3,635 research outputs found
Orbital-selective Mass Enhancements in Multi-band CaSrRuO Systems Analyzed by the Extended Drude Model
We investigated optical spectra of quasi-two-dimensional multi-band CaSrRuO systems. The extended Drude model analysis on the
ab-plane optical conductivity spectra indicates that the effective mass should
be enhanced near . Based on the sum rule argument, we showed that the
orbital-selective Mott-gap opening for the bands, the widely
investigated picture, could not be the origin of the mass enhancement. We
exploited the multi-band effects in the extended Drude model analysis, and
demonstrated that the intriguing heavy mass state near should come from
the renormalization of the band.Comment: 4 figure
Epitaxial growth and the magnetic properties of orthorhombic YTiO3 thin films
High-quality YTiO3 thin films were grown on LaAlO3 (110) substrates at low
oxygen pressures (<10-8 Torr) using pulsed laser deposition. The in-plane
asymmetric atomic arrangements at the substrate surface allowed us to grow
epitaxial YTiO3 thin films, which have an orthorhombic crystal structure with
quite different a- and b-axes lattice constants. The YTiO3 film exhibited a
clear ferromagnetic transition at 30 K with a saturation magnetization of about
0.7 uB/Ti. The magnetic easy axis was found to be along the [1-10] direction of
the substrate, which differs from the single crystal easy axis direction, i.e.,
[001].Comment: 14 pages, 4 figure
Predictability of reset switching voltages in unipolar resistance switching
In unipolar resistance switching of NiO capacitors, Joule heating in the
conducting channels should cause a strong nonlinearity in the low resistance
state current-voltage (I-V) curves. Due to the percolating nature of the
conducting channels, the reset current IR, can be scaled to the nonlinear
coefficient Bo of the I-V curves. This scaling relationship can be used to
predict reset voltages, independent of NiO capacitor size; it can also be
applied to TiO2 and FeOy capacitors. Using this relation, we developed an error
correction scheme to provide a clear window for separating reset and set
voltages in memory operations
Dielectric constants of Ir, Ru, Pt, and IrO2: Contributions from bound charges
We investigated the dielectric functions () of Ir, Ru, Pt,
and IrO, which are commonly used as electrodes in ferroelectric thin film
applications. In particular, we investigated the contributions from bound
charges (), since these are important scientifically as
well as technologically: the (0) of a metal electrode is one of
the major factors determining the depolarization field inside a ferroelectric
capacitor. To obtain (0), we measured reflectivity spectra of
sputtered Pt, Ir, Ru, and IrO2 films in a wide photon energy range between 3.7
meV and 20 eV. We used a Kramers-Kronig transformation to obtain real and
imaginary dielectric functions, and then used Drude-Lorentz oscillator fittings
to extract (0) values. Ir, Ru, Pt, and IrO produced
experimental (0) values of 4810, 8210, 5810, and
295, respectively, which are in good agreement with values obtained using
first-principles calculations. These values are much higher than those for
noble metals such as Cu, Ag, and Au because transition metals and IrO have
such strong d-d transitions below 2.0 eV. High (0) values will
reduce the depolarization field in ferroelectric capacitors, making these
materials good candidates for use as electrodes in ferroelectric applications.Comment: 26 pages, 6 figures, 2 table
Finite-size scaling theory for explosive percolation transitions
The finite-size scaling (FSS) theory for continuous phase transitions has
been useful in determining the critical behavior from the size dependent
behaviors of thermodynamic quantities. When the phase transition is
discontinuous, however, FSS approach has not been well established yet. Here,
we develop a FSS theory for the explosive percolation transition arising in the
Erd\H{o}s and R\'enyi model under the Achlioptas process. A scaling function is
derived based on the observed fact that the derivative of the curve of the
order parameter at the critical point diverges with system size in a
power-law manner, which is different from the conventional one based on the
divergence of the correlation length at . We show that the susceptibility
is also described in the same scaling form. Numerical simulation data for
different system sizes are well collapsed on the respective scaling functions.Comment: 5 pages, 5 figure
Optical Study of the Free Carrier Response of LaTiO3/SrTiO3 Superlattices
We used infrared spectroscopic ellipsometry to investigate the electronic
properties of LaTiO3/SrTiO3 superlattices (SLs). Our results indicated that,
independent of the SL periodicity and individual layer-thickness, the SLs
exhibited a Drude metallic response with sheet carrier density per interface
~3x10^14 cm^-2. This is probably due to the leakage of d-electrons at
interfaces from the Mott insulator LaTiO3 to the band insulator SrTiO3. We
observed a carrier relaxation time ~ 35 fs and mobility ~ 35 cm^2V^-1s^-1 at 10
K, and an unusual temperature dependence of carrier density that was attributed
to the dielectric screening of quantum paraelectric SrTiO3.Comment: 4 pages, 4 figure
Bandwidth-Controlled Insulator-Metal Transition and Correlated Metallic State in 5 Transition Metal Oxides SrIrO (=1, 2, and )
We investigated the electronic structures of the 5 Ruddlesden-Popper
series SrIrO (=1, 2, and ) using optical
spectroscopy and first-principles calculations. As 5 orbitals are spatially
more extended than 3 or 4 orbitals, it has been widely accepted that
correlation effects are minimal in 5 compounds. However, we observed a
bandwidth-controlled transition from a Mott insulator to a metal as we
increased . In addition, the artificially synthesized perovskite SrIrO
showed a very large mass enhancement of about 6, indicating that it was in a
correlated metallic state
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