One-dimensional transport in bundles of single-walled carbon nanotubes

We report measurements of the temperature and gate voltage dependence for individual bundles (ropes) of single-walled nanotubes. When the conductance is less than about e^2/h at room temperature, it is found to decrease as an approximate power law of temperature down to the region where Coulomb blockade sets in. The power-law exponents are consistent with those expected for electron tunneling into a Luttinger liquid. When the conductance is greater than e^2/h at room temperature, it changes much more slowly at high temperatures, but eventually develops very large fluctuations as a function of gate voltage when sufficiently cold. We discuss the interpretation of these results in terms of transport through a Luttinger liquid.Comment: 5 pages latex including 3 figures, for proceedings of IWEPNM 99 (Kirchberg

Measuring electron orbital magnetic moments in carbon nanotubes

The remarkable transport properties of carbon nanotubes (NTs) are determined by their unique electronic structure (1). The electronic states of a NT form one-dimensional electron and hole subbands which, in general, are separated by an energy gap (2,3). States near the energy gap are predicted to have a large orbital magnetic moment much larger than the Bohr magneton (4,5). The moment is due to electron motion around the NT circumference. This orbital magnetic moment is thought to play a role in the magnetic susceptibility of NTs (6-9) and the magneto-resistance observed in large multi-walled NTs (10-12). However, the coupling between magnetic field and the electronic states of an individual NT has not been experimentally quantified. We have made electrical measurements of relatively small diameter (2 - 5 nm) individual NTs in the presence of an axial magnetic field. We observe energy shifts of electronic states and the associated changes in subband structure. Our results quantitatively confirm predicted values for orbital magnetic moments in NTs.Comment: typos correcte

Ultrafast photocurrent measurement of the escape time of electrons and holes from carbon nanotube PN junction photodiodes

Ultrafast photocurrent measurements are performed on individual carbon nanotube PN junction photodiodes. The photocurrent response to sub-picosecond pulses separated by a variable time delay {\Delta}t shows strong photocurrent suppression when two pulses overlap ({\Delta}t = 0). The picosecond-scale decay time of photocurrent suppression scales inversely with the applied bias VSD, and is twice as long for photon energy above the second subband E22 as compared to lower energy. The observed photocurrent behavior is well described by an escape time model that accounts for carrier effective mass.Comment: 8 pages Main text, 4 Figure

Chemical doping of individual semiconducting carbon-nanotube ropes

We report the effects of potassium doping on the conductance of individual semiconducting single-walled carbon nanotube ropes. We are able to control the level of doping by reversibly intercalating and de-intercalating potassium. Potassium doping changes the carriers in the ropes from holes to electrons. Typical values for the carrier density are found to be ∼100–1000 electrons/μm. The effective mobility for the electrons is μeff∼20–60 cm2 V-1 s-1, a value similar to that reported for the hole effective mobility in nanotubes [R. Martel et al., Appl. Phys. Lett. 73, 2447 (1998)]

Transient absorption and photocurrent microscopy show hot electron supercollisions describe the rate-limiting relaxation step in graphene

Using transient absorption (TA) microscopy as a hot electron thermometer we show disorder-assisted acoustic-phonon supercollisions (SCs) best describes the rate-limiting relaxation step in graphene over a wide range of lattice temperatures ($T_l=$5-300 K), Fermi energies ($E_F=\pm0.35$ eV), and optical probe energies (~0.3 - 1.1 eV). Comparison with simultaneously collected transient photocurrent, an independent hot electron thermometer, confirms the rate-limiting optical and electrical response in graphene are best described by the SC-heat dissipation rate model, $H=A(T^3_e- T^3_l)$. Our data further shows the electron cooling rate in substrate supported graphene is twice as fast as in suspended graphene sheets, consistent with SC-model prediction for disorder.Comment: 6 pages, 5 figures. Nano Letters, 201

Dynamic nuclear polarization at the edge of a two-dimensional electron gas

We have used gated GaAs/AlGaAs heterostructures to explore nonlinear transport between spin-resolved Landau level (LL) edge states over a submicron region of two-dimensional electron gas (2DEG). The current I flowing from one edge state to the other as a function of the voltage V between them shows diode-like behavior---a rapid increase in I above a well-defined threshold V_t under forward bias, and a slower increase in I under reverse bias. In these measurements, a pronounced influence of a current-induced nuclear spin polarization on the spin splitting is observed, and supported by a series of NMR experiments. We conclude that the hyperfine interaction plays an important role in determining the electronic properties at the edge of a 2DEG.Comment: 8 pages RevTeX, 7 figures (GIF); submitted to Phys. Rev.