Superconductivity controlled bulk magnetism

Ferromagnetism's ability to influence superconducting order is well known and well established, but the converse phenomena remains relatively less explored. Theoretical work on the subject includes Anderson and Suhl prediction of a crypto-ferromagnetic state, and De Gennes proposal of two ferromagnetic insulators exchange coupled through a superconductor. In this study, we present compelling evidence of coexistence of both phenomena in a superconducting spin valve system. We demonstrate that superconducting exchange coupling enables reliable bistable states, and the coexistence of SEC and CFM leads to a wide range of reproducible zero field micro-magnetic states in the SSV, which are a function of the strength of the superconducting state. These micromagnetic states can in turn influence the superconducting state, leading to multiple reproducible and non-volatile resistance states; thus paving the way for a novel direction in cryogenic in-memory computing.Comment: 4 figure

Superconducting exchange coupling between ferromagnets.

Recent discoveries from superconductor (S)/ferromagnet (FM) heterostructures include π-junctions, triplet pairing, critical temperature (Tc) control in FM/S/FM superconducting spin valves (SSVs) and critical current control in S/FM/N/FM/S spin valve Josephson junctions (N: normal metal). In all cases, the magnetic state of the device, generally set by the applied field, controls the superconducting response. We report here the observation of the converse effect, that is, direct superconducting control of the magnetic state in GdN/Nb/GdN SSVs. A model for an antiferromagnetic effective exchange interaction based on the coupling of the superconducting condensation energy to the magnetic state can explain the Nb thickness and temperature dependence of this effect. This superconducting exchange interaction is fundamentally different in origin from the various exchange coupling phenomena that underlie conventional spin electronics (spintronics), and provides a mechanism for the active control of the magnetic state in superconducting spintronics.This work was supported by ERC AdG ‘Superspin’ and EPSRC Programme Grant EP/N017242/1.This is the author accepted manuscript. The final version is available from Nature Publishing Group at http://dx.doi.org/10.1038/nmat475

Large tuneable exchange fields due to purely paramagnetically limited domain wall superconductivity

The ability to locally apply and tune large magnetic fields is a crucial requirement for several devices, most notably for detection and generation of majorana fermions. Such a functionality can be achieved in Superconductor (S) /Ferromagnet (F) bilayers, where superconductivity is strengthened on top of domain walls due to local lowering of the proximity induced effective exchange fields. This is predicted to result in significant superconducting Tc enhancements and possible complete magnetic controlled switching on and off of the superconducting state. By using thin films of superconducting Nb and ferromagnetic insulating (GdN) bilayers, and through detailed magneto-transport measurements, we demonstrate the previously unobserved phenomena of complete switching in and out of the S state in S/F bilayers. In the thinnest of Nb layers, we estimate that the domain wall state induced tunability of proximity induced exchange fields can be as high as 1.3T with application of in plane external fields of only a few mT.Comment: 3 figure

Field-free Josephson diode with controllable efficiency using magnetic tunnel barrier

Josephson diodes (JDs) offer a promising route towards realizing dissipation-less rectification at low temperatures. To be practically viable, a JD must operate at zero magnetic fields, exhibit high operating frequencies and efficiency, and possess tunability and scalability. In this study, we propose and experimentally demonstrate a straightforward mechanism that encompasses all these crucial features. Our approach involves utilizing an asymmetric Josephson junction with a magnetic weak link to attain a diode effect in the switching current. We substantiate this concept experimentally through the fabrication of mesa-type sputter-deposited tri-layered ferromagnetic long NbN/GdN/NbN Josephson junctions (JJs) in cross geometry. A robust zero-field diode effect is observed with an efficiency boost of up to 40% achievable through modification of the micromagnetic structure of the barrier. Notably, these diodes maintain high efficiency across a wide temperature range, from the lowest temperatures up to at least 4.2K, and exhibit an operating frequency of nearly 28GHz

Triplet Cooper pairs induced in diffusive s-wave superconductors interfaced with strongly spin-polarized magnetic insulators or half-metallic ferromagnets.

Interfacing superconductors with strongly spin-polarized magnetic materials opens the possibility to discover new spintronic devices in which spin-triplet Cooper pairs play a key role. Motivated by the recent derivation of spin-polarized quasiclassical boundary conditions capable of describing such a scenario in the diffusive limit, we consider the emergent physics in hybrid structures comprised of a conventional s-wave superconductor (e.g. Nb, Al) and either strongly spin-polarized ferromagnetic insulators (e.g. EuO, GdN) or halfmetallic ferromagnets (e.g. CrO2, LCMO). In contrast to most previous works, we focus on how the superconductor itself is influenced by the proximity effect, and how the generated triplet Cooper pairs manifest themselves in the self-consistently computed density of states (DOS) and the superconducting critical temperature T c . We provide a comprehensive treatment of how the superconductor and its properties are affected by the triplet pairs, demonstrating that our theory can reproduce the recent observation of an unusually large zero-energy peak in a superconductor interfaced with a half-metal, which even exceeds the normal-state DOS. We also discuss the recent observation of a large superconducting spin-valve effect with a T c change ~1 K in superconductor/half-metal structures, in which case our results indicate that the experiment cannot be explained fully by a long-ranged triplet proximity effect

Superconducting exchange coupling between ferromagnets

Recent discoveries from superconductor (S)/ferromagnet (FM) heterostructures include π-junctions, triplet pairing, critical temperature (Tc) control in FM/S/FM superconducting spin valves (SSVs) and critical current control in S/FM/N/FM/S spin valve Josephson junctions (N: normal metal). In all cases, the magnetic state of the device, generally set by the applied field, controls the superconducting response. We report here the observation of the converse effect, that is, direct superconducting control of the magnetic state in GdN/Nb/GdN SSVs. A model for an antiferromagnetic effective exchange interaction based on the coupling of the superconducting condensation energy to the magnetic state can explain the Nb thickness and temperature dependence of this effect. This superconducting exchange interaction is fundamentally different in origin from the various exchange coupling phenomena that underlie conventional spin electronics (spintronics), and provides a mechanism for the active control of the magnetic state in superconducting spintronics.This work was supported by ERC AdG ‘Superspin’ and EPSRC Programme Grant EP/N017242/1.This is the author accepted manuscript. The final version is available from Nature Publishing Group at http://dx.doi.org/10.1038/nmat475

Spectroscopic evidence of odd frequency superconducting order

Spin filter superconducting S/I/N tunnel junctions (NbN/GdN/TiN) show a robust and pronounced Zero Bias Conductance Peak (ZBCP) at low temperatures, the magnitude of which is several times the normal state conductance of the junction. Such a conductance anomaly is representative of unconventional superconductivity and is interpreted as a direct signature of an odd frequency superconducting order

Low temperature characterization of high efficiency spin-filter Josephson junctions

The interplay between superconducting and ferromagnetic order pa¬rameters in S/F interfaces gives rise to a wide range of peculiar properties with applications in high-efficiency computation and in the emerging field of super¬conducting spintronics. In NbN/GdN/NbN Josephson junctions, GdN barriers give unique properties due to the double insulting and ferromagnetic nature of the material, as demonstrated in previous works. Here we focus on tunneling spectroscopy of these junctions down to 0.3 K when changing the barrier thick¬ness, which contributes to complete a consistent picture on the physics of these junctions and supports the previous indications of equal-spin Cooper pairs con¬tributing to the total supercurrent of the devices

Low temperature characterization of high efficiency spin-filter Josephson junctions

The interplay between superconducting and ferromagnetic order pa¬rameters in S/F interfaces gives rise to a wide range of peculiar properties with applications in high-efficiency computation and in the emerging field of super¬conducting spintronics. In NbN/GdN/NbN Josephson junctions, GdN barriers give unique properties due to the double insulting and ferromagnetic nature of the material, as demonstrated in previous works. Here we focus on tunneling spectroscopy of these junctions down to 0.3 K when changing the barrier thick¬ness, which contributes to complete a consistent picture on the physics of these junctions and supports the previous indications of equal-spin Cooper pairs con¬tributing to the total supercurrent of the devices