39 research outputs found
Exchange interactions and Curie temperature in (GaMn)As
We use supercell and frozen-magnon approaches to study the dependence of the
magnetic interactions in (Ga,Mn)As on the Mn concentration. We report the
parameters of the exchange interaction between Mn spins and the estimates of
the Curie temperature within the mean-field and random-phase approximations. In
agreement with experiment we obtain a nonmonotonous dependence of the Curie
temperature on the Mn concentration. We estimate the dependence of the Curie
temperature on the concentration of the carries in the system and show that the
decrease of the number of holes in the valence band leads to fast decrease of
the Curie temperature. We show that the hole states of the valence band are
more efficient in mediating the exchange interaction between Mn spins than the
electron states of the conduction band
Electronic structure, exchange interactions and Curie temperature in diluted III-V magnetic semiconductors: (GaCr)As, (GaMn)As, (GaFe)As
We complete our earlier (Phys. Rev. B, {\bf 66}, 134435 (2002)) study of the
electronic structure, exchange interactions and Curie temperature in (GaMn)As
and extend the study to two other diluted magnetic semiconductors (GaCr)As and
(GaFe)As. Four concentrations of the 3d impurities are studied: 25%, 12.5%,
6.25%, 3.125%. (GaCr)As and (GaMn)As are found to possess a number of similar
features. Both are semi-metallic and ferromagnetic, with similar properties of
the interatomic exchange interactions and the same scale of the Curie
temperature. In both systems the presence of the charge carriers is crucial for
establishing the ferromagnetic order. An important difference between two
systems is in the character of the dependence on the variation of the number of
carriers. The ferromagnetism in (GaMn)As is found to be very sensitive to the
presence of the donor defects, like As antisites. On the other hand,
the Curie temperature of (GaCr)As depends rather weakly on the presence of this
type of defects but decreases strongly with decreasing number of electrons. We
find the exchange interactions between 3d atoms that make a major contribution
into the ferromagnetism of (GaCr)As and (GaMn)As and propose an exchange path
responsible for these interactions. The properties of (GaFe)As are found to
differ crucially from the properties of (GaCr)As and (GaMn)As. (GaFe)As does
not show a trend to ferromagnetism and is not half-metallic that makes this
system unsuitable for the use in spintronic semiconductor devices
Composite excitation of Josephson phase and spin waves in Josephson junctions with ferromagnetic insulator
Coupling of Josephson-phase and spin-waves is theoretically studied in a
superconductor/ferromagnetic insulator/superconductor (S/FI/S) junction.
Electromagnetic (EM) field inside the junction and the Josephson current
coupled with spin-waves in FI are calculated by combining Maxwell and
Landau-Lifshitz-Gilbert equations. In the S/FI/S junction, it is found that the
current-voltage (I-V) characteristic shows two resonant peaks. Voltages at the
resonant peaks are obtained as a function of the normal modes of EM field,
which indicates a composite excitation of the EM field and spin-waves in the
S/FI/S junction. We also examine another type of junction, in which a
nonmagnetic insulator (I) is located at one of interfaces between S and FI. In
such a S/I/FI/S junction, three resonant peaks appear in the I-V curve, since
the Josephson-phase couples to the EM field in the I layer.Comment: 16 pages, 5 figure
Exchange coupling in Eu monochalcogenides from first principles
Using a density functional method with explicit account for strong Coulomb
repulsion within the 4f shell, we calculate effective exchange parameters and
the corresponding ordering temperatures of the (ferro)magnetic insulating Eu
monochalcogenides (EuX; X=O,S,Se,Te) at ambient and elevated pressure
conditions. Our results provide quantitative account of the many-fold increase
of the Curie temperatures with applied pressure and reproduce well the
enhancement of the tendency toward ferromagnetic ordering across the series
from telluride to oxide, including the crossover from antiferromagnetic to
ferromagnetic ordering under pressure in EuTe and EuSe. The first and second
neighbor effective exchange are shown to follow different functional
dependencies. Finally, model calculations indicate a significant contribution
of virtual processes involving the unoccupied f states to the effective
exchange.Comment: 4 pages, 6 figure
The Kondo effect in ferromagnetic atomic contacts
Iron, cobalt and nickel are archetypal ferromagnetic metals. In bulk,
electronic conduction in these materials takes place mainly through the and
electrons, whereas the magnetic moments are mostly in the narrow
-electron bands, where they tend to align. This general picture may change
at the nanoscale because electrons at the surfaces of materials experience
interactions that differ from those in the bulk. Here we show direct evidence
for such changes: electronic transport in atomic-scale contacts of pure
ferromagnets (iron, cobalt and nickel), despite their strong bulk
ferromagnetism, unexpectedly reveal Kondo physics, that is, the screening of
local magnetic moments by the conduction electrons below a characteristic
temperature. The Kondo effect creates a sharp resonance at the Fermi energy,
affecting the electrical properties of the system;this appears as a Fano-Kondo
resonance in the conductance characteristics as observed in other artificial
nanostructures. The study of hundreds of contacts shows material-dependent
lognormal distributions of the resonance width that arise naturally from Kondo
theory. These resonances broaden and disappear with increasing temperature,
also as in standard Kondo systems. Our observations, supported by calculations,
imply that coordination changes can significantly modify magnetism at the
nanoscale. Therefore, in addition to standard micromagnetic physics, strong
electronic correlations along with atomic-scale geometry need to be considered
when investigating the magnetic properties of magnetic nanostructures.Comment: 7 pages, 5 figure
The onset of magnetic order in fcc-Fe films on Cu(100)
On the basis of a first-principles electronic structure theory of finite
temperature metallic magnetism in layered materials, we investigate the onset
of magnetic order in thin (2-8 layers) fcc-Fe films on Cu(100) substrates. The
nature of this ordering is altered when the systems are capped with copper.
Indeed we find an oscillatory dependence of the Curie temperatures as a
function of Cu-cap thickness, in excellent agreement with experimental data.
The thermally induced spin-fluctuations are treated within a mean-field
disordered local moment (DLM) picture and give rise to layer-dependent `local
exchange splittings' in the electronic structure even in the paramagnetic
phase. These features determine the magnetic intra- and interlayer interactions
which are strongly influenced by the presence and extent of the Cu cap.Comment: 13 pages, 3 figure
First-Principles Dynamical Coherent-Potential Approximation Approach to the Ferromagnetism of Fe, Co, and Ni
Magnetic properties of Fe, Co, and Ni at finite temperatures have been
investigated on the basis of the first-principles dynamical CPA (Coherent
Potential Approximation) combined with the LDA (Local Density Approximation) +
Hamiltonian in the Tight-Binding Linear Muffintin Orbital (TB-LMTO)
representation. The Hamiltonian includes the transverse spin fluctuation terms.
Numerical calculations have been performed within the harmonic approximation
with 4th-order dynamical corrections. Calculated single-particle densities of
states in the ferromagnetic state indicate that the dynamical effects reduce
the exchange splitting, suppress the band width of the quasi-particle state,
and causes incoherent excitations corresponding the 6 eV satellites. Results of
the magnetization vs temperature curves, paramagnetic spin susceptibilities,
and the amplitudes of local moments are presented. Calculated Curie
temperatures () are reported to be 1930K for Fe, 2550K for Co, and
620K for Ni; for Fe and Co are overestimated by a factor of 1.8,
while in Ni agrees with the experimental result. Effective Bohr
magneton numbers calculated from the inverse susceptibilities are 3.0 (Fe), 3.0 (Co), and 1.6 (Ni), being in
agreement with the experimental ones. Overestimate of in Fe and Co
is attributed to the neglects of the higher-order dynamical effects as well as
the magnetic short range order.Comment: 10 pages, 13 figure