Double-electron ionization driven by inhomogeneous fields

Authors may self-archive the author’s accepted manuscript of their articles on their own websites. Authors may also deposit this version of the article in any repository, provided it is only made publicly available 12 months after official publication or later. He/ she may not use the publisher's version (the final article), which is posted on SpringerLink and other Springer websites, for the purpose of self-archiving or deposit. Furthermore, the author may only post his/her version provided acknowledgement is given to the original source of publication and a link is inserted to the published article on Springer's website. The link must be provided by inserting the DOI number of the article in the following sentence: “The final publication is available at Springer via https://link.springer.com/article/10.1007/s00340-017-6672-4"Electron–electron correlation effects play a crucial role in our understanding of sequential (SDI) and non-sequential double ionization (NSDI) mechanisms. Here, we present a theoretical study of NSDI driven by plasmonic-enhanced spatial inhomogeneous fields. By numerically solving the time-dependent Schrödinger equation for a linear reduced model of He and a double-electron time-evolution probability analysis, we provide evidence for enhancement effects in NSDI showing that the double ionization yield at lower laser peak intensities is increased due to the spatial inhomogeneous character of plasmonic-enhanced field. The change in the emission direction of the double-ion as a function of the field inhomogeneity degree demonstrates that plasmonic-enhanced fields could configure a reliable instrument to control the ion emission. Furthermore, our quantum mechanical model, as well as classical trajectory Monte Carlo simulations, show that inhomogeneous fields are as well as a useful tool for splitting the binary and recoil processes in the rescattering scenario.This work was supported by the project ELI-Extreme Light Infrastructure-phase 2 (Project No. CZ.02.1.01/0.0/0.0/ 15_008/0000162) from European Regional Development Fund, Spanish MINECO (National Plan grants FIS2011-30465-C02-01, FOQUS No. FIS2013-46768-P, FISICATEAMO FIS2016-79508-P and Severo Ochoa Excellence Grant No. SEV-2015-0522), the Generalitat de Catalunya (SGR 874 and CERCA/Program) and Fundació Privada Cellex Barcelona. N.S. was supported by the Erasmus Mundus Doctorate Program Europhotonics (Grant No. 159224-1-2009-1-FR-ERA MUNDUS-EMJD). N.S., A.C., and M.L. acknowledge ERC AdG OSYRIS, EU FETPRO QUIC and National Science Centre, Poland—Symfonia Grant 2016/20/W/ST4/00314. A. S. L. acknowledges Max Planck Center for Attosecond Science (MPC-AS). J. A. P.-H. acknowledges to the Spanish Ministerio de Economía y Competitivi- dad (FURIAM Project No. FIS2013-47741-R and PALMA project FIS2016- 81056-R) and Laserlab-Europe (EU-H2020 654148). L.O. acknowledges valuable input from Andre Staudte. The authors thankfully acknowledge the computer resources at MareNostrum, technical expertise and assistance provided by the Barcelona Supercomputing Center and the Red Española de Supercomputación (RES)Peer ReviewedPostprint (author's final draft

Fully differential cross sections in single ionization of helium by ion impact: Assessing the role of correlated wave functions

We study the effect of final state dynamic correlation in single ionization of atoms by ion impact analyzing fully differential cross sections (FDCS). We use a distorted wave model where the final state is represented by a Φ 2 type correlated function, solution of a non-separable three body continuum Hamiltonian. This final state wave function partially includes the correlation of electron-projectile and electron-recoil relative motion as coupling terms of the wave equation. A comparison of fully differential results using this model with other theories and experimental data reveals that inclusion of dynamic correlation effects have little influence on FDCS, and do not contribute to a better description of available data in the case of electronic emission out-of scattering plane.Fil: Ciappina, Marcelo Fabián. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Max Planck Institute for the Physics of Complex Systems; AlemaniaFil: Cravero, Walter Ruben. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Instituto de Física del Sur. Universidad Nacional del Sur. Departamento de Física. Instituto de Física del Sur; Argentin

Coherence and contextuality in scattering experiments

At a first sight, the description of a scattering experiment seems to be easy and unambiguous. A projectile, as for instance an electron or an ion, flies out of an accelerator with a given momentum p toward an atom or molecule, assumed to be at rest in the collision chamber, and interacts with it. This interaction might lead to different outcomes. For instance, the target might reach an excited bound state, or even loss an electron. These are only two examples of a myriad of options, which are usually called "channels". Thus, we can talk about the elastic channel, the excitation channel, the ionization channel, etc. Finally, one or some of the products of the collision are collected in order to investigate one of these channels.A closer look reveals that the description of any of these experiments is not quite as straight forward. More specifically, one major complication is that the Schrodinger equation is not analytically solvable for more than two mutually interacting particles, even when the underlying forces are precisely known. This is known as the few-body problem (FBP), which is formulated in the introduction to this book and theoretically discussed in other chapters. The FBP, in turn, is afflicted with an additional major complication which is usually overlooked. Addressing this drawback of the standard descriptions of the FBP is the main objective of the present chapter. Both the initial preparation of the projectiles and the final detection of the outgoing particles occur at macroscopic distances, and therefore it is assumed that they cannot have any effect on the scattering event, which occurs in a region of atomic dimensions. In other words, we might say that a scattering experiment is independent of its context. Furthermore, since both the beam of projectiles and the target gas can be described by pure quantum states, we are dealing with a purely coherent process.Unfortunately (or fortunately, depending on how each of us cope with uncertainties and broken paradigms), when we look deeper into this kind of experiments, we find out that they are trickier than expected. As we will discuss in the present chapter, all and every statement in the previous paragraph is false or at least doubtful. In what follows, we will discuss these issues, paying special attention to the assumption of coherence and lack of contextuality. But first, we will explore some basic ideas in very simple terms, which will pave the way for the discussion ahead.Fil: Barrachina Tejada, Raul Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro; ArgentinaFil: Navarrete, F.. Kansas State University; Estados UnidosFil: Ciappina, M.F.. Czech Academy of Sciences. Institute of Physics. ELI Beamlines; República ChecaFil: Schulz, Michael. Missouri University of Science and Technology. Department of Physics and LAMOR ; Estados Unido

Synthesis of ultrashort laser pulses for high-order harmonic generation

We present a technique for the synthesis of ultrashort laser pulses with approximately one cycle (FWHM) of temporal duration. These pulses are characterized by a certain degree of chirp. We show that these pulses produce both an enhancement of the high-order harmonic generation (HHG) cutoff and a noticeable increase of the yield, when interacting with an atomic system. Additionally, the asymmetric nature of the driven pulses plays an important role in the efficiency and cutoff extension of the high-order harmonics generated. Starting from the HHG spectra, we demonstrate it is possible to retrieve isolated attosecond pulses by spectral filtering. The analysis and interpretation of the different characteristics present in the HHG driven by this kind of pulse was carried out invoking classic arguments. Furthermore, a more complete description and validation of the HHG properties is performed by a quantum analysis, based on the integration of the time-dependent Schrödinger equation in full dimensionality.Fil: Neyra, Enrique Gustavo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Centro de Investigaciones Ópticas. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas. Centro de Investigaciones Ópticas. Universidad Nacional de La Plata. Centro de Investigaciones Ópticas; ArgentinaFil: Videla, Fabian Alfredo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Centro de Investigaciones Ópticas. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas. Centro de Investigaciones Ópticas. Universidad Nacional de La Plata. Centro de Investigaciones Ópticas; ArgentinaFil: Ciappina, Marcelo Fabián. Institute of Physics of the ASCR; República ChecaFil: Pérez Hernández, Javier Nicolás. Centro de Láseres Pulsados (CLPU); EspañaFil: Roso, L.. Centro de Láseres Pulsados (CLPU); EspañaFil: Torchia, Gustavo Adrian. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Centro de Investigaciones Ópticas. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas. Centro de Investigaciones Ópticas. Universidad Nacional de La Plata. Centro de Investigaciones Ópticas; Argentin

Double-electron ionization driven by inhomogeneous fields

Authors may self-archive the author’s accepted manuscript of their articles on their own websites. Authors may also deposit this version of the article in any repository, provided it is only made publicly available 12 months after official publication or later. He/ she may not use the publisher's version (the final article), which is posted on SpringerLink and other Springer websites, for the purpose of self-archiving or deposit. Furthermore, the author may only post his/her version provided acknowledgement is given to the original source of publication and a link is inserted to the published article on Springer's website. The link must be provided by inserting the DOI number of the article in the following sentence: “The final publication is available at Springer via https://link.springer.com/article/10.1007/s00340-017-6672-4"Electron–electron correlation effects play a crucial role in our understanding of sequential (SDI) and non-sequential double ionization (NSDI) mechanisms. Here, we present a theoretical study of NSDI driven by plasmonic-enhanced spatial inhomogeneous fields. By numerically solving the time-dependent Schrödinger equation for a linear reduced model of He and a double-electron time-evolution probability analysis, we provide evidence for enhancement effects in NSDI showing that the double ionization yield at lower laser peak intensities is increased due to the spatial inhomogeneous character of plasmonic-enhanced field. The change in the emission direction of the double-ion as a function of the field inhomogeneity degree demonstrates that plasmonic-enhanced fields could configure a reliable instrument to control the ion emission. Furthermore, our quantum mechanical model, as well as classical trajectory Monte Carlo simulations, show that inhomogeneous fields are as well as a useful tool for splitting the binary and recoil processes in the rescattering scenario.This work was supported by the project ELI-Extreme Light Infrastructure-phase 2 (Project No. CZ.02.1.01/0.0/0.0/ 15_008/0000162) from European Regional Development Fund, Spanish MINECO (National Plan grants FIS2011-30465-C02-01, FOQUS No. FIS2013-46768-P, FISICATEAMO FIS2016-79508-P and Severo Ochoa Excellence Grant No. SEV-2015-0522), the Generalitat de Catalunya (SGR 874 and CERCA/Program) and Fundació Privada Cellex Barcelona. N.S. was supported by the Erasmus Mundus Doctorate Program Europhotonics (Grant No. 159224-1-2009-1-FR-ERA MUNDUS-EMJD). N.S., A.C., and M.L. acknowledge ERC AdG OSYRIS, EU FETPRO QUIC and National Science Centre, Poland—Symfonia Grant 2016/20/W/ST4/00314. A. S. L. acknowledges Max Planck Center for Attosecond Science (MPC-AS). J. A. P.-H. acknowledges to the Spanish Ministerio de Economía y Competitivi- dad (FURIAM Project No. FIS2013-47741-R and PALMA project FIS2016- 81056-R) and Laserlab-Europe (EU-H2020 654148). L.O. acknowledges valuable input from Andre Staudte. The authors thankfully acknowledge the computer resources at MareNostrum, technical expertise and assistance provided by the Barcelona Supercomputing Center and the Red Española de Supercomputación (RES)Peer Reviewe

Attosecond spectroscopy using vacuum-ultraviolet pulses emitted from laser-driven semiconductors

International audienceStrongly laser-driven semiconductor crystals offer substantial advantages for the study of many-body physics and ultrafast optoelectronics via the high harmonic generation process. While this phenomenon has been employed to investigate the dynamics of solids in the presence of strong laser fields, its potential to be utilized as an attosecond light source has remained unexploited. Here, we demonstrate that the high harmonics generated through the interaction of mid--infrared pulses with a ZnO crystal leads to the production of attosecond pulses, that can be used to trace the ultrafast ionization dynamics of alkali metals. In a cross--correlation approach, we photoionize Cesium atoms with the vacuum-ultraviolet (VUV) high-harmonics in the presence of a mid-infrared laser field. We observe strong oscillations of the photoelectron yield originating from the instantaneous polarization of the atoms by the laser field. The phase of the oscillations encodes the attosecond synchronization of the ionizing high-harmonics and is used for attosecond pulse metrology. This light source opens a new spectral window for attosecond spectroscopy, paving the way for studies of systems with low ionization potentials including neutral atoms, molecules and solids. Additionally, our results highlight the significance of the source for generating non--classical massively entangled light states in the visible--VUV spectral region