278 research outputs found
Superconducting coplanar waveguide resonators for low temperature pulsed electron spin resonance spectroscopy
We discuss the design and implementation of thin film superconducting
coplanar waveguide micro- resonators for pulsed ESR experiments. The
performance of the resonators with P doped Si epilayer samples is compared to
waveguide resonators under equivalent conditions. The high achievable filling
factor even for small sized samples and the relatively high Q-factor result in
a sensitivity that is superior to that of conventional waveguide resonators, in
particular to spins close to the sample surface. The peak microwave power is on
the order of a few microwatts, which is compatible with measurements at ultra
low temperatures. We also discuss the effect of the nonuniform microwave
magnetic field on the Hahn echo power dependence
Spin relaxation dynamics of radical-pair processes at low magnetic fields
We report measurements of room-temperature spin-relaxation times and
of charge-carrier spins in a -conjugated polymer thin film under
bipolar injection and low (1\mbox{ mT}\lesssim B_0\lesssim 10\mbox{ mT})
static magnetic fields, using electrically detected magnetic resonant Hahn-echo
and inversion-recovery pulse sequences. The experiments confirm the correlation
between the magnetic-field sensitive observables of radical-pair processes,
which include both the spin-dependent recombination currents in organic
semiconductors and the associated spin-relaxation times when random local
hyperfine fields and external magnetic fields compete in magnitude. Whereas a
striking field dependence of spin-lattice relaxation exists in the low-field
regime, the apparent spin decoherence time remains field independent as the
distinction between the two is lifted at low fields.Comment: Manuscript: 14 pages, 4 figures; Supplemental Material: 13 pages, 7
figure
Morphology effects on spin-dependent transport and recombination in polyfluorene thin films
We have studied the role of spin-dependent processes on conductivity in
polyfluorene (PFO) thin films by conducting continuous wave (c.w.) electrically
detected magnetic resonance (EDMR) spectroscopy at temperatures between 10 K
and 293 K using microwave frequencies between about 100 MHz and 20 GHz as well
as pulsed EDMR at X-band. Variable frequency EDMR allows us to establish the
role of spin-orbit coupling in spin-dependent processes, pulsed EDMR probes
coherent spin motion effects. We used PFO for this study in order to allow for
the investigation of the effects of microscopic morphological ordering since
this material can adopt two distinct intrachain morphologies: an amorphous
(glassy) phase, and an ordered (beta) phase. In thin films of organic
light-emitting diodes (OLEDs) the appearance of a particular phase can be
controlled by deposition parameters, and is verified by electroluminescence
spectroscopy. We conducted multi-frequency c.w. EDMR, electrically detected
Rabi spinbeat experiments, Hahn-echo and inversion-recovery measurements.
Coherent echo spectroscopy reveals electrically detected electron spin-echo
envelope modulation (ESEEM) due to the precession of the carrier spins around
the protons. Our results demonstrate that while conformational disorder can
influence the observed EDMR signals, including the sign of the current changes
on resonance as well as the magnitudes of local hyperfine fields and charge
carrier spin-orbit interactions, it does not qualitatively affect the nature of
spin-dependent transitions in this material. At 293 K and 10 K, polaron-pair
recombination through weakly spin-spin coupled intermediate charge carrier pair
states is dominant, while at low temperatures, additional signatures of
spin-dependent charge transport through the interaction of polarons with
triplet excitons are seen in the half-field resonance of a triplet spin-1
species.Comment: 27 pages, 2 tables, 11 figures, full abstract in articl
Three-photon electron spin resonances
We report the observation of a three-photon resonant transition of
charge-carrier spins in an organic light-emitting diode using electrically
detected magnetic resonance (EDMR) spectroscopy at room temperature. Under
strong magnetic-resonant drive (drive field ~ static magnetic field
), a -field swept EDMR line emerges when is approximately
threefold the one-photon resonance field. Ratios of drive-induced shifts of
this line to those of two- and one-photon shifts agree with analytical
expressions derived from the Floquet Hamiltonian and confirm the nature of
these three-photon transitions, enabling access of spin physics to a hitherto
inaccessible domain of quantum mechanics.Comment: 32 pages, 18 figure
The Society for Microelectronics -Annual Report 2003 Spin Relaxation in Si Quantum Wells Suppressed by an Applied Magnetic Field
We investigate spin properties of the two-dimensional electron gas in Si quantum wells defined by SiGe barriers. We find, in contrast to predictions of the classical model of D'yakonov-Perel, a strong anisotropy of spin relaxation and a decrease of the spin relaxation rate with increasing electron mobility. We show that for high electron mobility the cyclotron motion causes an additional modulation of spin-orbit coupling which leads to an effective suppression of spin relaxation rate. In spintronics, the aim is to make use of the spin degrees of freedom in addition to the electronic ones. Therefore, spintronic devices based on spins of carriers in semiconductors appear particularly promising. In such elements carriers can be easily moved by applying external voltages, the well known tool of classical electronics. The utilization of spin properties, however, usually is limited by the fast spin relaxation of conduction electrons. Therefore analysis of the spin relaxation mechanisms and the search for a suitable material and optimum conditions are of primary interest in this field. In III-V compounds the spin relaxation time is below one nanosecond [1]. Silicon based devices, due to much weaker spin-orbit coupling, appear much more promising. 2D Si layers in Si/SiGe structures exhibit a spin relaxation time of the order of a few microseconds by measurements of electron spin resonance (ESR) [2] - The effect of BR coupling on spin, σ, of a conduction electron can be described by an effective magnetic field, B BR . This field is oriented in-plane and perpendicular to electron momentum, ħk. The resulting zero field splitting is given by: The direction of the BR field depends on the direction of electron k-vector, and therefore the spread of k-vectors results in a spread of the BR field. Consequently, the ESR resonance is shifted and broadened. Momentum scattering, described by a rate 1/τ k , causes a modulation of the BR field in time which leads to the so called D'yakonovPerel (DP) spin relaxatio
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