Instability of isolated triplet excitations on the Shastry-Sutherland lattice (SSL)

Configurations of singlets and triplets on the SSL have been proposed in the literature as variational ground states of the Shastry-Sutherland model at fixed magnetization M. We prove, that isolated triplet excitations on the SSL are unstable if the coupling alpha falls below a critical value alpha_c=2.0 (approx.). The instability should be visible in the compound SrCu_2(BO_3)_2 where a coupling alpha^*=1.48 is realized.Comment: 4 pages, 4 figures, RevTe

Low-Lying Magnetic Excitation of the Shastry-Sutherland Model

By using perturbation calculation and numerical diagonalization, low-energy spin dynamics of the Shastry-Sutherland model is investigated paying particular attention to the two-particle coherent motion. In addition to spin-singlet- and triplet bound states, we find novel branches of coherent motion of a bound quintet pair, which are usually unstable because of repulsion. Unusual dispersion observed in neutron-scattering measurements are explained by the present theory. The importance of the effects of phonon is also pointed out.Comment: 4 pages, 6 figures combined into 1 PSfile. Final version to appear in Phys.Rev.Lett. (Jan. 2000

Generalised Shastry-Sutherland Models in three and higher dimensions

We construct Heisenberg anti-ferromagnetic models in arbitrary dimensions that have isotropic valence bond crystals (VBC) as their exact ground states. The d=2 model is the Shastry-Sutherland model. In the 3-d case we show that it is possible to have a lattice structure, analogous to that of SrCu_2(BO_3)_2, where the stronger bonds are associated with shorter bond lengths. A dimer mean field theory becomes exact at d -> infinity and a systematic 1/d expansion can be developed about it. We study the Neel-VBC transition at large d and find that the transition is first order in even but second order in odd dimensions.Comment: Published version; slightly expande

Magnetization plateaus as insulator-superfluid transitions in quantum spin systems

We study the magnetization process in two-dimensional S=1/2 spin systems, to discuss the appearance of a plateau structure. The following three cases are considered: (1) the Heisenberg antiferromagnet and multiple-spin exchange model on the triangular lattice, (2) Shastry-Sutherland type lattice, [which is a possible model for SrCu2(BO3)2,] (3) 1/5-depleted lattice (for CaV4O9). We find in these systems that magnetization plateaus can appear owing to a transition from superfluid to a Mott insulator of magnetic excitations. The plateau states have CDW order of the excitations. The magnetizations of the plateaus depend on components of the magnetic excitations, range of the repulsive interaction, and the geometry of the lattice.Comment: 5 pages, RevTeX, 7 figures, note and reference adde

Quantum fluctuations in quantum lattice-systems with continuous symmetry

We discuss conditions for the absence of spontaneous breakdown of continuous symmetries in quantum lattice systems at $T=0$. Our analysis is based on Pitaevskii and Stringari's idea that the uncertainty relation can be employed to show quantum fluctuations. For the one-dimensional systems, it is shown that the ground state is invariant under the continuous transformation if a certain uniform susceptibility is finite. For the two- and three-dimensional systems, it is shown that truncated correlation functions cannot decay any more rapidly than $|r|^{-d+1}$ whenever the continuous symmetry is spontaneously broken. Both of these phenomena occur owing to quantum fluctuations. Our theorems cover a wide class of quantum lattice-systems having not-too-long-range interactions.Comment: 14 pages. To appear in J.Stat.Phy

Duality relations and exotic orders in electronic ladder systems

We discuss duality relations in correlated electronic ladder systems to clarify mutual relations between various conventional and unconventional phases. For the generalized two-leg Hubbard ladder, we find two exact duality relations, and also one asymptotic relation which holds in the low-energy regime. These duality relations show that unconventional (exotic) density-wave orders such as staggered flux or circulating spin-current are directly mapped to conventional density-wave orders, which establishes the appearance of various exotic states with time-reversal and/or spin symmetry breaking. We also study duality relations in the SO(5) symmetry that was proposed to unify antiferromagnetism and d-wave superconductivity. We show that the same SO(5) symmetry also unifies circulating spin current order and s-wave superconductivity.Comment: 9 pages, 2 figures; Proceedings of SPQS2004 (Sendai

Quantum melting of incommensurate domain walls in two dimensions

Quantum fluctuations of periodic domain-wall arrays in two-dimensional incommensurate states at zero temperature are investigated using the elastic theory in the vicinity of the commensurate-incommensurate transition point. Both stripe and honeycomb structures of domain walls with short-range interactions are considered. It is revealed that the stripes melt and become a stripe liquid in a large-wall-spacing (low-density) region due to dislocations created by quantum fluctuations. This quantum melting transition is of second order and characterized by the three-dimensional XY universality class. Zero-point energies of the stripe and honeycomb structures are calculated. As a consequence of these results, phase diagrams of the domain-wall solid and liquid phases in adsorbed atoms on graphite are discussed for various domain-wall masses. Quantum melting of stripes in the presence of long-range interactions that fall off as power laws is also studied. These results are applied to incommensurate domain walls in two-dimensional adsorbed atoms on substrates and in doped antiferromagnets, e.g. cuprates and nickelates.Comment: 11 pages, 5 figure

Low-Lying Excited States of Quantum Antiferromagnets on a Triangular Lattice

We study low-lying states of the XY and Heisenberg antiferromagnets on a triangular lattice to clarify whether spontaneous symmetry breaking occurs at $T=0$ in the thermodynamic limit. Approximate forms of low-lying states are proposed, in which degrees of freedom of the sublattice magnetization and of the chirality are separated. It is shown that low-lying states can be accurately described with the present approximation. It was argued that low-lying states play an important role in symmetry breaking. With help of this approximation, we discuss the contribution of low-lying states to symmetry breaking of two types, namely creation of the spontaneous sublattice magnetization and the spontaneous chirality. Furthermore, to show an evidence for the occurrence of the symmetry breaking, we numerically study the low-lying states of finite systems of the XY and Heisenberg antiferromagnets. It is found that the necessary conditions for the symmetry breaking to occur are satisfied in these models.Comment: LaTex 22 pages, figures included in uuencoded form, to be published in J.Stat.Phy

Two-Triplet-Dimer Excitation Spectra in the Shastry-Sutherland Model for SrCu_2(BO_3)_2

By using the perturbation expansion up to the fifth order, we study the two-triplet-dimer excitation spectra in the Shastry-Sutherland model, where the localized nature of a triplet-dimer, the propagation of a triplet-dimer pair by the correlated hopping and the long-range interactions between triplet-dimers play an essential role. It is found that the dispersion relations for first-neighbor triplet-dimer pair excitations with S=1 and p-type symmetry qualitatively explain the second-lowest branch observed in the neutron inelastic scattering experiment. It is also predicted that the second-lowest branch consists of two components, p_x- and p_y-states, with slightly different excitation energies. The origin of the singlet mode at 3.7meV observed in the Raman scattering experiment is also discussed.Comment: 5 pages, 3 figure