1,363 research outputs found
Thermal conductivity of anisotropic spin - 1/2 two leg ladder:Green's function approach
We study the thermal transport of a spin-1/2 two leg antiferromagnetic ladder
in the direction of legs. The possible effect of spin-orbit coupling and
crystalline electric field are investigated in terms of anisotropies in the
Heisenberg interactions on both leg and rung couplings. The original spin
ladder is mapped to a bosonic model via a bond-operator transformation where an
infinite hard-core repulsion is imposed to constrain one boson occupation per
site. The Green's function approach is applied to obtain the energy spectrum of
quasi-particle excitations responsible for thermal transport. The thermal
conductivity is found to be monotonically decreasing with temperature due to
increased scattering among triplet excitations at higher temperatures. A tiny
dependence of thermal transport on the anisotropy in the leg direction at low
temperatures is observed in contrast to the strong one on the anisotropy along
the rung direction, due to the direct effect of the triplet density. Our
results reach asymptotically the ballistic regime of the spin - 1/2 Heisenberg
chain and compare favorably well with exact diagonalization data
Dynamics in the dimerised and high field incommensurate phase of CuGeO
Temperature (\ K) and magnetic field (\ T) dependent far
infrared absorption spectroscopy on the spin-Peierls coumpound CuGeO\ has
revealed several new absorption processes in both the dimerised and high field
phase of CuGeO. These results are discussed in terms of the modulation of
the CuGeO\ structure. At low fields this is the well known spin-Peierls
dimerisation. At high fields the data strongly suggests a field dependent
incommensurate modulation of the lattice as well as of the spin structure.Comment: 12 pages (revtex), 2 figures (eps), csh selfextracting .uu file, To
appear in PRB-Rapid Com
Origin of the ESR spectrum in the Prussian Blue analogue RbMn[Fe(CN)6]*H2O
We present an ESR study at excitation frequencies of 9.4 GHz and 222.4 GHz of
powders and single crystals of a Prussian Blue analogue (PBA),
RbMn[Fe(CN)6]*H2O in which Fe and Mn undergoes a charge transfer transition
between 175 and 300 K. The ESR of PBA powders, also reported by Pregelj et al.
(JMMM, 316, E680 (2007)) is assigned to cubic magnetic clusters of Mn2+ ions
surrounding Fe(CN)6 vacancies. The clusters are well isolated from the bulk and
are superparamagnetic below 50 K. In single crystals various defects with lower
symmetry are also observed. Spin-lattice relaxation broadens the bulk ESR
beyond observability. This strong spin relaxation is unexpected above the
charge transfer transition and is attributed to a mixing of the Mn3+ - Fe2+
state into the prevalent Mn2+ - Fe3+ state.Comment: 5 pages, 4 figures, submitted to PR
One-magnon Raman scattering in La(2)CuO(4): the origin of the field-induced mode
We investigate the one-magnon Raman scattering in the layered
antiferromagnetic La(2)CuO(4) compound. We find that the Raman signal is
composed by two one-magnon peaks: one in the B1g channel, corresponding to the
Dzyaloshinskii-Moryia (DM) mode, and another in the B3g channel, corresponding
to the XY mode. Furthermore, we show that a peak corresponding to the XY mode
can be induced in the planar (RR) geometry when a magnetic field is applied
along the easy axis for the sublattice magnetization. The appearance of such
field-induced mode (FIM) signals the existence of a new magnetic state above
the Neel temperature T_N, where the direction of the weak-ferromagnetic moment
(WFM) lies within the CuO(2) planes.Comment: 4 pages, 3 figure
Dynamics of spin and orbital phase transitions in YVO3
YVO3 exhibits a well separated sequence of orbital and spin order transitions
at 200 K and 116 K, followed by a combined spin-orbital reorientation at 77 K.
It is shown that the spin order can be destroyed by a sufficiently strong
optical pulse within less than 4 ps. In contrast, the orbital reordering
transition from C-type to G-type orbital order is slower than 100 ps and goes
via an intermediate nonthermal phase. We propose that the dynamics of phase
transitions is subjected to symmetry relations between the associated phases.Comment: 5 pages, 3 figure
Coherent amplitudon generation in K_0.3MoO_3 through ultrafast inter-band quasi particle decay
The charge density wave system K_0.3MoO_3 has been studied using variable
energy pump-probe spectroscopy, ellipsometry, and inelastic light scattering.
The observed transient reflectivity response exhibits quite a complex behavior,
containing contributions due to quasi particle excitations, coherent
amplitudons and phonons, and heating effects. The generation of coherent
amplitudons is discussed in terms of relaxation of photo-excited quasi
particles, and is found to be resonant with the interband plasmon frequency.
Two additional coherent excitations observed in the transients are assigned to
zone-folding modes of the charge density wave state
Photo-induced magnetization enhancement in two-dimensional weakly anisotropic Heisenberg magnets
By comparing the photo-induced magnetization dynamics in simple layered
systems we show how light-induced modifications of the magnetic anisotropy
directly enhance the magnetization. It is observed that the spin precession in
(CH3NH3)2CuCl4, initiated by a light pulse, increases in amplitude at the
critical temperature TC. The phenomenon is related to the dependence of the
critical temperature on the axial magnetic anisotropy. The present results
underline the possibility and the importance of the optical modifications of
the anisotropy, opening new paths toward the control of the magnetization state
for ultrafast memories.Comment: 5 pages, 3 figures, supplementary info as SIr.pd
Mapping the B,T phase diagram of frustrated metamagnet CuFeO2
The magnetic phase diagram of CuFeO2 as a function of applied magnetic field
and temperature is thoroughly explored and expanded, both for magnetic fields
applied parallel and perpendicular to the material's c-axis. Pulsed field
magnetization measurements extend the typical magnetic staircase of CuFeO2 at
various temperatures, demonstrating the persistence of the recently discovered
high field metamagnetic transition up to Tn2 ~ 11 K in both field
configurations. An extension of the previously introduced phenomenological spin
model used to describe the high field magnetization process (Phys. Rev. B, 80,
012406 (2009)) is applied to each of the consecutive low-field commensurate
spin structures, yielding a semi-quantitative simulation and intuitive
description of the entire experimental magnetization process in both relevant
field directions with a single set of parameters.Comment: 14 pages, 11 figures, submitted to Phys. Rev.
Evidence for differentiation in the iron-helicoidal-chain in GdFe(BO)
We report on a single-crystal X-ray structure study of
at room temperature and at T=90 K. At room temperature
crystallizes in a trigonal space group R32 (No. 155), the same as found for
other members of iron-borate family . At 90 K the
structure of has transformed to the space group
(No. 152). The low-temperature structure determination gives new
insight into the weakly first-order structural phase transition at 156 K and
into the related Raman phonon anomalies. The discovery of two inequivalent iron
chains in the low temperature structure provide new point of view on the
low-temperature magnetic properties.Comment: Subm. to Acta Cryst.
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