Field-induced carrier delocalization in the strain-induced Mott insulating state of an organic superconductor

We report the influence of the field effect on the dc resistance and Hall coefficient in the strain-induced Mott insulating state of an organic superconductor $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Br. Conductivity obeys the formula for activated transport $\sigma_{\Box} = \sigma_{0}\exp(-W/k_{B}T)$, where $\sigma_{0}$ is a constant and $W$ depends on the gate voltage. The gate voltage dependence of the Hall coefficient shows that, unlike in conventional FETs, the effective mobility of dense hole carriers ($\sim1.6\times 10^{14}$ cm$^{-2}$) is enhanced by a positive gate voltage. This implies that carrier doping involves delocalization of intrinsic carriers that were initially localized due to electron correlation.Comment: 5 pages, 3 figure

Magnetic oscillations in a two-dimensional network of compensated electron and hole orbits

The FS of (ET)8Hg4Cl12(C6H5Br)2 can be regarded as a 2D network of compensated electron and hole orbits coupled by magnetic breakthrough. Simultaneous measurements of the interlayer magnetoresistance and magnetic torque have been performed up to 28 T. Magnetoresistance and de dHvA oscillations spectra exhibit frequency combinations typical of such a network. Even though some of the observed magnetoresistance oscillations cannot be interpreted on the basis of neither conventional SdH oscillations nor quantum interference, the temperature and magnetic field (both orientation and magnitude) dependence of all the Fourier components of the dHvA spectra can be consistently accounted for by the LK formula. This behaviour is at variance with that currently reported for compounds illustrating the linear chain of coupled orbits model.Comment: accepted for publication in europhysics Letter

Competing types of quantum oscillations in the 2D organic conductor (BEDT-TTF)8Hg4Cl12(C6H5Cl)2

Interlayer magnetoconductance of the quasi-two dimensional organic metal (BEDT-TTF)8Hg4Cl12(C6H5Cl)2 has been investigated in pulsed magnetic fields extending up to 36 T and in the temperature range from 1.6 to 15 K. A complex oscillatory spectrum, built on linear combinations of three basic frequencies only is observed. These basic frequencies arise from the compensated closed hole and electron orbits and from the two orbits located in between. The field and temperature dependencies of the amplitude of the various oscillation series are studied within the framework of the coupled orbits model of Falicov and Stachowiak. This analysis reveals that these series result from the contribution of either conventional Shubnikov-de Haas effect (SdH) or quantum interference (QI), both of them being induced by magnetic breakthrough. Nevertheless, discrepancies between experimental and calculated parameters indicate that these phenomena alone cannot account for all of the data. Due to its low effective mass, one of the QI oscillation series - which corresponds to the whole first Brillouin zone area - is clearly observed up to 13 K.Comment: 8 pages, 8 figures. To be published in Phys. Rev.

High frequency magnetic oscillations of the organic metal θ\theta-(ET)4_4ZnBr4_4(C6_6H4_4Cl2_2) in pulsed magnetic field of up to 81 T

De Haas-van Alphen oscillations of the organic metal $\theta$-(ET)$_4$ZnBr$_4$(C$_6$H$_4$Cl$_2$) are studied in pulsed magnetic fields up to 81 T. The long decay time of the pulse allows determining reliable field-dependent amplitudes of Fourier components with frequencies up to several kiloteslas. The Fourier spectrum is in agreement with the model of a linear chain of coupled orbits. In this model, all the observed frequencies are linear combinations of the frequency linked to the basic orbit $\alpha$ and to the magnetic-breakdown orbit $\beta$.Comment: 6 pages, 4 figure

Quantum oscillations in the linear chain of coupled orbits: the organic metal with two cation layers theta-(ET)(4)CoBr(4)(C(6)H(4)Cl(2))

Analytical formulae for de Haas-van Alphen (dHvA) oscillations in linear chain of coupled two-dimensional (2D) orbits (Pippard's model) are derived systematically taking into account the chemical potential oscillations in magnetic field. Although corrective terms are observed, basic (alpha) and magnetic breakdown-induced (beta and 2beta - alpha) orbits can be accounted for by the Lifshits-Kosevich (LK) and Falicov-Stachowiak semiclassical models in the explored field and temperature ranges. In contrast, the 'forbidden orbit' beta - alpha amplitude is described by a non-LK equation involving a product of two classical orbit amplitudes. Furthermore, strongly non-monotonic field and temperature dependence may be observed for the second harmonics of basic frequencies such as 2alpha and the magnetic breakdown orbit beta + alpha, depending on the value of the spin damping factors. These features are in agreement with the dHvA oscillation spectra of the strongly 2D organic metal theta- theta-(ET)(4)CoBr(4)(C(6)H(4)Cl(2)).Comment: to be published in Europhysics Letters (2012

Structure of the Fulde-Ferrell-Larkin-Ovchinnikov state in two-dimensional superconductors

Nonuniform superconducting state due to strong spin magnetism is studied in two-dimensional type-II superconductors near the second order phase transition line between the normal and the superconducting states. The optimum spatial structure of the orderparameter is examined in systems with cylindrical symmetric Fermi surfaces. It is found that states with two-dimensional structures have lower free energies than the traditional one-dimensional solutions, at low temperatures and high magnetic fields. For s-wave pairing, triangular, square, hexagonal states are favored depending on the temperature, while square states are favored at low temperatures for d-wave pairing. In these states, orderparameters have two-dimensional structures such as square and triangular lattices.Comment: 11 pages (LaTeX, revtex.sty), 3 figures; added reference

Different Types of Electron-Vibrational Interaction in BEDT-TTF Salts with Halide-Mercurate Anions Studied by IR Spectroscopy

Infrared optical properties of a large family of BEDT-TTF salts with mercury-halide anions are studied which exhibit different types of electron-vibrational spectra