photoemission to reveal its electronic structure as an exotic narrow-band semimetal. We discover remarkably narrow bands which originate from a confluence of strong spin-orbit interactions, dimensionality, and both in- and out-of-plane IrO6_6 octahedral rotations. The partial occupation of numerous bands with strongly mixed orbital characters signals the breakdown of the single-band Mott picture that characterizes its insulating two-dimensional counterpart, Sr2_{2}IrO4_{4}, illustrating the power of structure-property relations for manipulating the subtle balance between spin-orbit interactions and electron-electron interactions
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