Prediction of Orbital Ordering in Single-Layered Ruthenates

The key role of the orbital degree of freedom to understand the magnetic properties of layered ruthenates is here discussed. In the G-type antiferromagnetic phase of Ca$_2$RuO$_4$, recent X-ray experiments reported the presence of 0.5 hole per site in the $d_{xy}$ orbital, while the $d_{\rm yz}$ and $d_{zx}$ orbitals contain 1.5 holes. This unexpected $t_{2g}$ hole distribution is explained by a novel state with orbital ordering (OO), stabilized by a combination of Coulomb interactions and lattice distortions. In addition, the rich phase diagram presented here suggests the possibility of large magnetoresistance effects, and predicts a new ferromagnetic OO phase in ruthenates.Comment: 4 pages, Revtex, with 2 figures embedded in the text. Submitted to Phys. Rev. Let

Quasi-particle Density in Sr2RuO4 Probed by means of the Phonon Thermal Conductivity

The thermal conductivity of Sr2RuO4 along the least conducting direction perpendicular to the RuO2 plane has been studied down to 0.3 K. In this configuration the phonons remain the dominant heat carriers down to the lowest temperature, and their conductivity in the normal state is determined by the scattering on conduction electrons. We show that the phonon mean free path in the superconducting state is sensitive to the density of the quasi-particles in the bulk. An unusual magnetic field dependence of the phonon thermal conductivity is ascribed to the anisotropic superconducting gap structure in Sr2RuO4.Comment: 14 pages, 6 eps figures, Latex. This article corresponds to the reference 25 of Phys. Rev. Lett. vol.86 page2649-2652 (2001) and cond-mat/010449

Metamagnetic Quantum Criticality Revealed by 17O-NMR in the Itinerant Metamagnet Sr3Ru2O7

We have investigated the spin dynamics in the bilayered perovskite Sr3Ru2O7 as a function of magnetic field and temperature using 17O-NMR. This system sits close to a metamagnetic quantum critical point (MMQCP) for the field perpendicular to the ruthenium oxide planes. We confirm Fermi-liquid behavior at low temperatures except for a narrow field region close to the MMQCP. The nuclear spin-lattice relaxation rate divided by temperature 1/T1T is enhanced on approaching the metamagnetic critical field of 7.9 T and at the critical field 1/T1T continues to increase and does not show Fermi- liquid behavior down to 0.3 K. The temperature dependence of T1T in this region suggests the critical temperature Theta to be 0 K, which is a strong evidence that the spin dynamics possesses a quantum critical character. Comparison between uniform susceptibility and 1/T1T reveals that antiferromagnetic fluctuations instead of two-dimensional ferromagnetic fluctuations dominate the spin fluctuation spectrum at the critical field, which is unexpected for itinerant metamagnetism.Comment: 5 pages, 4 figures, Accepted by Phys. Rev. Let

Upper Critical Field of the 3 Kelvin Phase in Sr2RuO4

The inhomogeneous 3 Kelvin phase is most likely a superconducting state nucleating at the interface between micrometer-sized Ru-metal inclusions and Sr2RuO4 above the bulk onset of superconductivity. This filamentary superconducting state yields a characteristic temperature dependence of the upper critical field which is sublinear, i.e., H_{c2} (T) \propto (T^* - T)^{\gamma} with 0.5 \leq \gamma < 1 (T^*: nucleation temperature). The Ginzburg-Landau theory is used to analyze the behavior of the nucleated spin-triplet phase in a field and the characteristic features of H_{c2} observed in the experiment are explained based on a two-component order parameter in the presence of a filament of enhanced superconductivity with a finite width.Comment: 4 pages, 3 figure

Possibility of Macroscopic resonant Tunneling near the Superconductor- Insulator Transition in YBaCuO Thin Films

Experimental results of I-V characteristics near the superconductor-insulator transition observed for disorder-tuned YBaCuO thinfilms are presented. The I-V characteristics exibit new quasiperiodic structures as a function of the current. The current interval, the number of the dI/dV peaks, and the magnetic field dependence of the peaks are consistent with the theoretical predictions of the resonant tunneling of a phase particle ina tilted-cosine potential for asingle Josephson junction with small capacitance.Comment: 7 pages, 4 figures, in press (Europhys. Lett.

Muon-spin-relaxation and magnetic-susceptibility studies of effects of the magnetic impurity Ni on the Cu-spin dynamics and superconductivity in La_2-x_Sr_x_Cu_1-y_Ni_y_O_4_ with x = 0.13

Effects of the magnetic impurity Ni on the Cu-spin dynamics and superconductivity have been studied in La_2-x_Sr_x_Cu_1-y_Ni_y_O_4_ with x = 0.13 changing y finely up to 0.10. Compared with the case of the nonmagnetic impurity Zn, it has been found from the muon-spin-relaxation measurements that a large amount of Ni is required to stabilize a magnetic order of Cu spins. However, the evolution toward the stabilization of the magnetic order with increasing impurity concentration is qualitatively similar to each other. The area of the non-superconducting and slowly fluctuating or static region of Cu spins around Ni has been found to be smaller than that around Zn, suggesting that the pinning of rather long-ranged dynamical spin correlation such as the so-called dynamical stripe by Ni is weaker than that by Zn. This may be the reason why Zn destroys the superconductivity in the hole-doped high-T_c_ cuprates more markedly than Ni.Comment: 4 pages, 4 figures, accepted for publication in Phys. Rev.

Superconductivity in heavily boron-doped silicon carbide

The discoveries of superconductivity in heavily boron-doped diamond (C:B) in 2004 and silicon (Si:B) in 2006 renew the interest in the superconducting state of semiconductors. Charge-carrier doping of wide-gap semiconductors leads to a metallic phase from which upon further doping superconductivity can emerge. Recently, we discovered superconductivity in a closely related system: heavily-boron doped silicon carbide (SiC:B). The sample used for that study consists of cubic and hexagonal SiC phase fractions and hence this lead to the question which of them participates in the superconductivity. Here we focus on a sample which mainly consists of hexagonal SiC without any indication for the cubic modification by means of x-ray diffraction, resistivity, and ac susceptibility.Comment: 9 pages, 5 figure

Magnetic ordering in Sr2RuO4 induced by nonmagnetic impurities

We report unusual effects of nonmagnetic impurities on the spin-triplet superconductor Sr2RuO4. The substitution of nonmagnetic Ti4+ for Ru4+ induces localized-moment magnetism characterized by unexpected Ising anisotropy with the easy axis along the interlayer c direction. Furthermore, for x(Ti) > 0.03 magnetic ordering occurs in the metallic state with the remnant magnetization along the c-axis. We argue that the localized moments are induced in the Ru4+ and/or oxygen ions surrounding Ti4+ and that the ordering is due to their interaction mediated by itinerant Ru-4d electrons with strong spin fluctuations.Comment: 5 pages, 4figure