291 research outputs found
Layer- and bulk roton excitations of 4He in porous media
We examine the energetics of bulk and layer-roton excitations of 4He in
various porous medial such as aerogel, Geltech, or Vycor, in order to find out
what conclusions can be drawn from experiments on the energetics about the
physisorption mechanism. The energy of the layer-roton minimum depends
sensitively on the substrate strength, thus providing a mechanism for a direct
measurement of this quantity. On the other hand, bulk-like roton excitations
are largely independent of the interaction between the medium and the helium
atoms, but the dependence of their energy on the degree of filling reflects the
internal structure of the matrix and can reveal features of 4He at negative
pressures. While bulk-like rotons are very similar to their true bulk
counterparts, the layer modes are not in close relation to two-dimensional
rotons and should be regarded as a third, completely independent kind of
excitation
Mixing Effects in the Crystallization of Supercooled Quantum Binary Liquids
By means of Raman spectroscopy of liquid microjets we have investigated the
crystallization process of supercooled quantum liquid mixtures composed of
parahydrogen (pH) diluted with small amounts of up to 5\% of either neon or
orthodeuterium (oD), and of oD diluted with either Ne or pH. We
show that the introduction of Ne impurities affects the crystallization
kinetics in both the pH-Ne and oD-Ne mixtures in terms of a significant
reduction of the crystal growth rate, similarly to what found in our previous
work on supercooled pH-oD liquid mixtures [M. K\"uhnel et {\it al.},
Phys. Rev. B \textbf{89}, 180506(R) (2014)]. Our experimental results, in
combination with path-integral simulations of the supercooled liquid mixtures,
suggest in particular a correlation between the measured growth rates and the
ratio of the effective particle sizes originating from quantum delocalization
effects. We further show that the crystalline structure of the mixture is also
affected to a large extent by the presence of the Ne impurities, which likely
initiate the freezing process through the formation of Ne crystallites.Comment: 19 pages, 7 figures, submitted to J. Chem. Phy
Interatomic Coulombic Decay following Photoionization of the Helium Dimer: Observation of Vibrational Structure
Using synchrotron radiation we simultaneously ionize and excite one helium
atom of a helium dimer (He_2) in a shakeup process. The populated states of the
dimer ion (i.e. He^[*+](n = 2; 3)-He) are found to deexcite via interatomic
coulombic decay. This leads to the emission of a second electron from the
neutral site and a subsequent coulomb explosion. In this letter we present a
measurement of the momenta of fragments that are created during this reaction.
The electron energy distribution and the kinetic energy release of the two He^+
ions show pronounced oscillations which we attribute to the structure of the
vibrational wave function of the dimer ion.Comment: 8 pages, 5 figure
Single photon double ionization of the helium dimer
We show that a single photon can ionize the two helium atoms of the helium
dimer in a distance up to 10 {\deg}A. The energy sharing among the electrons,
the angular distributions of the ions and electrons as well as comparison with
electron impact data for helium atoms suggest a knock-off type double
ionization process. The Coulomb explosion imaging of He_2 provides a direct
view of the nuclear wave function of this by far most extended and most diffuse
of all naturally existing molecules.Comment: 10 pages, 5 figure
Scattering length for helium atom-diatom collision
We present results on the scattering lengths of ^4He--^4He_2 and ^3He--^4He_2
collisions. We also study the consequence of varying the coupling constant of
the atom-atom interaction.Comment: Contribution to Proceedings of the International Workshop ``Critical
Stability of Few-Body Quantum Systems'' (Dresden, October 17--22, 2005
Nearest-neighbour distribution of distances in crystals from extended X-ray absorption fine structure
Extended X-ray absorption fine structure (EXAFS) is a powerful probe of the distribution of nearest-neighbour distances around selected atomic species. We consider here the effect of vibrational disorder in crystals. The potential of EXAFS for the accurate evaluation of the coefficient of bond thermal expansion and its temperature dependence is discussed, with the aim of stimulating and facilitating the comparison with the results from total scattering experiments. The meaning of the distribution asymmetry in crystals and its connection with the effective potential anharmonicity and the bond expansion is quantitatively explored by comparing the results for a number of different systems. The extent of the relative atomic vibrations perpendicular to the bond direction and the perpendicular to parallel anisotropy are correlated with the extent of lattice negative thermal expansion as well as with the ionic mobility in superionic crystals
Compact Cryogenic Source of Periodic Hydrogen and Argon Droplet Beams for Relativistic Laser-Plasma Generation
We present a cryogenic source of periodic streams of micrometer-sized
hydrogen and argon droplets as ideal mass-limited target systems for
fundamental intense laser-driven plasma applications. The highly compact design
combined with a high temporal and spatial droplet stability makes our injector
ideally suited for experiments using state-of-the-art high-power lasers in
which a precise synchronization between the laser pulses and the droplets is
mandatory. We show this by irradiating argon droplets with multi-Terawatt
pulses.Comment: To be published in Review of Scientific Instrument
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