74 research outputs found
Polaronic transport induced by competing interfacial magnetic order in a LaCaMnO/BiFeO heterostructure
Using ultrafast optical spectroscopy, we show that polaronic behavior
associated with interfacial antiferromagnetic order is likely the origin of
tunable magnetotransport upon switching the ferroelectric polarity in a
LaCaMnO/BiFeO (LCMO/BFO) heterostructure. This is
revealed through the difference in dynamic spectral weight transfer between
LCMO and LCMO/BFO at low temperatures, which indicates that transport in
LCMO/BFO is polaronic in nature. This polaronic feature in LCMO/BFO decreases
in relatively high magnetic fields due to the increased spin alignment, while
no discernible change is found in the LCMO film at low temperatures. These
results thus shed new light on the intrinsic mechanisms governing
magnetoelectric coupling in this heterostructure, potentially offering a new
route to enhancing multiferroic functionality
Softening of the insulating phase near Tc for the photo-induced insulator-to-metal phase transition in vanadium dioxide
We use optical-pump terahertz-probe spectroscopy to investigate the
near-threshold behavior of the photoinduced insulator-to-metal (IM) transition
in vanadium dioxide thin films. Upon approaching Tc a reduction in the fluence
required to drive the IM transition is observed, consistent with a softening of
the insulating state due to an increasing metallic volume fraction (below the
percolation limit). This phase coexistence facilitates the growth of a
homogeneous metallic conducting phase following superheating via
photoexcitation. A simple dynamic model using Bruggeman effective medium theory
describes the observed initial condition sensitivity.Comment: accepted for publication in Physical Review Letter
Coexistence of coupled magnetic phases in epitaxial TbMnO3 films revealed by ultrafast optical spectroscopy
Ultrafast optical pump-probe spectroscopy is used to reveal the coexistence
of coupled antiferromagnetic/ferroelectric and ferromagnetic orders in
multiferroic TbMnO3 films through their time domain signatures. Our
observations are explained by a theoretical model describing the coupling
between reservoirs with different magnetic properties. These results can guide
researchers in creating new kinds of multiferroic materials that combine
coupled ferromagnetic, antiferromagnetic and ferroelectric properties in one
compound.Comment: Accepted by Appl. Phys. let
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