Cavity ring-up spectroscopy for ultrafast sensing with optical microresonators

Spectroscopy of whispering-gallery mode (WGM) microresonators has become a powerful scientific tool, enabling detection of single viruses, nanoparticles, and even single molecules. Yet the demonstrated timescale of these schemes has been limited so far to milliseconds or more. Here we introduce a novel scheme that is orders of magnitude faster, capable of capturing complete spectral snapshots of WGM resonances at nanosecond timescales: cavity ring-up spectroscopy (CRUS). Based on sharply-rising detuned probe pulses, CRUS combines the sensitivity of heterodyne measurements with the highest possible, transform-limited acquisition rate. As a demonstration we capture spectra of microtoroid resonators at time intervals as short as 16 ns, directly monitoring sub-microsecond dynamics of their optomechanical vibrations, thermorefractive response and Kerr nonlinearity. CRUS holds promise for the study of fast biological processes such as enzyme kinetics, protein folding and light harvesting, with applications in other fields such as cavity QED and pulsed optomechanics.Comment: 6 pages, 4 figure

How single-photon nonlinearity is quenched with multiple quantum emitters: Quantum Zeno effect in collective interactions with Λ\Lambda-level atoms

Single-photon nonlinearity, namely the change in the response of the system as the result of the interaction with a single photon, is generally considered an inherent property of a single quantum emitter. Understanding the dependence of the nonlinearity on the number of emitters is important both fundamentally and practically, as strong light-matter coupling is more readily achieved through collective interactions than with a single emitter. Here, we theoretically consider a system that explores the transition from a single to multiple emitters with a $\Lambda$-level scheme. We show that the single-photon nonlinearity indeed vanishes with the number of emitters. Interestingly, the mechanism behind this behavior is the quantum Zeno effect, manifested in the slowdown of the photon-controlled dynamics.Comment: 6 pages, 4 figures + Supplementary material

Recovering quantum coherence of a cavity qubit through environment monitoring and active feedback

Decoherence in qubits, caused by their interaction with a noisy environment, poses a significant challenge to developing reliable quantum processors. Monitoring the qubit's environment enables not only to identify decoherence events but also to reverse these errors, thereby restoring the qubit coherence. This approach is particularly beneficial for superconducting cavity qubits, whose unavoidable interaction with auxiliary transmons impacts their coherence. In this work, we uncover the intricate dynamics of cavity decoherence by tracking the noisy trajectory of a transmon acting as the cavity's environment. Using real-time feedback, we successfully recover the lost coherence of the cavity qubit, achieving a fivefold increase in its dephasing time. Alternatively, by detecting transmon errors and converting them into erasures, we improve the cavity phase coherence by more than an order of magnitude. These advances are essential for implementing long-lived cavity qubits with high-fidelity gates and can enable more efficient bosonic quantum error correction codes.Comment: 17 pages, 10 figures, including supplementary informatio