30 research outputs found
Cluster Spin Glass Distribution Functions in LaSrCuO
Signatures of the cluster spin glass have been found in a variety of
experiments, with an effective onset temperature that is frequency
dependent. We reanalyze the experimental results and find that they are
characterized by a distribution of activation energies, with a nonzero glass
transition temperature . While the distribution of activation
energies is the same, the distribution of weights depends on the process.
Remarkably, the weights are essentially doping independent.Comment: 5 pages, 5 ps figure
Recommended from our members
Electronic properties of LaO1-xFxFeAs in the normal state probed by nmr/nqr
We report 139La, 57Fe and 75As nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements on powders of the new LaO1−xFxFeAs superconductor for x=0 and 0.1 at temperatures up to 480 K, and compare our measured NQR spectra with local density approximation (LDA) calculations. For all three nuclei in the x=0.1 material, it is found that the local Knight shift increases monotonically with an increase in temperature, and scales with the macroscopic susceptibility, suggesting a single magnetic degree of freedom. Surprisingly, the spin lattice relaxation rates for all nuclei also scale with one another, despite the fact that the form factors for each site sample different regions of q-space. This result suggests a lack of any q-space structure in the dynamical spin susceptibility that might be expected in the presence of antiferromagnetic correlations. Rather, our results are more compatible with simple quasi-particle scattering. Furthermore, we find that the increase in the electric field gradient at the As cannot be accounted for by LDA calculations, suggesting that structural changes, in particular the position of the As in the unit cell, dominate the NQR response
Anomalous NMR Magnetic Shifts in CeCoIn_5
We report ^{115}In and ^{59}Co Nuclear Magnetic Resonance (NMR) measurements
in the heavy fermion superconductor CeCoIn_5 above and below T_c. The hyperfine
couplings of the In and Co are anisotropic and exhibit dramatic changes below
50K due to changes in the crystal field level populations of the Ce ions. Below
T_c the spin susceptibility is suppressed, indicating singlet pairing.Comment: 4 pages, 4 figure
Probing The Electronic Structure Of Pure And Doped Cem In5 (m=co,rh,ir) Crystals With Nuclear Quadrupolar Resonance
We report calculations of the electric-field gradients (EFGs) in pure and doped CeM In5 (M=Co, Rh, and Ir) compounds and compare with experiment. The degree to which the Ce4f electron is localized is treated within various models: the local-density approximation, generalized gradient approximation (GGA), GGA+U, and 4f -core approaches. We find that there is a correlation between the observed EFG and whether the 4f electron participates in the band formation or not. We also find that the EFG evolves linearly with Sn doping in CeRhIn5, suggesting the electronic structure is modified by doping. In contrast, the observed EFG in CeCoIn5 doped with Cd changes little with doping. These results indicate that nuclear quadrupolar resonance is a sensitive probe of electronic structure. © 2008 The American Physical Society.7724Slichter, C.P., (1990) Principles of Magnetic Resonance, , 3rd ed. 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Pressure Induced Change in the Magnetic Modulation of CeRhIn5
We report the results of a high pressure neutron diffraction study of the
heavy fermion compound CeRhIn5 down to 1.8 K. CeRhIn5 is known to order
magnetically below 3.8 K with an incommensurate structure. The application of
hydrostatic pressure up to 8.6 kbar produces no change in the magnetic wave
vector qm. At 10 kbar of pressure however, a sudden change in the magnetic
structure occurs. Although the magnetic transition temperature remains the
same, qm increases from (0.5, 0.5, 0.298) to (0.5, 0.5, 0.396). This change in
the magnetic modulation may be the outcome of a change in the electronic
character of this material at 10 kbar.Comment: 4 pages, 3 figures include
Charge order and low frequency spin dynamics in lanthanum cuprates revealed by Nuclear Magnetic Resonance
We report detailed 17O, 139La, and 63Cu Nuclear Magnetic Resonance (NMR) and
Nuclear Quadrupole Resonance (NQR) measurements in a stripe ordered
La1.875Ba0.125CuO4 single crystal and in oriented powder samples of
La1.8-xEu0.2SrxCuO4. We observe a partial wipeout of the 17O NMR intensity and
a simultaneous drop of the 17O electric field gradient (EFG) at low
temperatures where the spin stripe order sets in. In contrast, the 63Cu
intensity is completely wiped out at the same temperature. The drop of the 17O
quadrupole frequency is compatible with a charge stripe order. The 17O spin
lattice relaxation rate shows a peak similar to that of the 139La, which is of
magnetic origin. This peak is doping dependent and is maximal at x ~ 1/8.Comment: submitted to European Physical Journal Special Topic
Heat capacity studies of Ce and Rh site substitution in the heavy fermion antiferromagnet CeRhIn_5;: Short-range magnetic interactions and non-Fermi-liquid behavior
In heavy fermion materials superconductivity tends to appear when long range
magnetic order is suppressed by chemical doping or applying pressure. Here we
report heat capacity measurements on diluted alloyes of the heavy fermion
superconductor CeRhIn_5;. Heat capacity measurements have been performed on
CeRh_{1-y}Ir_{y}In_5; (y <= 0.10) and Ce_{1-x}La_{x}Rh_{1-y}Ir_{y}In_5; (x <=
0.50) in applied fields up to 90 kOe to study the affect of doping and magnetic
field on the magnetic ground state. The magnetic phase diagram of
CeRh_{0.9}Ir_{0.1}In_5; is consistent with the magnetic structure of CeRhIn_5;
being unchanged by Ir doping. Doping of Ir in small concentrations is shown to
slightly increase the antiferromagnetic transition temperature T_{N} (T_{N}=3.8
K in the undoped sample). La doping which causes disorder on the Ce sublattice
is shown to lower T_{N} with no long range order observed above 0.34 K for
Ce_{0.50}La_{0.50}RhIn_5;. Measurements on Ce_{0.50}La_{0.50}RhIn_5; show a
coexistence of short range magnetic order and non-Fermi-liquid behavior. This
dual nature of the Ce 4f-electrons is very similar to the observed results on
CeRhIn_5; when long range magnetic order is suppressed at high pressure.Comment: 8 pages, 9 figure
Magnetic structure of CeRhIn_5 as a function of pressure and temperature
We report magnetic neutron-diffraction and electrical resistivity studies on
single crystals of the heavy-fermion antiferromagnet CeRhIn at pressures
up to 2.3 GPa. These experiments show that the staggered moment of Ce and the
incommensurate magnetic structure change weakly with applied pressure up to
1.63 GPa, where resistivity, specific heat and NQR measurements confirm the
presence of bulk superconductivity. This work places new constraints on an
interpretation of the relationship between antiferromagnetism and
unconventional superconductivity in CeRhIn.Comment: 6 pages, 6 figures, submitted to Phys. Rev.
Structural and Magnetic Instabilities of LaSrCaCuO
A neutron scattering study of nonsuperconducting
LaSrCaCuO (x=0 and 0.2), a bilayer copper oxide without CuO
chains, has revealed an unexpected tetragonal-to-orthorhombic transition with a
doping dependent transition temperature. The predominant structural
modification below the transition is an in-plane shift of the apical oxygen. In
the doped sample, the orthorhombic superstructure is strongly disordered, and a
glassy state involving both magnetic and structural degrees of freedom develops
at low temperature. The spin correlations are commensurate.Comment: published versio